English
Related papers

Related papers: Impulsive Laser Induced Alignment of Molecules Dis…

200 papers

The surface of metal nanoparticles can support plasmonic excitations. These excitations dramatically amplify the electric field of incident light (by several orders of magnitude), potentially ionizing the irradiated nanoparticles in a…

Optics · Physics 2025-04-08 Dmitri E. Kharzeev , Jacob Levitt , Carlos Trallero-Herrero

The relaxation dynamics of a model fluid of platelike colloidal particles is investigated by means of a phenomenological dynamic density functional theory. The model fluid approximates the particles within the Zwanzig model of restricted…

Soft Condensed Matter · Physics 2011-09-14 Markus Bier , Rene van Roij

Recent work applying multidimentional coherent electronic spectroscopy at dilute samples in the gas phase is reviewed. The development of refined phase-cycling approaches with improved sensitivity has opened-up new opportunities to probe…

Atomic and Molecular Clusters · Physics 2019-09-12 Lukas Bruder , Ulrich Bangert , Marcel Binz , Daniel Uhl , Frank Stienkemeier

Recently, it was shown how the primary steps of solvation of a single Na$^+$ ion, instantly created at the surface of a nanometer-sized droplet of liquid helium, can be followed at the atomic level [Albrectsen et al. Nature $\textbf{623}$,…

Controlling the interactions between atoms with external fields opened up new branches in physics ranging from strongly correlated atomic systems to ideal Bose and Fermi gases and Efimov physics. Such control usually prepares samples that…

We make use of an inhomogeneous electrostatic dipole field to impart a quantum-state-dependent deflection to a pulsed beam of OCS molecules, and show that those molecules residing in the absolute ground state, $X ^1\Sigma^+$, $\ket{00^00}$,…

We present experimental results for the ionization of aniline and benzene molecules subjected to intense ultrashort laser pulses. Measured parent molecular ions yields were obtained using a recently developed technique capable of…

We show that a combination of a half-cycle pulse and a short nonresonant laser pulse produces a strongly enhanced postpulse orientation. Robust transients that display both efficient and long-lived orientation are obtained. The mechanism is…

Quantum Physics · Physics 2007-05-23 D. Daems , S. Guérin , D. Sugny , H. R. Jauslin

We present the results of experimental and theoretical studies of fast anisotropic relaxation and rotational diffusion in the first electron excited state of biological coenzyme NADH in water-ethanol solutions. The experiments have been…

We present a theoretical study of the time-dependent laser alignment of molecules taking into account the hyperfine coupling due to nuclear-quadrupole interactions. The coupling of nuclear spins to the overall angular momentum of molecules…

Chemical Physics · Physics 2020-06-18 Linda V. Thesing , Andrey Yachmenev , Rosario González-Férez , Jochen Küpper

We propose new nanotargets as nano-layered flat-top cone targets to be used for future laser-ion acceleration experiments at ELI-NP. We study their behaviour at the interaction with an ultra-high intensity laser pulse by performing…

Plasma Physics · Physics 2019-07-24 O Budrigă , E d'Humières , L E Ionel , M Martiş , M Carabaş

Self-guided femtosecond laser pulses propagating in low-pressure gas can generate plasma filaments, establishing a new framework for plasma wakefield acceleration. Unlike conventional schemes relying on mechanically confined or preformed…

The ro--vibrational spectra of molecules dissolved in liquid $^4$He nanodroplets display rotational structure. Where resolved, this structure has been used to determine a temperature that has been assumed to equal that of the intrinsic…

Chemical Physics · Physics 2009-11-10 Kevin K. Lehmann

We show that the decays with pressure of the alignment echoes induced in N2O-He gas mixtures by two laser pulses with various delays bring detailed information on collision-induced changes of the rotational speed. Measurements and…

The generation of ultra-strong attosecond pulses through laser-plasma interactions offers the opportunity to surpass the intensity of any known laboratory radiation source, giving rise to new experimental possibilities, such as quantum…

Helium nanodroplets are ideal model systems to unravel the complex interaction of condensed matter with ionizing radiation. Here we study the effect of purely elastic electron scattering on angular and energy distributions of photoelectrons…

We describe an approach to detecting ionizing radiation that combines the special properties of superfluid helium with the sensitivity of quantum optics techniques. Ionization in liquid helium results in the copious production of metastable…

Nuclear Experiment · Physics 2009-11-11 D. N. McKinsey , W. H. Lippincott , J. Nikkel , W. Rellergert

High-order harmonic generation (HHG) from aligned acetylene molecules interacting with mid infra-red (IR), linearly polarized laser pulses is studied theoretically using a mixed quantum-classical approach in which the electrons are…

Atomic Physics · Physics 2018-05-18 Peter Mulholland , Daniel Dundas

We propose and computationally study a method for simultaneously orienting the angular momentum of asymmetric top molecules along: 1) a laboratory-fixed direction; 2) the molecular intermediate moment of inertia axis; 3) the laser field…

Quantum Physics · Physics 2022-11-21 Emil J. Zak

The mixed-field orientation of an asymmetric-rotor molecule with its permanent dipole moment non-parallel to the principal axes of polarizability is investigated experimentally and theoretically. We find that for the typical case of a…