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Related papers: Evolution of magnetic interactions in a pressure-i…

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We report an extraordinary pressure dependence of the magnetic interactions in the metal-organic system [(CuF$_2$(H$_2$O)$_2$)$_2$pyrazine]. At zero pressure, this material realizes a quasi-two-dimensional (Q2D) spin-1/2 square-lattice…

Metal organic magnets have enormous potential to host a variety of electronic and magnetic phases that originate from a strong interplay between the spin, orbital and lattice degrees of freedom. We control this interplay in the quantum…

Strongly Correlated Electrons · Physics 2017-08-14 M. Skoulatos , M. Månsson , C. Fiolka , K. W. Krämer , J. Schefer , J. S. White , Ch. Rüegg

Cu(pz)2(ClO4)2 (with pz denoting pyrazine, C4H4N2) is among the best realizations of a two-dimensional spin-1/2 square-lattice antiferromagnet. Below T_N = 4.21 K, its weak interlayer couplings induce a 3D magnetic order, strongly…

Strongly Correlated Electrons · Physics 2016-02-29 N. Barbero , T. Shiroka , C. P. Landee , M. Pikulski , H. -R. Ott , J. Mesot

The low-doped magnetic perovskite La_{7/8}Sr_{1/8}MnO_3 undergoes within the paramagnetic-semiconducting phase a first-order structural transition due to antiferrodistorsive ordering of Jahn-Teller deformed MnO_6 octahedra. This allows to…

Strongly Correlated Electrons · Physics 2009-10-31 P. Wagner , I. Gordon , S. Mangin , V. V. Moshchalkov , Y. Bruynseraede , L. Pinsard , A. Revcolevschi

Using dc and ac magnetometry, the pressure dependence of the magnetization of the three-dimensional antiferromagnetic coordination polymer Mn(N(CN)$_{2}$)$_{2}$ was studied up to 12 kbar and down to 8K. The magnetic transition temperature,…

Materials Science · Physics 2015-02-03 P. A. Quintero , D. Rajan , M. K. Peprah , T. V. Brinzari , R. S. Fishman , D. R. Talham , M. W. Meisel

The high-pressure behaviour of Na$_2$CuF$_4$ is explored by powder neutron diffraction and density functional theory (DFT) calculations. A first-order phase transition is observed to take place between 2.4 - 2.9 GPa, involving a…

Pulsed-field magnetization experiments (fields $B$ of up to 85 T and temperatures $T$ down to 0.4 K) are reported on nine organic Cu-based two-dimensional (2D) Heisenberg magnets. All compounds show a low-$T$ magnetization that is concave…

We present an investigation of the effect of randomizing exchange strengths in the $S=1/2$ square lattice quasi-two-dimensional quantum Heisenberg antiferromagnet (QuinH)$_2$Cu(Cl$_{x}$Br$_{1-x}$)$_{4}\cdot$2H$_2$O (QuinH$=$Quinolinium,…

We present the results of a muon-spin relaxation (muSR) investigation into magnetic ordering in several families of layered quasi-two-dimensional molecular antiferromagnets based on transition metal ions such as S=1/2 Cu2+ bridged with…

Ferroelectric control of altermagnetism in momentum space has been studied widely, while the control of magnetism in real space of altermagnets are still rare. We present a design rule to identify multiferroicity in n=2 Ruddlesden-Popper…

Materials Science · Physics 2025-08-20 Ying Zhou , Hui-Min Zhang , Cheng-Ao Ji , Hongjun Xiang , Shuai Dong , James M. Rondinelli , Xue-Zeng Lu

Using density functional theory (DFT) with local density approximation (LDA) and generalized gradient approximation (GGA) correlation functionals, the electronic and magnetic structures of cubic BaFeO$_{3}$ in the ferromagnetic (FM) and…

Materials Science · Physics 2013-10-15 Gul Rahman , Juliana M. Morbec , Rubén Ferradás , Víctor M. García-Suárez

In the heavy-fermion system $Yb_2Pd_2In_{1-x}Sn_x$, the interplay of crystal-field splitting, Kondo effect, and Ruderman-Kittel-Kasuya-Yosida interactions leads to complex chemical-, pressure-, and magnetic-field phase diagrams, still to be…

We use first-principles theory to predict that the application of uniaxial compressive strain leads to a transition from an antiferromagnetic insulator to a ferromagnetic half-metal phase in LaMnO$_3$. We identify the Q2 Jahn-Teller mode as…

Materials Science · Physics 2016-03-23 Pablo Rivero , Vincent Meunier , William Shelton

We have studied the temperature dependence of crystal and magnetic structures of the Jahn-Teller distorted transition metal difluorides CrF$_2$ and CuF$_2$ by neutron powder diffraction in the temperature range 2-280 K. The lattice…

Strongly Correlated Electrons · Physics 2012-07-03 Tapan Chatterji , Thomas C. Hansen

We report results of magnetization and $^{31}$P NMR measurements under high pressure up to 6.4~GPa on RbMoOPO$_4$Cl, which is a frustrated square-lattice antiferromagnet with competing nearest-neighbor and next-nearest-neighbor…

Strongly Correlated Electrons · Physics 2021-03-10 Hikaru Takeda , Touru Yamauchi , Masashi Takigawa , Hajime Ishikawa , Zenji Hiroi

We investigate the properties of CuVOF$_4$(H$_2$O)$_6$$\cdot$H$_2$O, in which two different spin species, Cu(II) and V(IV), form antiferromagnetic spin-1/2 dimers with weak interdimer coupling provided via hydrogen bonding. Using…

Our experimental (neutron diffraction, M\"ossbauer spectroscopy, magnetic susceptibility, specific heat) and numerical studies on the evolution of short- and long-range magnetic order in $\gamma_{\rm II}$-Li\(_2\)FeSiO\(_4\) suggest a…

Strongly Correlated Electrons · Physics 2025-01-20 W. Hergett , N. Bouldi , M. Jonak , C. Neef , C. Ritter , M. Abdel-Hafiez , F. Seewald , H. -H. Klauss , M. W. -Haverkort , R. Klingeler

Measurements of magnetic susceptibility, heat capacity and thermal expansion are reported for single crystalline CuSb$_{2}$O$_{6}$ in the temperature range $5<T<350$ K. The magnetic susceptibility exhibits a broad peak centered near 60 K…

Strongly Correlated Electrons · Physics 2015-06-16 A. Rebello , M. G. Smith , J. J. Neumeier , B. D. White , Yi-Kuo Yu

We report a detailed $\mu$SR study of the pressure evolution of the magnetic order in the manganese based pnictide MnP, which has been recently found to undergo a superconducting transition under pressure once the magnetic ground state is…

Superconductivity · Physics 2016-06-01 R. Khasanov , A. Amato , P. Bonfà , Z. Guguchia , H. Luetkens , E. Morenzoni , R. De Renzi , N. D. Zhigadlo

It was discovered in La1-xSrxMnO3(x~1/8) that a field induced phase transition occurs from a ferromagnetic metal(FM) phase to a ferromagnetic insulator (FI) phase. The magnetization shows a sharp jump at the transition field accompanying…

Strongly Correlated Electrons · Physics 2016-08-31 H. Nojiri , K. Kaneko , M. Motokawa , K. Hirota , K. Takahashi , Y. Endoh
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