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Material systems with lone-pair electrons have long been a treasure trove in the search for large second harmonic generation effects. Revealing the origin of second harmonic generation in nonlinear optical materials can provide theoretical…

Materials Science · Physics 2025-05-13 Fuming Li , Shilie Pan , Zhihua Yang

Efficient nonlinear wave mixing is of paramount importance for a wide range of applications. However, weak optical nonlinearities pose significant challenges for accessing nonlinear light-matter interaction in compact systems. Here, we…

The success of isolating small flakes of atomically thin layers through mechanical exfoliation has triggered enormous research interest in graphene and other two-dimensional materials. For device applications, however, controlled large-area…

Materials Science · Physics 2014-07-17 Yingnan Liu , Rudresh Ghosh , Di Wu , Ariel Ismach , Rodney Ruoff , Keji Lai

Rigorous electrodynamical simulations based on the nonlinear Drude model are performed to investigate the influence of strong coupling on high harmonic generation by periodic metal gratings. It is shown that a thin dispersive material with…

Mesoscale and Nanoscale Physics · Physics 2019-08-13 Elena Drobnyh , Ruth Pachter , Maxim Sukharev

A comprehensive study of second harmonic generation on thermally oxidized MoS2 flakes with thickness ranging from monolayer up to seven layers is presented. Observing the fundamental nonlinear behavior for non-treated and oxidized MoS2…

Janus transition metal dichalcogenides are an emerging class of atomically thin materials with engineered broken mirror symmetry that gives rise to long-lived dipolar excitons, Rashba splitting, and topologically protected solitons. They…

Second-harmonic emission at a frequency that is twice the laser frequency is an important diagnostic for nonlinear laser-plasma interaction. It is forbidden for centrosymmetric materials such as the bulk of sapphire. The symmetry, however,…

Silica-based optical fibers are a workhorse of nonlinear optics. They have been used to demonstrate nonlinear phenomena such as solitons and self-phase modulation. Since the introduction of the photonic crystal fiber, they have found many…

Intense laser-driven nonlinear optical phenomena in two-dimensional (2D) nodal-line semimetals (NLS) exhibit complex mechanisms, particularly in the NbSi$_{x}$Te$_{2}$ material systems characterized by nonsymmorphic symmetry-protected band…

Optics · Physics 2025-08-25 Navdeep Rana , M. S. Mrudul , Amar Bharti , Sucharita Giri , Gopal Dixit

Lattice {\em Kirigami}, ultra-light metamaterials, poly-disperse aggregates, ceramic nano-lattices, and two-dimensional (2-D) atomic materials share an inherent structural discreteness, and their material properties evolve with their shape.…

The nonlinear properties of a metamaterial sample composed of double-layer metallic patterns and voltage controllable diodes are experimentally investigated. Second harmonics and spectrum modulations are clearly observed in a wide band of…

Nonlinear second harmonic optical activity of graphene covering a gold photon sieve was determined for different polarizations. The photon sieve consists of a subwavelength gold nanohole array placed on glass. It combines the benefits of…

Mesoscale and Nanoscale Physics · Physics 2016-01-14 Michael Lobet , Michael Sarrazin , Francesca Cecchet , Nicolas Reckinger , Alexandru Vlad , Jean-François Colomer , Dan Lis

The efficient optical second-harmonic generation (SHG) of two-dimensional (2D) crystals, coupled with their atomic thickness that circumvents the phase-match problem, has garnered considerable attention. While various 2D heterostructures…

Materials Science · Physics 2023-10-31 Wontaek Kim , Gyouil Jeong , Juseung Oh , Jihun Kim , Kenji Watanabe , Takashi Taniguchi , Sunmin Ryu

The PhD thesis is devoted to the study of second harmonic generation of narrow beams in photonic crystals. The basic idea is that if both frequencies, the fundamental and second harmonics are in the region of self-collimation, then the…

Optics · Physics 2013-11-06 Cristian Nistor

Atomically thin two dimensional (2D) layered materials have emerged as a new class of material for nanoelectromechanical systems (NEMS) due to their extraordinary mechanical properties and ultralow mass density. Among them, graphene has…

Mesoscale and Nanoscale Physics · Physics 2015-05-28 C. Samanta , P. R. Yasasvi Gangavarapu , A. K. Naik

ReS$_2$ has recently emerged as a new member in the rapidly growing family of two-dimensional materials. Unlike MoS$_2$ or WSe$_2$, the optical and electrical properties of ReS$_2$ are not isotropic due to the reduced symmetry of the…

Mesoscale and Nanoscale Physics · Physics 2016-02-17 Philipp Nagler , Gerd Plechinger , Christian Schüller , Tobias Korn

The crystal structure of La 4 Ge 3S 12 has been known to be noncentrosymmetric for almost four decades. This characteristic inversion symmetry breaking suggests the presence of nonlinear optical properties. Yet only recently have nonlinear…

Materials Science · Physics 2026-02-19 Hiroya Ohtsuki , Suguru Nakata , Yu Yamane , Ryunosuke Takahashi , Koichi Kusakabe , Hiroki Wadati

Recent experimental results have demonstrated the ability of monolayer MoS$_2$ to efficiently generate second harmonic fields with susceptibilities between 0.1 and 100 nm/V. However, no theoretical calculations exist with which to interpret…

Mesoscale and Nanoscale Physics · Physics 2014-06-18 Mads Lund Trolle , Gotthard Seifert , Thomas Garm Pedersen

Two dimensional (2D) layered materials have recently gained renewed interest due to their exotic electronic properties along with high specific surface area. The prospects of exploiting these properties in sensing, catalysis, energy…

Materials Science · Physics 2015-05-20 Sumit Saxena , Raghvendra Pratap Choudhary , Shobha Shukla

We study the nonlinear process of second harmonic generation in photonic time-crystals, materials with refractive index that varies abruptly and periodically in time, and obtain the phase matching condition for this process. We find…