Related papers: Observation of Intense Second Harmonic Generation …
We develop a multipolar theory of second-harmonic generation (SHG) by dielectric nanoparticles made of noncentrosymmetric materials with bulk quadratic nonlinearity. We specifically analyze two regimes of optical excitation: illumination by…
An overview is given of recent advances in experimental and theoretical understanding of optical properties of ultra-thin crystal structures (graphene, phosphorene, silicene, MoS2, MoSe2 , WS2 , WSe2 , h-AlN, h-BN, fluorographene,…
We investigate the generation of ultraviolet (UV) second-harmonic radiation on the boundary of a UV transparent crystal, which is derived from the automatic partial phase matching of the incident wave and the total internal reflection. By…
In moir\'e crystals resulting from the stacking of twisted two-dimensional (2D) layered materials, a subtle adjustment in the twist angle surprisingly gives rise to a wide range of correlated optical and electrical properties. Herein, we…
The study of graphene, since its discovery around 2004, is possibly the largest and fastest growing field of research in material science, because of its exotic mechanical, thermal, electronic, optical and chemical properties. The studies…
Deeply sub-wavelength two-dimensional films may exhibit extraordinarily strong nonlinear effects. Here we show that 2D films exhibit the remarkable property of a phase-controllable nonlinearity, i.e., the amplitude of the nonlinear…
The field of two-dimensional materials has been developing at an impressive pace, with atomically thin crystals of an increasing number of different compounds that have become available, together with techniques enabling their assembly into…
Second-order nonlinear optical processes are fundamental to photonics, spectroscopy, and information technologies, with material platforms playing a pivotal role in advancing these applications. Here, we demonstrate the exceptional…
We show that spatially structured radiation generates second harmonic in a two-dimensional system even if the system is homogeneous and isotropic. The effect originates from non-locality of electric response to structured electromagnetic…
Extreme intensity contrast is considered essential for ultraintense, femtosecond laser excitation of solid targets, in particular for studies with structured or ultra-thin targets. Second-harmonic generation has been used to maximize the…
We report about the experimental observation and characterization of nonlinear optical properties of individual silicon nanowires of different dimensions. Our results show that the nonlinear light has different components, one of them…
While two-dimensional (2D) materials have intriguing second-order nonlinearities with ultrahigh coefficient and electrical tunability, their atomic layer thicknesses hinder explorations of other optical frequency-conversions (OFCs) than…
Collective modes of doped two-dimensional crystalline materials, namely graphene, MoS$_2$ and phosphorene, both monolayer and bilayer structures, are explored using the density functional theory simulations together with the random phase…
Phosphorene is a new family member of two-dimensional materials. We observed strong and highly layer-dependent photoluminescence in few-layer phosphorene (2 to 5 layers). The results confirmed the theoretical prediction that few-layer…
Spectroscopies utilizing free electron beams as probes offer detailed information on the reciprocal-space excitations of 2D materials such as graphene and transition metal dichalcogenide monolayers. Yet, despite the attention paid to such…
Hyperbolic plasmonic metamaterials provide numerous opportunities for designing unusual linear and nonlinear optical properties. We show that the modal overlap of fundamental and second-harmonic light in an anisotropic plasmonic…
We show that a dimer made of two gold nanospheres exhibits a remarkable efficiency for second-harmonic generation under femtosecond optical excitation. The detectable nonlinear emission for the given particle size and excitation wavelength…
Second harmonic (SH) radiation can only be generated in non-centrosymmetric bulk crystals under the electric-dipole approximation. Nonlinear thin films made from bulk crystals are technologically challenging because of complex and high…
We report on theoretical study of second harmonic generation in graphene. Phenomenological analysis based on symmetry arguments is carried out. It is demontrated, that in ideal graphene samples second harmonic generation is possible only if…
A comparative experimental investigation of the dependence of second harmonic generation (SHG) on applied external voltage between the standard nematic liquid crystalline material and an analogue ferromagnetic nematic liquid crystalline…