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Related papers: Extraction of attosecond time delay using the soft…

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We study real-time photoionization flux at the $3s$ Amusia-Cooper minimum (ACM) in argon using \textit{ab initio} simulations with the relativistic time-dependent configuration-interaction singles (RTDCIS) method in length (LG) and velocity…

Atomic Physics · Physics 2026-01-14 Rezvan Tahouri , Jan Marcus Dahlström

Photoelectron spectra obtained from the ab initio solution of the time-dependent Schr\"odinger equation can be in striking disagreement with predictions by the strong-field approximation (SFA) not only at low energy but also around twice…

Atomic Physics · Physics 2016-12-14 Th. Keil , S. V. Popruzhenko , D. Bauer

We develop a first-principles simulation method for attosecond time-resolved photoelectron spectroscopy. This method enables us to directly simulate the whole experimental processes, including excitation, emission and detection on equal…

Atomic Physics · Physics 2018-08-01 Shunsuke A. Sato , Hannes Hübener , Angel Rubio , Umberto De Giovannini

Time-delays in the photoionization of molecules are investigated. As compared to atomic ionization, the time-delays expected from molecular ionization present a much richer phenomenon, with a strong spatial dependence due to the anisotropic…

Atomic Physics · Physics 2017-02-14 P. Hockett , E. Frumker , D. M. Villeneuve , P. B. Corkum

More than 100 years after its discovery and its explanation in the energy domain, the duration of the photoelectric effect is still heavily studied. The emission time of a photoelectron can be quantified by the Wigner time delay.…

If matter absorbs a photon of sufficient energy it emits an electron. The question of the duration of the emission process has intrigued scientists for decades. With the advent of attosecond metrology, experiments addressing such ultrashort…

We revisit the time-resolved photoemission in neon atoms as probed by attosecond streaking. We calculate streaking time shifts for the emission of 2p and 2s electrons and compare the relative delay as measured in a recent experiment by…

We explore stimulated photo-association in the context of attosecond pump-probe schemes of atomic matter. An attosecond pulse -- the probe -- is used to induce photo-association of an electronic wave packet which had been created before,…

Atomic Physics · Physics 2009-11-13 Paula Rivière , Camilo Ruiz , Jan-Michael Rost

We report measurements of energy-dependent attosecond photoionization delays between the two outer-most valence shells of N$_2$O and H$_2$O. The combination of single-shot signal referencing with the use of different metal foils to filter…

Atomic Physics · Physics 2016-09-21 Martin Huppert , Inga Jordan , Denitsa Baykusheva , Aaron von Conta , Hans Jakob Wörner

We investigate the photoionization spectrum of helium by attosecond XUV pulses both in the spectral region of doubly excited resonances as well as above the double ionization threshold. In order to probe for convergence, we compare three…

We present a new method to estimate time delays from light curves of lensed quasars. The method is based on chi^2 minimization between the data and a numerical model light curve. A linear variation can be included in order to correct for…

Astrophysics · Physics 2007-05-23 I. Burud , P. Magain , S. Sohy , J. Hjorth

To measure and control the electron motion in atoms and molecules by the strong laser field on the attosecond time scale is one of the research frontiers of atomic and molecular photophysics. It involves many new phenomena and processes and…

Atomic Physics · Physics 2022-03-30 Chao Chen , Jiayin Che , Shang Wang , Guoguo Xin , Yanjun Chen

The photoionization of the CO molecule from the C$-1s$ orbital does not obey the Franck-Condon approximation, as a consequence of the nuclear recoil that accompanies the direct emission and intra-molecular scattering of the photoelectron.…

Atomic Physics · Physics 2021-11-24 Bejan Ghomashi , Nicolas Douguet , Luca Argenti

Electronic processes within atoms and molecules reside on the timescale of attoseconds. Recent advances in the laser-based pump-probe interrogation techniques have made possible the temporal resolution of ultrafast electronic processes on…

Atomic Physics · Physics 2024-02-16 Yongzhe Ma , Hongcheng Ni , Jian Wu

The use of semiclassical models based on the Strong Field Approximation (SFA) is ubiquitous in strong field multi-photon ionization and underlies many key developments in attosecond science, including the description of High Harmonic…

Photon exchange due to nuclear bremsstrahlung during nuclear collisions can cause Coulomb excitation in the projectile and the target nuclei. The corresponding process originated in nuclear timescales can also be observed in atomic…

We investigate an angular dependence of the photoemission time delay in helium as measured by the RABBITT (Reconstruction of Attosecond Beating By Interference of Two-photon Transitions) technique. The measured time delay $…

Atomic Physics · Physics 2016-05-17 I A Ivanov , J M Dahlström , E Lindroth , A S Kheifets

We report the experimental point-by-point sampling of the Wigner function for nonclassical states created in an ultrafast pulsed type-II parametric down-conversion source. We use a loss-tolerant time-multiplexed detector based on a…

Quantum Physics · Physics 2016-04-20 G. Harder , Ch. Silberhorn , J. Rehacek , Z. Hradil , L. Motka , B. Stoklasa , L. L. Sanchez-Soto

Ji \etal [New J. Phys. {\bf 26}, 093014 (2024)] established a direct link between the photoionization cross section and the attosecond time delay near Cooper minima (CM) in the valence shells of noble-gas atoms. This link is based on the…

Atomic Physics · Physics 2026-03-03 Adam J. C. Singor , Dmitry V. Fursa , Igor Bray , Anatoli S. Kheifets

Electrons in atoms and molecules can not react immediately to the action of intense laser field. A time lag (about 100 attoseconds) between instants of the field maximum and the ionization-rate maximum emerges. This lag characterizes the…

Atomic Physics · Physics 2021-04-01 J. Y. Che , C. Chen , S. Wang , G. G. Xin , Y. J. Chen