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Dynamic nuclear polarization (DNP) enhances the intensity of NMR signals by transferring polarization from electron spins to nuclei via microwave irradiation. Pulsed DNP methods offer more control on the spin dynamics than conventional…

Chemical Physics · Physics 2026-01-07 Lorenzo Niccoli , Gian-Marco Camenisch , Matías Chávez , Matthias Ernst

Solid-state spins in diamond are promising building blocks for quantum computing and quantum sensing, both of which require precise nanoscale addressing of individual spins. To explore the resolution limit of this approach, we demonstrate…

Quantum Physics · Physics 2026-03-25 Peihan Lei , You Huang , Zhi Cheng , Fazhan Shi , Pengfei Wang

Nuclear magnetic resonance (NMR) spectroscopy is a powerful technique to study local magnetism in a variety of materials. However, the inherently low sensitivity of conventional inductively detected solid state NMR typically requires a…

Mesoscale and Nanoscale Physics · Physics 2025-12-16 Louis Beaudoin , Aimé Verrier , Youcef A. Bioud , Mathieu Massicotte , Bertrand Reulet , Jeffrey A. Quilliam

Distance measurements via the dipolar interaction are fundamental to the application of nuclear magnetic resonance (NMR) to molecular structure determination, but they only provide information on the absolute distance $r$ and polar angle…

Quantum Physics · Physics 2018-10-30 J. Zopes , K. Herb , K. S. Cujia , C. L. Degen

Pulsar timing is used for a variety of applications including tests of fundamental physics, probing the structure of neutron stars, and detecting nanohertz gravitational waves. Development of robust methods and generation of high-quality…

Nitrogen-vacancy (NV) magnetometry is a new technique for imaging spin waves in magnetic materials. It detects spin waves by their microwave magnetic stray fields, which decay evanescently on the scale of the spin-wavelength. Here, we use…

Mesoscale and Nanoscale Physics · Physics 2022-12-08 Brecht G. Simon , Samer Kurdi , Joris J. Carmiggelt , Michael Borst , Allard Katan , Toeno van der Sar

This work demonstrates nanoscale magnetic imaging using bright circularly polarized high-harmonic radiation. We utilize the magneto-optical contrast of worm-like magnetic domains in a Co/Pd multilayer structure, obtaining quantitative…

The optically induced polarization of localized electron spins in an ensemble of quantum dots (QDs) dephases due to the interaction with the surrounding nuclear spins. Despite this dephasing, the spins in the QDs can be controlled to…

Mesoscale and Nanoscale Physics · Physics 2022-04-08 P. Schering , G. S. Uhrig

Optical pump-probe techniques are used to generate and measure electron spin polarization in a gallium arsenide epilayer in which the electron spin coherence time exceeds the mode-locked laser repetition period. Resonant spin amplification…

Mesoscale and Nanoscale Physics · Physics 2020-09-14 Michael Macmahon , Joseph R. Iafrate , Michael J. Dominguez , Vanessa Sih

Magnetic resonance detection is one of the most important tools used in life-sciences today. However, as the technique detects the magnetization of large ensembles of spins it is fundamentally limited in spatial resolution to mesoscopic…

We propose a scheme to increase the sensitivity and thus the detection volume of nanoscale single molecule magnetic resonance imaging. The proposal aims to surpass the T1 limited detection of the sensor by taking advantage of a long-lived…

Quantum Physics · Physics 2015-11-05 Johannes N. Greiner , D. D. Bhaktavatsala Rao , Philipp Neumann , Jörg Wrachtrup

Nanoscale magnetic resonance imaging (NanoMRI) is an active area of applied research with potential use in structural biology and quantum engineering. The success of this technological vision hinges on improving the instrument's sensitivity…

Conventional nuclear magnetic resonance (NMR) spectroscopy relies on acquiring signal from a macroscopic ensemble of molecules to gain information about molecular structure and dynamics. Transferring this technique to nanoscale sample sizes…

Mesoscale and Nanoscale Physics · Physics 2019-02-06 Jeffrey Holzgrafe , Qiushi Gu , Jan Beitner , Dhiren Kara , Helena S. Knowles , Mete Atatüre

We perform pulsed optically detected electron spin resonance to measure the DC magnetic field sensitivity and electronic spin coherence time T_2 of an ensemble of near-surface, high-density nitrogen-vacancy (NV) centers engineered to have a…

Mesoscale and Nanoscale Physics · Physics 2017-05-11 Kento Sasaki , Ed E. Kleinsasser , Zhouyang Zhu , Wen-Di Li , Hideyuki Watanabe , Kai-Mei C. Fu , Kohei M. Itoh , Eisuke Abe

Birefringence in ionized, magnetized media is usually measured as Faraday rotation of linearly polarized radiation. However, pulses propagating through regions with very large Faraday rotation measures (RMs) can split into circularly…

High Energy Astrophysical Phenomena · Physics 2019-01-23 Akshay Suresh , James M. Cordes

We describe a new approach to precision NMR with hyperpolarized gases designed to mitigate NMR frequency shifts due to the alkali spin exchange field. The electronic spin polarization of optically pumped alkali atoms is square-wave…

Atomic Physics · Physics 2015-12-23 Anna Korver , Daniel Thrasher , Mike Bulatowicz , Thad Walker

We report on imaging of microwave (MW) magnetic fields using a magnetometer based on the electron spin of a nitrogen vacancy center in diamond. We quantitatively image the magnetic field generated by high frequency (GHz) MW current with…

Mesoscale and Nanoscale Physics · Physics 2015-11-16 Patrick Appel , Marc Ganzhorn , Elke Neu , Patrick Maletinsky

The nuclear spin is a prime candidate for quantum information applications due to its weak coupling to the environment and inherently long coherence times. However, this weak coupling also challenges the addressability of the nuclear spin.…

Quantum Physics · Physics 2025-12-15 Hester G. Vennema , Cristina Mier , Evert W. Stolte , Leonard Edens , Jinwon Lee , Sander Otte

Nuclear Magnetic Resonance (NMR) is an intriguing quantum-mechanical effect that is used for daily life medical diagnostics and chemical analysis alike. Numerous advancements have contributed to the success of the technique, including…

Chemical Physics · Physics 2020-04-28 Andrey N. Pravdivtsev , Frank D. Sönnichsen , Jan-Bernd Hövener

It is demonstrated that the time evolution of the electron-nuclear polarization transfer process during pulsed dynamic nuclear polarization (DNP) can be reversed on a microsecond timescale, leading to the observation of DNP echoes. The DNP…

Chemical Physics · Physics 2024-06-28 Nino Wili , Anders B. Nielsen , José P. Carvalho , Niels Chr. Nielsen
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