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We photoionize nitrogen molecules with a train of extreme ultraviolet attosecond pulses together with a weak infrared field. We measure the phase of the two-color two-photon ionization transition (molecular phase) for different states of…

Attosecond ionization time-delays at photoelectron energies above typically 10 eV are usually interpreted using the so called asymptotic approximation as a sum of the atomic or molecular delays with a universal laser-induced contribution.…

In the semiclassical picture of photoionization process in intense laser fields, the ionization rate solely depends on the amplitude of the electric field and the final photoelectron momentum corresponds to the instant of ionization of the…

Atomic Physics · Physics 2019-05-09 Li Guo , Shilin Hu , Mingqing Liu , Zheng Shu , Xiwang Liu , Jie Li , Weifeng Yang , Ronghua Lu , Shensheng Han , Jing Chen

Characterizing the quantum state of intense light fields on sub-cycle timescales remains beyond the reach of existing methods. Here, we show that attosecond streaking provides direct, phase-sensitive access to the quantum properties of the…

Quantum Physics · Physics 2026-04-16 En-Rui Zhou , Yi-Jia Mao , Pei-Lun He , Feng He

The implementation of attosecond photoelectron-photoion coincidence spectroscopy for the investigation of atomic and molecular dynamics calls for a high-repetition-rate driving source combined with experimental setups characterized by…

Time-resolved studies have so far relied on rapidly triggering a photo-induced dynamic in chemical or biological ions or molecules and subsequently probing them with a beam of fast moving photons or electrons that crosses the studied…

Chemical Physics · Physics 2021-03-19 Hazem Daoud , R. J. Dwayne Miller

We demonstrate a Wiley-McClaren Time of Flight Mass Spectrometer modified to allow direct extraction of ions from a laser-induced plasma. Unlike many other methods that utilize mass spectrometry to investigate laser-induced plasmas, no…

Plasma Physics · Physics 2020-10-21 James O. F. Thompson , S. Tahereh Alavi , Justin R. Walensky , Arthur G. Suits

Recollision physics and attosecond pulse generation meld the precision of optics with collision physics. As a follow-up to our previous work, we reveal a new direction for the study of electronic structure and multielectron dynamics by…

Atomic Physics · Physics 2023-06-06 Chunmei Zhang , Graham G. Brown , Dong Hyuk Ko , Paul B. Corkum

This paper proposes a novel method to filter out the false alarm of LiDAR system by using the temporal correlation of target reflected photons. Because of the inevitable noise, which is due to background light and dark counts of the…

Instrumentation and Detectors · Physics 2017-08-22 Zhenchao Feng , Weiji He , Jian Fang , Guohua Gu , Qian Chen , Ping Zhang , Yuanjin Chen , Beibei Zhou , Minhua Zhou

This paper investigates the use of gravitational time delays of macro-lenses to constrain a possible photon mass. The time delay between the 2 compact images of a source of massive photons is computed. Explicit expressions are given for…

High Energy Astrophysical Phenomena · Physics 2017-12-06 J-F. Glicenstein

Resonant scattering of weak coherent laser pulses on a single two-level system (TLS) realized in a semiconductor quantum dot is investigated with respect to a time delay between incoming and scattered light. This type of time delay was…

We investigate attosecond time delays in the emission of photoelectrons using a hierarchy of models of the $CO_2$ molecule including the strong field approximation, Coulomb-scattering, short-range parts of the molecular potential, Hartree…

Atomic Physics · Physics 2021-03-30 Hakon Volkmann , Vinay P. Majety , Armin Scrinzi

The time-dependent variational principle is used to optimize the linear and nonlinear parameters of Gaussian basis functions to solve the time-dependent Schrodinger equation in 1 and 3 dimensions for a one-body soft Coulomb potential in a…

Determining the pulse duration of femtosecond electron bunches is challenging and often experimentally invasive. An effective method for measuring the duration based on the time-dependent variations in electron beam divergence induced by a…

Accelerator Physics · Physics 2025-07-01 Andreas Seidel , Carola Zepter , Alexander Sävert , Stephan Kuschel , Matt Zepf

Characterizing time delays in molecular photoionization as a function of the ejected electron emission direction relative to the orientation of the molecule and the light polarization axis pro-vides unprecedented insights into the…

We report a numerical calculation of the two-photon absorption coefficient of electrons in a binding potential using the real-time real-space higher-order difference method. By introducing random vector averaging for the intermediate state,…

Materials Science · Physics 2009-10-31 Yoshiyuki Kurokawa , Shintaro Nomura , Tadashi Takemori , Yoshinobu Aoyagi

Streaked photoemission metrology allows the observation of an apparent relative time delay between the detection of photoelectrons from different initial electronic states. This relative delay is obtained by recording the photoelectron…

Other Condensed Matter · Physics 2015-05-28 Chang-hua Zhang , Uwe Thumm

The method of H- photoionization is interesting for laser assisted charge exchange injection. In this paper, the model and computation of photoionization of negative hydrogen ion by using strong lasers is considered. The development of this…

Atomic Physics · Physics 2025-01-15 T. V. Gorlov , A. Aleksandrov , S. Cousineau , Y. Liu , A. Oguz , N. Evans

We present ionization probability and line shape calculations for the two-step 3-photon ionization process, $1S \stackrel{2\hbar \omega}{\longrightarrow}2S \stackrel{\hbar \omega}{\longrightarrow}\epsilon P $, of the ground state of…

Atomic Physics · Physics 2016-08-15 V Yakhontov , R. Santra , K. Jungmann

After photon absorption, electrons from a dispersive band of a solid require a finite time in the photoemission process before being photoemitted as free particles, in line with recent attosecondresolved photoemission experiments. According…

Mesoscale and Nanoscale Physics · Physics 2017-02-15 Mauro Fanciulli , Henrieta Volfová , Stefan Muff , Jürgen Braun , Hubert Ebert , Jan Minár , Ulrich Heinzmann , J. Hugo Dil
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