Related papers: Few-Photon All-Optical {\pi} Phase modulation Base…
Two-photon excitation (TPE) proceeds via a "virtual" pathway, which depends on the accessibility of one or more intermediate states, and, in the case of non-centrosymmetric molecules, an additional "dipole" pathway involving the…
We present and implement a new scheme for independent control of both the final and the transient population utilizing the symmetry properties of the system. By proper pulse shaping, utilizing the invariance of the two-photon absorption to…
While the phase of a coherent light field can be precisely known, the phase of the individual photons that create this field, considered individually, cannot. Phase changes within single-photon wave packets, however, have observable…
We evaluate the advantages of performing cross-phase modulation (XPM) on a very-far-off-resonance atomic system. We consider a ladder system with a weak (few-photon level) control coherent field imparting a conditional nonlinear phase shift…
The theoretically predicted correlation of laser phase fluctuations in Lambda-type interaction schemes is experimentally demonstrated. We show, that the mechanism of correlation in a Lambda scheme is restricted to high frequency noise…
The frequency conversion of light has proved to be a crucial technology for communication, spectroscopy, imaging, and signal processing. In the quantum regime, it also offers great potential for realizing quantum networks incorporating…
We study a four-level atomic scheme interacting with four lasers in a closed-loop configuration with a $\diamondsuit$ (diamond) geometry. We investigate the influence of the laser phases on the steady state. We show that, depending on the…
We study the interaction of two photons in a Rydberg atomic ensemble under the condition of electromagnetically induced transparency, combining a semi-classical approach for pulse propagation and a complete quantum treatment for quantum…
We report on coherent control of excitation processes of translationally ultracold rubidium dimers in a magneto-optical trap by using shaped femtosecond laser pulses. Evolution strategies are applied in a feedback loop in order to optimize…
We calculate the frequency-dispersed nonlinear transmission signal of a phase-shaped visible pulse to fourth order in the field. Two phase profiles, a phase-step and phase-pulse, are considered. Two dimensional signals obtained by varying…
We present a general model for an atomic memory using ultra-short pulses of light, which allows both spatial and temporal multimode storage. The process involves the storage of a faint quantum light pulse into the spin coherence of the…
The absorption of a single photon that excites a quantum system from a low to a high energy level is an elementary process of light-matter interaction, and a route towards realizing pure single-photon absorption has both fundamental and…
In a three-level atomic system coupled by two equal-amplitude laser fields with a frequency separation 2$\delta$, a weak probe field exhibits a multiple-peaked absorption spectrum with a constant peak separation $\delta$. The corresponding…
Observing few-photon optomechanical effects remains a significant challenge in optomechanical systems. To investigate intrinsic radiation-pressure-induced nonlinear effects in the few-photon regime, it is essential to strengthen the…
Path-entangled multi-photon states allow optical phase-sensing beyond the shot-noise limit, provided that an efficient parity measurement can be implemented. Realising this experimentally is technologically demanding, as it requires…
Photoassociation with short laser pulses has been proposed as a technique to create ultracold ground state molecules. A broad-band excitation seems the natural choice to drive the series of excitation and deexcitation steps required to form…
In one-dimensional optical setups, light-matter interaction is drastically enhanced by the interference between the incident and scattered fields. Particularly, in the impedance-matched \Lambda-type three-level systems, a single photon…
A scheme is proposed here to achieve swapping and entangling of photonic and atomic qubits with high fidelity. The mechanism is based on the scattering of a single photon from a $\Lambda$-type three-level atom. The evolution of the coupled…
The ability to design, fabricate and control systems that can convert photons with dissimilar frequencies has technological implications in classical as well as quantum communications. Laser heating and thermal-mechanical motion in…
We show that coupling ultracold atoms in optical lattices to quantized modes of an optical cavity leads to quantum phases of matter, which at the same time posses properties of systems with both short- and long-range interactions. This…