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Coherent excitation of materials via ultrafast laser pulses can have interesting, observable dynamics in time-resolved photoemission measurements. The broad spectral width of ultrafast pump pulses can coherently excite multiple exciton…

Mesoscale and Nanoscale Physics · Physics 2019-03-27 Avinash Rustagi , Alexander F. Kemper

The critical temperature of high-$T_c$ superconductors is determined, at least in part, by the electron-phonon coupling. We include the effect of an exchange interaction between the electrons and calculate the renormalization of the bare…

Condensed Matter · Physics 2009-10-22 D. Manske , C. T. Rieck , D. Fay

Electron-phonon coupling, being one of the most important parameters governing the material evolution after ultrafast energy deposition, yet remains the most unexplored one. In this work, we applied the dynamical coupling approach to…

Materials Science · Physics 2020-08-05 N. Medvedev , I. Milov

Recent experiments access the time-resolved photoelectron signal originating from plasmon satellites in correlated materials and address their build-up and decay in real time. Motivated by these developments, we present the Kadanoff-Baym…

Strongly Correlated Electrons · Physics 2016-02-24 Michael Schüler , Jamal Berakdar , Yaroslav Pavlyukh

An integrable nonlinear model for the time-dependent equilibration of a bosonic system that has been devised earlier is solved exactly with boundary conditions that are appropriate for a truncated Bose-Einstein distribution, and include the…

Statistical Mechanics · Physics 2020-02-05 N. Rasch , G. Wolschin

In this work, we use neural quantum states (NQS) to describe the high-dimensional wave functions of electron-phonon coupled systems. We demonstrate that NQS can accurately and systematically learn the underlying physics of such problems…

Strongly Correlated Electrons · Physics 2025-01-30 Ankit Mahajan , Paul J. Robinson , Joonho Lee , David R. Reichman

We analyze theoretically the effects of electron-phonon interaction in the dynamics of an electron that can be trapped to a localized state and detrapped to an extended band state of a small quantum dot (QD) using a simple model system. In…

Mesoscale and Nanoscale Physics · Physics 2021-12-03 R. Carmina Monreal

This work addresses the one-dimensional problem of Bloch electrons when they are rapidly driven by a homogeneous time-periodic light and linearly coupled to vibrational modes. Starting from a generic time-periodic electron-phonon…

Mesoscale and Nanoscale Physics · Physics 2017-01-20 C. Dutreix , M. I. Katsnelson

The excited state population of single solid-state emitters is subjected to energy fluctuations around the equilibrium driven by the bath and relaxation through the emission of phonons or photons. Simultaneous measurement of the associated…

Quantum Physics · Physics 2021-05-12 Hendrik Utzat , Moungi G. Bawendi

We address the question whether observables of an exactly solvable model of electrons coupled to (optical) phonons relax into large time stationary state values and investigate if the asymptotic expectation values can be computed using a…

Strongly Correlated Electrons · Physics 2010-08-25 D. M. Kennes , V. Meden

We investigate the excitation of phonons in photoexcited antimony and demonstrate that the entire electron-lattice interactions, in particular coherent and incoherent electron-phonon coupling, can be probed simultaneously. Using femtosecond…

Recent advances in techniques for generating quantum light have stimulated research on novel spectroscopic measurements using quantum entangled photons. One such spectroscopy technique utilizes non-classical correlations among entangled…

Chemical Physics · Physics 2021-07-28 Yuta Fujihashi , Akihito Ishizaki

The low-frequency vibrational spectrum of an isolated nanometer-scale solid differs dramatically from that of a bulk crystal, causing the decay of a localized electronic state by phonon emission to be inhibited. We show, however, that an…

Materials Science · Physics 2009-10-31 Ho-Soon Yang , Michael R. Geller , W. M. Dennis

The exciton relaxation dynamics of photoexcited electronic states in poly($p$-phenylenevinylene) (PPV) are theoretically investigated within a coarse-grained model, in which both the exciton and nuclear degrees of freedom are treated…

Chemical Physics · Physics 2018-02-14 Jonathan R. Mannouch , William Barford , Sarah Al-Assam

We describe the temporal evolution of the time-resolved photoemission response of the spinless Falicov-Kimball model driven out of equilibrium by strong applied fields. The model is one of the few possessing a metal-insulator transition and…

Strongly Correlated Electrons · Physics 2010-04-23 B. Moritz , T. P. Devereaux , J. K. Freericks

The origin of the coherences in two-dimensional spectroscopy of photosynthetic complexes remains disputed. Recently it has been shown that in the ultrashort-pulse limit, oscillations in a frequency-integrated pump-probe signal correspond…

Quantum Physics · Physics 2015-06-22 Allan S. Johnson , Joel Yuen-Zhou , Alán Aspuru-Guzik , Jacob J. Krich

The chaotic nature of x-ray free-electron-laser pulses is a major bottleneck that has limited the joint temporal and spectral resolution of spectroscopic measurements. We show how to use the stochastic x-ray field statistics to overcome…

Optics · Physics 2021-02-15 Stefano M. Cavaletto , Daniel Keefer , Shaul Mukamel

I construct a simple model to demonstrate that when the many-electron quantum state of a material is near a quantum phase transition and the vibrational motion of a phonon explores the potential energy surface near the transition point,…

Other Condensed Matter · Physics 2022-02-03 Nikitas I. Gidopoulos

High-harmonic spectroscopy has become an essential ingredient in probing various ultrafast electronic processes in solids with sub-cycle temporal resolution. Despite its immense importance, sensitivity of high-harmonic spectroscopy to…

Optics · Physics 2022-12-07 Navdeep Rana , Gopal Dixit

Time-resolved spectroscopy provides the main tool for analyzing the dynamics of excitonic energy transfer in light-harvesting complexes. To infer time-scales and effective coupling parameters from experimental data requires to develop…

Chemical Physics · Physics 2018-11-28 Tobias Kramer , Mirta Rodriguez , Yaroslav Zelinskyy