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We report a novel scheme to generate laser-induced, ultrafast, intense (Tesla scale), spatially isolated, magnetic fields. Three-dimensional particle-in-cell simulations show that a femtosecond azimuthally-polarized infrared vector beam,…

We study interaction of generic asymmetric molecules with a pair of strong time-delayed short laser pulses with crossed linear polarizations. We show that such an excitation not only provides unidirectional rotation of the most polarizable…

Chemical Physics · Physics 2018-02-28 E. Gershnabel , I. Sh. Averbukh

We address the influence of the orbital symmetry and of the molecular alignment with respect to the laser-field polarization on laser-induced nonsequential double ionization of diatomic molecules, in the length and velocity gauges. We work…

Atomic Physics · Physics 2009-11-13 C. Figueira de Morisson Faria , T. Shaaran , X. Liu , W. Yang

We report the observation of macroscopic field-free orientation, i.e. more than 73 % of CO molecules pointing in the same direction. This is achieved through an all-optical scheme operating at high particle densities ($>10^{17}$cm$^{-3}$)…

Chemical Physics · Physics 2014-07-09 P. M. Kraus , D. Baykusheva , H. J. Wörner

Recently, S. Mitryukovskiy et al. presented experimental evidence showing that backward stimulated radiation at 337 nm can be obtained from plasma filaments in nitrogen gas pumped by circularly polarized 800 nm femtosecond pulses (Opt.…

Rotationally resolved infrared spectra are reported for halogen atom - HF free radical complexes formed in helium nanodroplets. An effusive pyrolysis source is used to dope helium droplets with Cl, Br and I atoms, formed by thermal…

Atomic and Molecular Clusters · Physics 2016-04-13 Jeremy M. Merritt , Jochen Küpper , Roger E. Miller

Laser-assisted electron scattering (LAES), a light-matter interaction process that facilitates energy transfer between strong light fields and free electrons, has so far been observed only in gas phase. Here we report on the observation of…

We describe numerically the ionization process induced by linearly and circularly polarized XUV attosecond laser pulses on an aligned atomic target, specifically, the excited state…

Atomic Physics · Physics 2021-05-26 Juan J. Omiste , Lars Bojer Madsen

Helium (He) nanodroplets irradiated by intense near-infrared laser pulses form a nanoplasma by avalanche-like electron impact ionizations even at lower laser intensities where He is not directly field ionized, provided that the droplets…

Atomic and Molecular Clusters · Physics 2017-12-06 Andreas Heidenreich , Dominik Schomas , Marcel Mudrich

The predissociation dynamics of lithium iodide (LiI) in the first excited A-state is investigated for molecules in the gas phase and embedded in helium nanodroplets, using femtosecond pump-probe photoionization spectroscopy. In the gas…

Atomic and Molecular Clusters · Physics 2015-03-03 H. Schmidt , J. von Vangerow , F. Stienkemeier , A. S. Bogomolov , A. V. Baklanov , D. M. Reich , W. Skomorowski , C. P. Koch , M. Mudrich

A significant fraction of superfluid helium nanodroplets produced in a free-jet expansion have been observed to gain high angular momentum resulting in large centrifugal deformation. We measured single-shot diffraction patterns of…

Optically generated electron-hole plasma in high-index dielectric nanostructures was demonstrated as a means of tuning of their optical properties. However, until now an ultrafast operation regime of such plasma driven nanostructures has…

We report on generation of a rotational wavepacket in the ground vibronic state (v = 0) of excited electronic B2{\Sigma}u+ state of N2+ in a femtosecond laser induced plasma spark. Decoding of the rotational wavepacket is achieved with the…

We present quantum mechanical explanations for unresolved phenomena observed in field-free molecular alignment by a femtosecond laser pulse. Quantum phase analysis of molecular rotational states reveals the physical origin of the following…

Optics · Physics 2015-04-09 Sang Jae Yun , Chul Min Kim , Jongmin Lee , Chang Hee Nam

We use ultrafast pump-probe transmission spectroscopy to measure the electronic relaxation time for electrons in cobalt nanoparticles embedded on glass substrate using femtosecond laser pulses. We found that the plasmon excitation is…

Optics · Physics 2013-07-10 R. K. Shrestha , H. Garcia

A novel polarization-modulation transient method has been developed for studying fast anisotropic relaxation in electronic excited states of polyatomic and biologically relevant molecules under excitation with femtosecond laser pulses. The…

Chemical Physics · Physics 2020-05-12 Ioanna Gorbunova , Nikolay Bezverkhnii , Maxim Sasin , Idris Gagzhiev , Oleg Vasyutinskii

We theoretically investigate the impact of multiple plasmon resonances on the charging of Xe clusters embedded in He nanodroplets under intense pump-probe laser excitation. Our molecular dynamics simulations on Xe309He10000$ and comparison…

Atomic and Molecular Clusters · Physics 2015-05-20 Christian Peltz , Thomas Fennel

We report an overall enhancement of a laser wakefield acceleration (LWFA) using the ionization injection in a mixture of 0.3 % nitrogen gas in 99.7 % helium gas. Upon the interaction of 30 TW, 30 fs laser pulses with a gas jet of the above…

Collision of laser-driven subrelativistic high density ion flows provides a way to create extremely compressed ion conglomerates and study their properties. This paper presents a theoretical study of the electrodynamic implosion of ions…

Plasma Physics · Physics 2025-12-03 S. Yu. Guskov , Ph. Korneev , M. Murakami

We use laser-induced rotation of single molecules embedded in superfluid helium nanodroplets to reveal angular momentum dynamics and transfer in a controlled setting, under far-from-equilibrium conditions. As an unexpected result, we…

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