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We study the evaporation-induced stratification of a mixture of short and long polymer chains in a drying droplet using molecular simulations. We systematically investigate the effects of hydrodynamic interactions (HI) on this process by…

Soft Condensed Matter · Physics 2020-08-26 Michael P. Howard , Arash Nikoubashman

We present a coarse-grained lattice model to study the influence of water on the recognition process of two rigid proteins. The basic model is formulated in terms of the hydrophobic effect. We then investigate several modifications of our…

Biological Physics · Physics 2015-05-13 Johannes Taktikos , Hans Behringer

Recent studies of the hydration of micro- and nanoscale solutes have demonstrated a strong {\it coupling} between hydrophobic, dispersion and electrostatic contributions, a fact not accounted for in current implicit solvent models. We…

Chemical Physics · Physics 2009-11-11 J. Dzubiella , J. M. J. Swanson , J. A. McCammon

We have carried out experiments to probe the static and dynamic interfacial properties of $\beta$--casein monolayers spread at the air-buffer interface, and analysed these results in the context of models of weak polyampholytes.…

Soft Condensed Matter · Physics 2009-11-07 Pietro Cicuta , Ian Hopkinson

Infinite-layer nickelate superconductors have recently been discovered to share both similarities and differences with cuprate superconductors. Notably, the incorporation of hydrogen (H) through topotactic reduction has been found to play a…

Superconductivity · Physics 2023-07-25 Chenye Qin , Mi Jiang , Liang Si

Lipid bilayers forming biological membranes are known to behave as viscous 2D fluids on submicrometer scales; usually they contain a large number of active protein inclusions. Recently, it has been shown [Proc. Nat. Acad. Sci. USA 112,…

Soft Condensed Matter · Physics 2016-08-31 Yuki Koyano , Hiroyuki Kitahata , Alexander S. Mikhailov

Understanding solution-phase aggregation and dynamics in complex fluids is critical for material processing, yet widely used dynamic light scattering (DLS) fails for strongly attenuating systems such as conjugated polymers. We use X-ray…

The possibility to use sucrose solutions as medium for X-ray and neutron small-angle scattering experiments has been explored for dimyristoylphosphatidylcholine (DMPC) vesicles and mixed DMPC/C_(12)E_(8) aggregates. The influence of sucrose…

Biological Physics · Physics 2007-05-23 M. A. Kiselev , P. Lesieur , A. M. Kisselev , D. Lombardo , M. Killany , S. Lesieur

The stabilization of liquid biological products is a complex task that depends on the chemical composition of both the active ingredient and any excipients in solution. Frequently, a large number of unique excipients are required to…

Soft Condensed Matter · Physics 2024-07-02 Jonathan W. P. Zajac , Praveen Muralikrishnan , Caryn L. Heldt , Sarah L. Perry , Sapna Sarupria

How do solute concentration and molecular chemistry govern the transition from membrane saturation to destabilization? We address this using microsecond-scale molecular dynamics simulations of dipalmitoylphosphatidylcholine (DPPC) bilayers…

Soft Condensed Matter · Physics 2026-05-12 Anirban Polley

We report a high energy-resolution neutron backscattering study to investigate slow motions on nanosecond time scales in highly oriented solid supported phospholipid bilayers of the model system DMPC -d54 (deuterated…

Soft Condensed Matter · Physics 2007-05-23 Maikel C. Rheinstädter , Tilo Seydel , Franz Demmel , Tim Salditt

We present a probabilistic approach to water-water hydrogen bonding that allows one to obtain an analytic expression for the number of bonds per water molecule as a function of both its distance to a hydrophobic particle and hydrophobe…

Soft Condensed Matter · Physics 2013-03-20 Yuri S. Djikaev , Eli Ruckenstein

The molecular arrangement of lipids and proteins within biomembranes and monolayers gives rise to complex film morphologies as well as regions of distinct electrical surface potential, topographical and electrostatic nanoscale domains. To…

Soft Condensed Matter · Physics 2016-11-28 Elizabeth Drolle , W. F. D. Bennett , K. Hammond , Edward Lyman , Mikko Karttunen , Zoya Leonenko

We consider a solute-solvent-structure mutually coupled system of equations given by an Oldroyd-type model for a two-dimensional dilute corotational polymer fluid with solute diffusion and damping that is interacting with a one-dimensional…

Analysis of PDEs · Mathematics 2026-02-24 Prince Romeo Mensah

The associative interaction, such as hydrogen bonding, can bring about versatile functionalities to polymer systems, which has been investigated by tremendous researches, but the fundamental understanding on association process is still…

Soft Condensed Matter · Physics 2025-01-20 Xiangyu Zhang , Dong Meng

The hydrodynamic effects of macromolecular crowding inside cells is often studied in vitro by using polymers as crowding reagents. Confinement of polymers inside cell-sized droplets has been shown to affect the diffusion of small molecules.…

Soft Condensed Matter · Physics 2023-04-28 Yaam Deckel , Lauren A. Lowe , Siddharth Rawat , Matthew Turner , James Luong , Anna Wang

This paper presents a new solver developed in OpenFOAM for the modeling of lubricant in the narrow gap between two surfaces inducing hydrodynamic pressures up to few gigapascal. Cavitation is modeled using the homogeneous equilibrium model.…

Computational Engineering, Finance, and Science · Computer Science 2024-12-18 Nicolas Delaissé , Peyman Havaej , Dieter Fauconnier , Joris Degroote

An analytically solvable model of unsaturated lipid bilayer is derived by introducing finite bending angle of the unsaturated bond relative to straight part of the lipid chain considered previously in our model of semi-flexible strings. It…

Soft Condensed Matter · Physics 2024-07-18 Boris Kheyfets , Sergei Mukhin

The collapse and swelling behavior of a generic homopolymer is studied using implicit-solvent, explicit-cosolvent Langevin dynamics computer simulations for varying interaction strengths. The systematic investigation reveals that polymer…

Soft Condensed Matter · Physics 2012-11-06 Anja Muzdalo , Jan Heyda , Joachim Dzubiella

Aqueous solutions of LiCl are probably the most studied electrolyte solutions related to the complexity of liquid water at low temperatures. Despite the large amount of available experimental data hardly any computational studies were…

Soft Condensed Matter · Physics 2020-04-29 Philip H. Handle
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