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Sizable hyperpolarisation, i.e. an imbalance of the occupation numbers of nuclear spins in a sample deviating from thermal equilibrium, is needed in various fields of science. For example, hyperpolarised tracers are utilised in magnetic…

We report the development of a fast pulse polarimeter for the application to quantum non-demolition measurement of atomic spin (Spin QND). The developed system was tunable to the atomic resonance of ytterbium atom and has narrow laser…

Quantum Physics · Physics 2009-11-11 M. Takeuchi , T. Takano , S. Ichihara , A. Yamaguchi , M. Kumakura , T. Yabuzaki , Y. Takahashi

Surface plasmon polariton is collective oscillation of the free electrons at metal dielectric interface. As a wave phenomenon, surface plasmon polaritons can be focused using appropriate excitation geometry of metallic structures. We…

Optics · Physics 2015-10-22 P. A. Golovinski , V. A. Astapenko , E. S. Manuylovich

We experimentally demonstrate a simple and robust protocol for the detection of weak radio-frequency magnetic fields using a single electron spin in diamond. Our method relies on spin locking, where the Rabi frequency of the spin is…

Quantum Physics · Physics 2013-01-14 M. Loretz , T. Rosskopf , C. L. Degen

Quantum sensors based on solid-state spins provide tremendous opportunities in a wide range of fields from basic physics and chemistry to biomedical imaging. However, integrating them into a scanning probe microscope to enable practical,…

Mesoscale and Nanoscale Physics · Physics 2016-01-19 Jean-Philippe Tetienne , Alain Lombard , David A. Simpson , Cameron Ritchie , Jianing Lu , Paul Mulvaney , Lloyd C. L. Hollenberg

We report the use of an atomic magnetometer based on nonlinear magneto-optical rotation with frequency modulated light (FM NMOR) to detect nuclear magnetization of xenon gas. The magnetization of a spin-exchange-polarized xenon sample ($1.7…

Magnetic microscopy that combines nanoscale spatial resolution with picosecond scale temporal resolution uniquely enables direct observation of the spatiotemporal magnetic phenomena that are relevant to future high-speed, high-density…

Mesoscale and Nanoscale Physics · Physics 2021-07-07 Chi Zhang , Jason M. Bartell , Jonathan C. Karsch , Isaiah Gray , Gregory D. Fuchs

We demonstrate a wide-band all-optical method of nanoscale magnetic resonance (MR) spectroscopy under ambient conditions. Our method relies on cross-relaxation between a probe spin, the electronic spin of a nitrogen-vacancy centre in…

We introduce an alternate route to dynamically polarize the nuclear spin host of nitrogen-vacancy (NV) centers in diamond. Our approach articulates optical, microwave and radio-frequency pulses to recursively transfer spin polarization from…

Quantum Physics · Physics 2014-12-18 Daniela Pagliero , Abdelghani Laraoui , Jacob D. Henshaw , Carlos A. Meriles

Magnetic torque is used to actuate nano-torsional resonators, which are fabricated by focused-ion-beam milling of permalloy coated silicon nitride membranes. Optical interferometry is used to measure the mechanical response of two torsion…

Mesoscale and Nanoscale Physics · Physics 2010-03-09 J. P. Davis , D. Vick , D. C. Fortin , J. A. J. Burgess , W. K. Hiebert , M. R. Freeman

Spin polarized atomic ensembles can be used for the precise measurement of magnetic field. Conventional atomic magnetometers have demonstrated high sensitivities, albeit at low detection bandwidth, fundamentally limited by the Larmor…

Detecting nuclear spins using single Nitrogen-Vacancy (NV) centers is of particular importance in nano-scale science and engineering, but often suffers from the heating effect of microwave fields for spin manipulation, especially under high…

Quantum Physics · Physics 2024-09-06 Zhiyi Hu , Fengjian Jiang , Jingyan He , Yulin Dai , Ya Wang , Nanyang Xu , Jiangfeng Du

We report on measurements of the spin lifetime of nuclear spins strongly coupled to a micromechanical cantilever as used in magnetic resonance force microscopy. We find that the rotating-frame correlation time of the statistical nuclear…

Mesoscale and Nanoscale Physics · Physics 2008-04-04 C. L. Degen , M. Poggio , H. J. Mamin , D. Rugar

Nuclear Magnetic Resonance (NMR) spans diverse fields from biology to quantum science. Employing NMR on a floating object could unveil novel possibilities beyond conventional operational paradigms. Here, we observe Nuclear Magnetic…

Quantum Physics · Physics 2024-07-30 J. Voisin , A. Durand , T. Copie , M. Perdriat , G. Hétet

Till now the nanoscale focussing and imaging in the sub-diffraction limit is achieved mainly with the help of plasmonic field enhancement assisted with noble metal nanoparticles. Using far field imaging technique, we have recorded polarized…

Materials Science · Physics 2017-04-05 A. K. Sivadasan , Manas Sardar , Sandip Dhara

Nanomechanical spectroscopy (NMS) is a recently developed approach to determine optical absorption spectra of nanoscale materials via mechanical measurements. It is based on measuring changes in the resonance frequency of a membrane…

In this work, we develop a nanoscale magnetic field sensor based on a spin-Hall nano-oscillator (SHNO) device. We fabricate constriction-based SHNO devices using Ni$_{81}$Fe$_{19}$/Au$_{0.25}$Pt$_{0.75}$ bilayer and use them to demonstrate…

Mesoscale and Nanoscale Physics · Physics 2023-03-07 Yanyou Xie , Hil Fung Harry Cheung , Gregory D. Fuchs

We demonstrate nuclear double resonance for nanometer-scale volumes of spins where random fluctuations rather than Boltzmann polarization dominate. When the Hartmann-Hahn condition is met in a cross-polarization experiment, flip-flops occur…

Statistical Mechanics · Physics 2017-08-07 M. Poggio , H. J. Mamin , C. L. Degen , M. H. Sherwood , D. Rugar

Nitrogen vacancy (NV) color centers in diamond are a leading modality for both superresolution optical imaging and nanoscale magnetic field sensing. In this work, we solve the remaining key challenge of performing optical magnetic imaging…

Nuclear magnetic resonance (NMR) at the single-molecule level with atomic resolution holds transformative potential for structural biology and surface chemistry. Near-surface solid-state spin sensors with optical readout ability offer a…

Quantum Physics · Physics 2025-12-12 Yu Chen , Qi Zhang , Yuanhong Teng , Chihang Luo , Zhijie Li , Jinpeng Liu , Ya Wang , Fazhan Shi , Jiangfeng Du