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In heterostructures consisting of different transition-metal dichalcogenide monolayers, a staggered band alignment can occur, leading to rapid charge separation of optically generated electron-hole pairs into opposite monolayers. These…

We develop a time-dependent theory to investigate electron dynamics and photoionization processes of diatomic molecules interacting with strong laser fields including electron-electron correlation effects. We combine the recently formulated…

Chemical Physics · Physics 2016-02-02 Henrik R. Larsson , Sebastian Bauch , Lasse Kragh Sørensen , Michael Bonitz

We concentrate here on photon absorption as well as electron and positron scattering upon endohedrals that consist of a fullerenes shell and an inner atom A. The aim is to understand the effect of fullerene electron shell in formation of…

Atomic and Molecular Clusters · Physics 2018-02-12 M. Ya. Amusia , A. F. Ioffe

We propose a protocol to probe the ultrafast evolution and dephasing of coherent electronic excitation in molecules in the time domain by the intrinsic streaking field generated by the molecule itself. Coherent electronic motion in the…

Coupled colloidal quantum dot molecules composed of two fused CdSe/CdS core/shell sphere monomers were recently presented. Upon fusion, the potential energy landscape is changing into two quantum dots separated by a pre-tuned potential…

Mesoscale and Nanoscale Physics · Physics 2019-12-11 Yossef E. Panfil , Doaa Shamalia , Jiabin Cui , Somnath Koley , Uri Banin

Interlayer excitons, comprising an electron in one material bound by Coulomb attraction to a hole in an adjacent material, are composite bosons that can assume a variety of many-body phases. The phase diagram of the bosonic system is…

Mesoscale and Nanoscale Physics · Physics 2016-06-08 Brian Skinner

We develop a general theory of electron--hole recombination in organic light emitting diodes that leads to formation of emissive singlet excitons and nonemissive triplet excitons. We briefly review other existing theories and show how our…

Materials Science · Physics 2009-11-07 K. Tandon , S. Ramasesha , S. Mazumdar

The layered graphene systems exhibit the rich and unique excitation spectra arising from the electron-electron Coulomb interactions. The generalized tight-binding model is developed to cover the planar/buckled/cylindrical structures,…

Computational Physics · Physics 2019-01-15 Chiun-Yan Lin , Jhao-Ying Wu , Chih-Wei Chiu , Ming-Fa Lin

We studied a vertical ``quantum dot molecule'', where one of the dots is occupied with electrons and the other with holes. We find that different phases occur in the ground state, depending on the carrier density and the interdot distance.…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 K. Karkkainen , M. Koskinen , M. Manninen , S. M. Reimann

The x-ray energies and transition rates associated with single and double electron radiative transitions from the double K hole state $2s2p$ to the $1s2s$ and $1s^{2}$ configurations of 11 He-like ions ($10\!\leq\!Z\!\leq\!47$) are…

Atomic Physics · Physics 2020-02-10 Xiaobin Ding , Mingxin Cao , Denghong Zhang , Mingwu Zhang , Yingli Xue , Deyang Yu , Chenzhong Dong

Transient extreme ultraviolet (XUV) spectroscopy probes core level transitions to unoccupied valence and conduction band states. Uncertainty remains to what degree the core-hole created by the XUV transition modifies the measurement of…

High-energy nuclear collisions have opened a new experimental method to reveal collective behavior in nuclear ground states through the lens of many-body correlations of nucleons. Using ab initio lattice and variational calculations of…

Nuclear Theory · Physics 2025-12-23 Jean-Paul Blaizot , Giuliano Giacalone , Alessandro Lovato

Optical transitions in a semiconductor quantum dot are theoretically investigated, with emphasis on the coupling to longitudinal optical phonons, and including excitonic effects. When limiting to a finite number of $m$ electron and $n$ hole…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 T. Stauber , R. Zimmermann

A proper theoretical description of electronic structure of the 3d orbitals in the metal centers of functional metalorganics is a challenging problem. In this letter, we apply density functional theory and an exact diagonalization method in…

High-harmonic generation (HHG) is a coherent optical process in which the incident photon energy is up-converted to the multiples of its initial energy. In solids, under the influence of a strong laser field, electron-hole (e-h) pairs are…

The effect of intermolecular interactions on intensity redistribution between individual electronic transitions in different polymorphs of fluorene and dibenzofuran was studied by transmittance electronic spectroscopy in the energy range…

Materials Science · Physics 2013-05-09 Lina Nakhimovsky

We consider the interaction of electromagnetic radiation of arbitrary polarization with multi-level atoms in a self-consistent manner, taking into account both spatial and temporal dependencies of local fields. This is done by numerically…

Mesoscale and Nanoscale Physics · Physics 2015-03-19 Maxim Sukharev , Abraham Nitzan

For certain systems, the N-particle ground-state wavefunctions of the bulk happen to be exactly equal to the N-point space-time correlation functions at the edge, in the infrared limit. We show why this had to be so for a class of…

Strongly Correlated Electrons · Physics 2015-05-28 R. Shankar , Ashvin Vishwanath

In monolayer transition-metal dichalcogenide semiconductors, many-body correlations can manifest in optical spectra when photoexcited electron-hole pairs (excitons) are introduced into a 2D Fermi sea of mobile carriers. At low carrier…

Mesoscale and Nanoscale Physics · Physics 2022-01-04 Jing Li , Mateusz Goryca , Junho Choi , Xiaodong Xu , Scott A. Crooker

We present a qualitative model for a fundamental process in molecular electronics: the change in conductance upon bond breaking. In our model a diatomic molecule is attached to spin-polarized contacts. Employing a Hubbard Hamiltonian,…

Materials Science · Physics 2008-06-24 Ali Goker , Francois Goyer , Matthias Ernzerhof