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The end section of a carbon nanotube, cut by acid treatment, contains hydrophillic oxygen groups. Water molecules can self-assemble around these groups to seal off a carbon nanotube and form an "aqueous valve". Molecular dynamics…

Mesoscale and Nanoscale Physics · Physics 2012-07-02 H. Y. Chen , D. Y. Sun , X. G. Gong , Zhi-Feng Liu

We report results of diffusion Monte Carlo calculations for both $^4$He absorbed in a narrow single walled carbon nanotube (R = 3.42 \AA) and strictly one dimensional $^4$He. Inside the tube, the binding energy of liquid $^4$He is…

Statistical Mechanics · Physics 2009-10-31 M. C. Gordillo , J. Boronat , J. Casulleras

We combine modeling and measurements to investigate the dynamics of convective carbon dioxide (CO$_2$) dissolution in a pressure-volume-temperature cell, extending a recent study by Wen et al. (J. Fluid Mech., vol. 854, 2018, pp. 56--87) at…

Fluid Dynamics · Physics 2021-07-07 Baole Wen , Zhuofan Shi , Kristian Jessen , Marc A. Hesse , Theodore T. Tsotsis

The fabrication of metallic single-walled carbon nanotube electrodes separated by gaps of typically 20nm width by electron-beam-induced oxidation is studied within an active device configuration. The tube conductance is measured…

The use of pressure to obtain new materials that can be recovered under ambient conditions is a central problem in high-pressure physics. Despite decades of research, this goal has only been achieved in the laboratory for a few notable…

Materials Science · Physics 2025-08-19 Reetam Paul , Jonathan C. Crowhurst , Stanimir A. Bonev

Nano-materials, such as metal-organic frameworks, have been considered to capture CO$_2$. However, their application has been limited largely because they exhibit poor selectivity for flue gases and low capture capacity under low pressures.…

By means of Diffusion Monte Carlo calculations, we obtained the complete phase diagrams of H$_2$ adsorbed on the outer surface of isolated armchair carbon nanotubes of radii ranging from 3.42 to 10.85 \AA. We only considered density ranges…

Mesoscale and Nanoscale Physics · Physics 2015-05-28 M. C. Gordillo , J. Boronat

A novel system containing nanoporous materials and carbonate ions is proposed, which is capable to capture CO2 from ambient air simply by controlling the amount of water (humidity) in the system. The system absorbs CO2 from the air when the…

Chemical Physics · Physics 2017-02-02 Xiaoyang Shi , Hang Xiao , Xi Chen , Klaus. S. Lackner

Pore structures and gas transport properties in porous separators for polymer electrolyte fuel cells are evaluated both experimentally and through simulations. In the experiments, the gas permeabilities of two porous samples, a conventional…

A pristine suspended carbon nanotube is a near ideal environment to host long-lived quantum states. For this reason, they have been used as the core element of qubits and to explore numerous condensed matter physics phenomena. One of the…

Applied Physics · Physics 2024-01-09 Tim Althuon , Tino Cubaynes , Aljoscha Auer , Christoph Sürgers , Wolfgang Wernsdorfer

The dissolution and subsequent mass transfer of carbon dioxide gas into liquid barriers plays a vital role in many environmental and industrial applications. In this work, we study the downward dissolution and propagation dynamics of CO2…

Membrane-based CO$_2$ removal from exhaust streams has recently gained much attention as a means of reducing emissions and limiting climate change. Novel membranes for CO$_2$ removal include so called facilitated transport membranes (FTMs),…

Soft Condensed Matter · Physics 2023-08-02 M. Logemann , J. Gujt , T. Harhues , T. D. Kühne , M. Wessling

The phase diagrams of $^4$He adsorbed on the external surfaces of single armchair carbon nanotubes with radii in the range 3.42 -- 10.85 \AA \ are calculated using the diffusion Monte Carlo method. For nanotubes narrower than a (10,10) one,…

Materials Science · Physics 2015-06-11 M. C. Gordillo , J. Boronat

We report on high efficency coupling of individual air-suspended carbon nanotubes to silicon photonic crystal nanobeam cavities. Photoluminescence images of dielectric- and air-mode cavities reflect their distinctly different mode profiles…

Mesoscale and Nanoscale Physics · Physics 2014-11-27 R. Miura , S. Imamura , R. Ohta , A. Ishii , X. Liu , T. Shimada , S. Iwamoto , Y. Arakawa , Y. K. Kato

The energy absorption on nanometer scale is vital for many bio and chemical systems. We report here that a two times amplification in absorption efficiency can be achieved by water molecules confined in carbon nanotubes with small radius,…

Mesoscale and Nanoscale Physics · Physics 2022-07-19 Rong-Yao Yang , Wei-Zhou Jiang , Pei-Ying Huo , Qi-Lin Zhang

The van der Waals and Casimir interactions of a hydrogen atom (molecule) with a single-walled and a multiwalled carbon nanotubes are compared. It is shown that the macroscopic concept of graphite dielectric permittivity is already…

Statistical Mechanics · Physics 2009-11-13 G. L. Klimchitskaya , E. V. Blagov , V. M. Mostepanenko

Diffusion Monte Carlo calculations on the adsorption of $^4$He in open-ended single walled (10,10) nanotubes are presented. We have found a first order phase transition separating a low density liquid phase in which all $^4$He atoms are…

Materials Science · Physics 2009-11-13 M. C. Gordillo , J. Boronat , J. Casulleras

Nanoporous materials have the potential to be used as \emph{molecular sieves} to separate chemical substances in a mixture via selective adsorption and kinetic sieving. The separation of isotopologues is also possible via the so-called…

Mesoscale and Nanoscale Physics · Physics 2021-09-15 Manel Mondelo-Martell , Fermín Huarte-Larrañaga

We have observed the transversal vibration mode of suspended carbon nanotubes at millikelvin temperatures by measuring the single-electron tunneling current. The suspended nanotubes are actuated contact-free by the radio frequency electric…

Mesoscale and Nanoscale Physics · Physics 2009-07-18 A. K. Huettel , G. A. Steele , B. Witkamp , M. Poot , L. P. Kouwenhoven , H. S. J. van der Zant

We use electrostatic force microscopy and scanned gate microscopy to probe the conducting properties of carbon nanotubes at room temperature. Multi-walled carbon nanotubes are shown to be diffusive conductors, while metallic single-walled…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 A. Bachtold , M. S. Fuhrer , S. Plyasunov , M. Forero , Erik H. Anderson , A. Zettl , Paul L. McEuen