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We study the growing time scales and length scales associated with dynamical slow down for a realistic glass former, using computer simulations. We perform finite size scaling to evaluate a length scale associated with dynamical…

Statistical Mechanics · Physics 2009-11-13 Smarajit Karmakar , Chandan Dasgupta , Srikanth Sastry

We identify a link between the glass transition and percolation of mobile regions in configuration space. We find that many hallmarks of glassy dynamics, for example stretched-exponential response functions and a diverging structural…

Statistical Mechanics · Physics 2009-11-13 Gregg Lois , Jerzy Blawzdziewicz , Corey S. O'Hern

We study the relaxation process in a simple glass-former - the KA lattice gas model. We show that, for this model, structural relaxation is due to slow percolation of regions of co-operatively moving particles, which leads to heterogeneous…

Statistical Mechanics · Physics 2009-11-13 Pinaki Chaudhuri , Srikanth Sastry , Walter Kob

The Adam-Gibbs view of the glass transition relates the relaxation time to the configurational entropy, which goes continuously to zero at the so-called Kauzmann temperature. We examine this scenario in the context of a dimer model with an…

Statistical Mechanics · Physics 2007-05-23 Dibyendu Das , Greg Farrell , Jane' Kondev , Bulbul Chakraborty

The dramatic dynamic slowing down associated with the glass transition is considered by many to be related to the existence of a static length scale that grows when temperature decreases. Defining, identifying and measuring such a length is…

Statistical Mechanics · Physics 2014-05-29 Giulio Biroli , Smarajit Karmakar , Itamar Procaccia

The effects of randomly pinning particles in a model glass-forming fluid are studied, with a focus on the dynamically heterogeneous relaxation in the presence of pinning. We show how four-point dynamical correlations can be analysed in real…

Statistical Mechanics · Physics 2013-10-30 Robert L. Jack , Christopher J. Fullerton

X-ray photon correlation is used to probe the slow dynamics of the glass-former B2O3 across the glass transition. In the undercooled liquid phase the decay times of the measured correlation functions are consistent with visible light…

Disordered Systems and Neural Networks · Physics 2019-07-03 Giovanna Pintori , Giacomo Baldi , Beatrice Ruta , Giulio Monaco

Stress relaxation following deformation of an entangled polymeric liquid is thought to be affected by transient reforming of chain entanglements. In this work, we use single molecule techniques to study the relaxation of individual polymers…

Soft Condensed Matter · Physics 2018-07-04 Yuecheng Zhou , Charles M. Schroeder

We use X-Ray Photon Correlation Spectroscopy to investigate the structural relaxation process in a metallic glass on the atomic length scale. We report evidence for a dynamical crossover between the supercooled liquid phase and the…

Soft Condensed Matter · Physics 2015-06-11 B. Ruta , Y. Chushkin , G. Monaco , L. Cipelletti , E. Pineda , P. Bruna , V. M. Giordano , M. Gonzalez-Silveira

Particle motion of a Lennard-Jones supercooled liquid near the glass transition is studied by molecular dynamics simulations. We analyze the wave vector dependence of relaxation times in the incoherent self scattering function and show that…

Soft Condensed Matter · Physics 2016-08-31 D. A. Stariolo , G. Fabricius

Relaxation processes in supercooled liquids are known to exhibit interesting as well as complex behavior. One of the hallmarks of this relaxation process observed in the measured auto correlation function is occurrence of multiple steps of…

Soft Condensed Matter · Physics 2018-08-01 Rajsekhar Das , Indrajit Tah , Smarajit Karmakar

We propose a connection between self-similar, focusing dynamics in nonlinear partial differential equations (PDEs) and macroscopic dynamic features of the glass transition. In particular, we explore the divergence of the appropriate…

Condensed Matter · Physics 2015-06-24 P. G. Kevrekidis , S. K. Kumar , I. G. Kevrekidis

We show that in the equilibrium phase of glass-forming hard-sphere fluids in three dimensions, the static length scales tentatively associated with the dynamical slowdown and the dynamical length characterizing spatial heterogeneities in…

Disordered Systems and Neural Networks · Physics 2013-04-16 Patrick Charbonneau , Gilles Tarjus

We combine the swap Monte Carlo algorithm to long multi-CPU molecular dynamics simulations to analyse the equilibrium relaxation dynamics of model supercooled liquids over a time window covering ten orders of magnitude for temperatures down…

Soft Condensed Matter · Physics 2022-12-16 Camille Scalliet , Benjamin Guiselin , Ludovic Berthier

The dynamics of structural relaxation in a model polymer glass subject to spatially-homogeneous, time-periodic shear deformation is investigated using molecular dynamics simulations. We study a coarse-grained bead-spring model of short…

Soft Condensed Matter · Physics 2014-01-10 Nikolai V. Priezjev

We investigate the heterogeneous dynamics in a model, where chemical gelation and glass transition interplay, focusing on the dynamical susceptibility. Two independent mechanisms give raise to the correlations, which are manifested in the…

Soft Condensed Matter · Physics 2017-05-09 Antonio de Candia , Annalisa Fierro , Raffaele Pastore , Massimo Pica Ciamarra , Antonio Coniglio

The dynamical behaviours of a kinetically constrained spin model (Fredrickson-Andersen model) on a Bethe lattice are investigated by a perturbation analysis that provides exact final states above the nonergodic transition point. It is…

Statistical Mechanics · Physics 2015-05-19 Hiroki Ohta

We propose a spatio-temporal characterization of the entanglement dynamics in many-body localized (MBL) systems, which exhibits a striking resemblance with dynamical heterogeneity in classical glasses. Specifically, we find that the…

Disordered Systems and Neural Networks · Physics 2022-05-17 Claudia Artiaco , Federico Balducci , Markus Heyl , Angelo Russomanno , Antonello Scardicchio

The relaxation to equilibrium of lattice systems with long-range interactions is investigated. The timescales involved depend polynomially on the system size, potentially leading to diverging equilibration times. A kinetic equation for…

Statistical Mechanics · Physics 2019-10-23 T. M. Rocha Filho , R. Bachelard

We numerically study the equilibrium relaxation dynamics of a two-dimensional Mari-Kurchan glass model. The tree-like structure of particle interactions forbids both non-trivial structural motifs and the emergence of a complex free-energy…

Disordered Systems and Neural Networks · Physics 2022-06-27 Yoshihiko Nishikawa , Atsushi Ikeda , Ludovic Berthier