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Time-resolved spectroscopic temperature measurements of a sealed carbon dioxide sample cell were realized with an optical frequency comb combined with a two-dimensional dispersive spectrometer. A supercontinuum laser source based on an…

We have carried out a high spectral resolution line survey towards the Orion Kleinmann-Low (KL) cluster from 44-188 um. The observations were taken with the Long Wavelength Spectrometer (LWS) in Fabry-Perot mode, on board the Infrared Space…

We present a system for molecular spectroscopy using a broadband mid-infrared laser with near infrared detection. Difference frequency generation of a Yb:fiber femtosecond laser produced a mid-infrared (MIR) source tunable from 2100-3700…

Optics · Physics 2015-05-30 Todd A. Johnson , Scott A. Diddams

Mid infrared (MIR) photonics is a key region for molecular physics [1]. High-resolution spectroscopy in the 1--10 {\mu}m region, though, has never been fully tackled for the lack of widely-tunable and practical light sources. Indeed, all…

Numerous molecules exhibit unique absorption bands in the fingerprint infrared (IR) region, allowing chemical identification and detection. This makes IR spectroscopy an essential tool in biomedical diagnostics, sensing, and material…

Optics · Physics 2022-02-04 Anna V. Paterova , Zi S. D. Toa , Hongzhi Yang , Leonid A. Krivitsky

A compact and versatile femtosecond mid-IR source is presented, based on an optical parametric oscillator (OPO) synchronously pumped by a commercial 250-MHz Er:fiber laser. The mid-IR spectrum can be tuned in the range 2.25-2.6 \mu m…

We discuss a simple, linear, zero-delay implementation of spectral shearing interferometry for amplitude and phase characterization of optical frequency comb sources and arbitrary waveforms. We demonstrate this technique by characterizing…

Measuring microcombs in amplitude and phase provides unique insight into the nonlinear cavity dynamics but spectral phase measurements are experimentally challenging. Here, we report a linear heterodyne technique assisted by electro-optic…

The on-chip creation of coherent light at visible wavelengths is crucial to field-level deployment of spectroscopy and metrology systems. Although on-chip lasers have been implemented in specific cases, a general solution that is not…

A femtosecond pump-probe setup is described that is optimised for broadband transient reflectivity experiments on solid samples over a wide range of temperatures. By combining a temporal resolution of 45 fs and a broad detection range…

Instrumentation and Detectors · Physics 2016-08-12 Edoardo Baldini , Andreas Mann , Simone Borroni , Christopher Arrell , Frank van Mourik , Fabrizio Carbone

Phase-sensitive detection is the essential projective measurement for measurement-based continuous-variable quantum information processing. The bandwidth of conventional electrical phase-sensitive detectors is up to several gigahertz, which…

Dual-comb interferometry is a measurement technique that uses two laser frequency combs to retrieve complex spectra in a line-by-line basis. This technique can be implemented with electro-optic frequency combs, offering intrinsic mutual…

Optics · Physics 2016-09-21 Vicente Duran , Peter A. Andrekson , Victor Torres-Company

Laser frequency combs are coherent light sources that emit a broad spectrum consisting of discrete, evenly spaced narrow lines, each having an absolute frequency measurable within the accuracy of an atomic clock. Their development, a decade…

Optics · Physics 2017-06-13 Albert Schliesser , Nathalie Picqué , Theodor W. Hänsch

The mid-infrared spectral range (2 to 20 \mu m) is of particular importance for chemistry, biology and physics as many molecules exhibit strong ro-vibrational fingerprints. Frequency combs - broad spectral bandwidth coherent light sources…

Context: Over the past thirty years a wealth of observations of CO and other molecules in optical/uv absorption in diffuse clouds has accumulated for which no comparable CO emission line data exist. Aims: To acquire mm-wave J=1-0 CO…

Astrophysics of Galaxies · Physics 2009-11-13 H. S. Liszt

We present a 100 MHz repetition rate Yb-fiber-laser-pumped synchronously pumped optical parametric oscillator (SPOPO) delivering tunable frequency combs covering almost the entire visible spectral range. By intracavity doubling both the…

Broadband and high-resolution spectroscopy in the visible and ultraviolet is central to advances in multiple fields, including fundamental quantum physics, biology, atmospheric science and astronomy. Traditionally, these measurements are…

Optical spectroscopy is a fundamental tool in numerous areas of science and technology. Much effort has focused on miniaturizing spectrometers, but thus far at the cost of high spectral resolution and broad operating range. Here, we…

We have demonstrated a new technique that provides massively parallel comb spectroscopy sensitive specifically to ions through the combination of cavity-enhanced direct frequency comb spectroscopy with velocity modulation spectroscopy.…

Atomic Physics · Physics 2015-05-28 Laura C. Sinclair , Kevin C. Cossel , Tyler Coffey , Jun Ye , Eric A. Cornell

Cavity-enhanced direct frequency comb spectroscopy (CE-DFCS) has demonstrated powerful potential for trace gas detection based on its unique combination of high bandwidth, rapid data acquisition, high sensitivity, and high resolution, which…