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Experimental and theoretical studies of unusual polar, dielectric and magnetic properties of room temperature multiferroics, such as perovskites Pb(Fe$_{1/2}$Nb$_{1/2}$)O$_3$ (PFN) and Pb(Fe$_{1/2}$Ta$_{1/2}$)O$_3$ (PFT), are very…

Molecular ferroelectric materials have attracted widespread attention due to their abundant chemical diversity, structural tunability, low synthesis temperature, and high flexibility. Meanwhile, the integration of molecular ferroelectric…

Materials Science · Physics 2023-10-03 Congqin Zheng , Xin Li , Yuhui Huang , Yongjun Wu , Zijian Hong

A combined experimental and computational investigation of coupling between polarization and epitaxial strain in highly polar ferroelectric PbZr_0.2Ti_0.8O_3 (PZT) thin films is reported. A comparison of the properties of relaxed…

The microstructure and phase transition in relaxor ferroelectric Pb(Mg1/3Nb2/3)O3 (PMN) and its solid solution with PbTiO3 (PT), PMN-xPT, remain to be one of the most puzzling issues of solid state science. In the present work we have…

Materials Science · Physics 2009-11-07 Z. -G. Ye , Y. Bing , J. Gao , A. A. Bokov , P. Stephens , B. Noheda , G. Shirane

The structure of Nd$_{1-x}$Pb$_{x}$MnO$_{3}$ crystals is determined by single crystal X-ray diffraction. Substitution of Pb at the Nd site results in structural phase change from tetragonal (x = 0.25) to cubic (x = 0.37). These changes are…

Strongly Correlated Electrons · Physics 2007-05-23 Nilotpal Ghosh , Suja Elizabeth , H. L. Bhat , G. Nalini , B. Muktha , T. N. Guru Row

We study from first-principles calculations the ferroelectric structural phase transition of Pb$_5$Ge$_3$O$_{11}$ crystal. The calculations of phonons and Born effective charges of the paraelectric phase allow us to identify a polar…

Materials Science · Physics 2024-01-18 Mauro Fava , William Lafargue-Dit-Hauret , Aldo H. Romero , Eric Bousquet

Ferroelectrics form domain patterns that minimize their energy subject to imposed boundary conditions. In a linear, constrained theory, that neglects domain wall energy, periodic domain patterns in the form of multi-rank laminates can be…

Materials Science · Physics 2018-03-20 Ananya Renuka Balakrishna , John E. Huber , Ingo Münch

In this work, a way to improve the piezoelectric properties of Bi0.5Na0.5TiO3 (BNT) is demonstrated by introducing a new poling protocol. A customized corona poling unit with a low temperature (77 K) sample stage is suggested. Using this…

Materials Science · Physics 2022-06-07 Mukesh Kumari , Ratnamala Chatterjee

The origin of the very large piezoelectric response observed in the vicinity of the morphotropic phase boundary (MPB) in perovskite lead zirconate titanate and related systems has been under intensive studies. Polarization rotation ideas…

Materials Science · Physics 2009-11-13 Johannes Frantti , Yukari Fujioka , Risto M. Nieminen

We report on structural, magnetic, dielectric, and thermodynamic properties of (Eu:Y)MnO3 for Y doping levels 0 <= x < 1. This system resembles the multiferroic perovskite manganites RMnO3 (with R= Gd, Dy, Tb) but without the interference…

Strongly Correlated Electrons · Physics 2015-06-25 J. Hemberger , F. Schrettle , A. Pimenov , P. Lunkenheimer , V. Yu. Ivanov , A. A. Mukhin , A. M. Balbashov , A. Loidl

Structural phase transformations in (001)-oriented (1-x)Pb(Mg1/3Nb2/3O3)-32%PbTiO3 (PMN-x%PT) crystals have been investigated by x-ray diffraction. A C->T->MC sequence was observed in both the field-cooled (FC) and zero-field-cooled (ZFC)…

Materials Science · Physics 2009-11-10 Hu Cao , Feiming Bai , Jiefang Li , D. Viehland , Guangyong Xu , H. Hiraka , G. Shirane

The symmetric studies on the structure-property relationship of the unpoled and poled states of 0.67BiFeO3-0.33BaTiO3 (0.67BF-0.33BT) were conducted to understand the origin of the morphotropic phase boundary (MPB) in BF-BT. A typical…

Materials Science · Physics 2020-03-24 Yongxing Wei , Jiahao Shen , Chenxing Bai , Changqing Jin , Weitong Zhu , Ye Tian , Gang Xu

Structural phase transformations of [110] electric field cooled Pb(Mg1/3Nb2/3)O3-30%PbTiO3 (PMN-30%PT) crystals have been performed by x-ray diffraction in a field-cooled (FC) condition. A phase sequence of…

Materials Science · Physics 2009-11-11 Hu Cao , Feiming Bai , Naigang Wang , Jiefang Li , D. Viehland , Guangyong Xu , Gen Shirane

Millimeter size single crystals of double perovskite La2NiMnO6 (LNMO) were grown by the High Temperature Solution Growth Method. The magnetic measurements and polarized Raman spectra between 5 and 350K provide evidence that the crystals…

Materials Science · Physics 2009-05-05 M. N. Iliev , M. M. Gospodinov , M. P. Singh , J. Meen , K. D. Truong , P. Fournier , S. Jandl

The distorted phases of monolayer 1T-MoS$_2$ have distinct electronic properties, with potential applications in optoelectronics, catalysis, and batteries. We theoretically investigate the use of Ni-doping to generate distorted 1T phases,…

Materials Science · Physics 2024-06-13 Rijan Karkee , David A. Strubbe

3$d$ based double perovskite materials have received much attention in recent years due to their exotic magnetic structure and magneto-electric coupling. In this work we have prepared and studied the nano-crystalline sample of…

Strongly Correlated Electrons · Physics 2019-09-25 Ilyas Noor Bhatti , Imtiaz Noor Bhatti , Rabindra Nath Mahato , M. A. H. Ahsan

Charge-neutral 180$^\circ$ domain walls that separate domains of antiparallel polarization directions are common structural topological defects in ferroelectrics. In normal ferroelectrics, charged 180$^\circ$ domain walls running…

Materials Science · Physics 2017-06-07 Shi Liu , R. E. Cohen

Using density functional calculations we explore the properties of as-yet-unsynthesized $3d - 5d$ ordered double perovskites ($A_2BB'$O$_6$) with highly polarizable Bi$^{3+}$ ions on the $A$ site. We find that the Bi$_2$NiReO$_6$ and…

Materials Science · Physics 2015-03-13 Marjana Ležaić , Nicola A. Spaldin

A phenomenological treatment of domain walls based on the Ginzburg-Landau-Devonshire theory is developed for uniaxial, trigonal ferroelectrics lithium niobate and lithium tantalate. The contributions to the domain wall energy from…

Materials Science · Physics 2009-11-11 David A Scrymgeour , Venkatraman Gopalan , Amit Itagi , Avadh Saxena , Pieter J Swart

Polarized absorption spectra of single-crystal Nd0.5Gd0.5Fe3(BO3)4 were studied in the region of transition 4I9/2-(4G5/2+2G7/2) in Nd3+ ion as a function of temperature (2-34 K) and magnetic field (0-65 kOe). Spectra of natural circular…

Strongly Correlated Electrons · Physics 2014-07-18 A. V. Malakhovskii , S. L. Gnatchenko , I. S. Kachur , V. G. Piryatinskaya , A. L. Sukhachev , V. L. Temerov