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The high quantum efficiency of photosynthetic complexes has inspired researchers to explore new routes to utilize this process for photovoltaic devices. Quantum coherence has been demonstrated to play a crucial role within this process.…

Chemical Physics · Physics 2015-06-23 Yiteng Zhang , Sangchul Oh , Fahhad H. Alharbi , Greg Engel , Sabre Kais

A general semiclassical approach to quantum systems with system-bath interactions is developed. We study system decoherence in detail using a coherent state semiclassical wavepacket method which avoids singularity issues arising in the…

Quantum Physics · Physics 2009-11-07 Gregory A. Fiete , Eric J. Heller

We use coherent states as trial states for a variational approach to study a system of a finite number of three-level atoms interacting in a dipolar approximation with a one-mode electromagnetic field. The atoms are treated as…

Quantum Physics · Physics 2018-06-20 L. F. Quezada , E. Nahmad-Achar

Coherent quantum optics, where the interaction of a photon with an emitter does not scramble phase coherence, lies at the heart of many quantum optical effects and emerging technologies. Solid-state emitters coupled to nanophotonic…

Non-equilibrium transport properties and energy conversion performance of a molecular photo-voltaic cell are analyzed using the Lindblad master equation within the open quantum systems approach. The method allows us to calculate the…

Mesoscale and Nanoscale Physics · Physics 2015-04-09 Shigeru Ajisaka , Bojan Zunkovic , Yonatan Dubi

The question of whether sunlight induces coherent dynamics in biological systems is under debate. Here we show, on the basis of an exact fully quantum mechanical treatment, that thermal light induces excited-state coherences in matter…

Quantum Physics · Physics 2015-05-04 David Avisar , Asaf Eilam , A. D. Wilson-Gordon

We study a two-level system (atom, superconducting qubit or quantum dot) strongly coupled to the single photonic mode of a cavity, in the presence of incoherent pumping and including detuning and dephasing. This system displays a striking…

Quantum Physics · Physics 2011-10-12 E. del Valle , F. P. Laussy

We propose a novel general approximation to transform and simplify the description of a complex fully-quantized system describing the interacting light and matter. The method has some similarities to the time-dependent Born-Oppenheimer…

Quantum Physics · Physics 2021-07-01 Ivan Gonoskov , Stefanie Gräfe

Obtaining the total wavefunction evolution of interacting quantum systems provides access to important properties, such as entanglement, shedding light on fundamental aspects, e.g. quantum energetics and thermodynamics, and guiding towards…

Quantum Physics · Physics 2022-02-02 Maria Maffei , Patrice A. Camati , Alexia Auffèves

The incoherence of sunlight has long been suspected to have an impact on solar cell energy conversion efficiency, although the extent of this is unclear. Existing computational methods used to optimize solar cell efficiency under incoherent…

Optics · Physics 2014-01-16 Aline Herman , Michael Sarrazin , Olivier Deparis

Intense light-matter interaction largely relies on the use of high-power light sources, creating fields comparable to, or even stronger than, the field keeping the electrons bound in atoms. Under such conditions, the interaction induces…

Quantum Physics · Physics 2025-10-23 P. Stammer , J. Rivera-Dean , P. Tzallas , M. F. Ciappina , M. Lewenstein

The implementation of a wide range of novel concepts for next-generation high-efficiency solar cells is based on nanostructures with configuration-tunable optoelectronic properties. On the other hand, effective nano-optical light-trapping…

Materials Science · Physics 2018-04-04 Urs Aeberhard

We present a comprehensive theoretical investigation of high-order harmonic generation in H$_2^+$ molecular ions within a quantum optical framework. Our study focuses on characterizing various quantum optical and quantum information…

Intense laser-matter interactions are at the center of interest in research and technology since the development of high power lasers. They have been widely used for fundamental studies in atomic, molecular, and optical physics, and they…

We introduce a combination of coherent states as variational test functions for the atomic and radiation sectors to describe a system of Na three- level atoms interacting with a one-mode quantised electromagnetic field, with and without the…

Quantum Physics · Physics 2015-10-22 R. López-Peña , S. Cordero , E. Nahmad-Achar , O. Castaños

Dye-sensitized solar cells (DSC), built upon organic/inorganic hybrid materials, are promising third generation solar cells, which attract wide attentions due to their low-cost, flexibility and environment-friendly properties. We review…

Materials Science · Physics 2015-02-09 Wei Ma , Fan Zhang , Sheng Meng

Theoretical and experimental studies have suggested the relevance of quantum coherence to the performance of photovoltaic and light-harvesting complex molecular systems. However, there are ambiguities regarding the validity of statements we…

Chemical Physics · Physics 2022-08-31 Sahar Basiri-Esfahani , Farid Shahandeh

The preparation and control of quantum states lie at the heart of quantum information science (QIS). Recent advances in solid-state quantum emitters (QEs) and nanophotonics have transformed the landscape of quantum photonic technologies,…

A design tool was formulated for optimizing the efficiency of inorganic, thin-film, photovoltaic solar cells. The solar cell can have multiple semiconductor layers in addition to antireflection coatings, passivation layers, and buffer…

Numerical Analysis · Mathematics 2024-09-23 Tom H. Anderson , Benjamin J. Civiletti , Peter Monk , Akhlesh Lakhtakia

We investigate a laser model for a resonant system of photons and ion cluster-solvated rotating water molecules in which ions in the cluster are identical and have very low, non-relativistic velocities and direction of motion parallel to a…

Quantum Physics · Physics 2017-03-08 Eiji Konishi
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