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We apply a recently proposed theoretical concept and numerical approach to obtain time delays in extreme ultraviolet (XUV) photoionization of an electron in a short- or long-range potential. The results of our numerical simulations on a…

Atomic Physics · Physics 2015-06-12 Jing Su , Hongcheng Ni , Andreas Becker , Agnieszka Jaron-Becker

This tutorial presents an introduction to the interaction of light and matter on the attosecond timescale. Our aim is to detail the theoretical description of ultra-short time-delays, and to relate these to the phase of extreme ultraviolet…

Atomic Physics · Physics 2012-07-20 J. M. Dahlström , A. L'Huillier , A. Maquet

We study the temporal aspects of laser-assisted extreme ultraviolet (XUV) photoionization using attosecond pulses of harmonic radiation. The aim of this paper is to establish the general form of the phase of the relevant transition…

We consider the time delay of electron detachment from a Coulomb center and two-center systems in the process of ionization. It is shown that the attosecond streaking, most usual method of time delay measure, can be formally described by…

Atomic Physics · Physics 2015-06-15 Vladislav V. Serov , Vladimir L. Derbov , Tatyana A. Sergeeva

Relative phases of atomic above-threshold ionization wavepackets have been investigated in a recent experiment [L. J. Zipp, A. Natan, and P. H. Bucksbaum, Optica \textbf{1}, 361-364 (2014)] exploiting interferences between different…

Atomic Physics · Physics 2021-11-10 S. D. López , S. Donsa , S. Nagele , D. G. Arbó , J. Burgdörfer

The generation of a streaking spectrogram is based on energy absorption from the streaking laser. Investigating this absorption we show rigorously under which condition the measured time shift is independent of properties of the streaking…

Atomic Physics · Physics 2020-09-16 Ulf Saalmann , Jan M Rost

Ultrafast processes in matter, such as the electron emission following light absorption, can now be studied using ultrashort light pulses of attosecond duration ($10^{-18}$s) in the extreme ultraviolet spectral range. The lack of spectral…

We study laser-assisted photodetachment time delays by attosecond pulse trains from the closed-shell negative ions F- and Cl-. We investigate the separability of the delay into two contributions: (i) the Wigner-like delay associated with…

Atomic Physics · Physics 2017-09-13 Eva Lindroth , Jan Marcus Dahlström

We propose a method to study the tunneling process by analyzing the time-dependent ionization yield in circularly polarized laser. A numerical calculation shows that for an atom exposed to a long laser pulse, if its initial electronic state…

Atomic Physics · Physics 2016-06-08 MingHu Yuan , PeiPei Xin , TianShu Chu , HongPing Liu

We use a Wigner distribution-like function based on the strong field approximation theory to obtain the time-energy distributions and the ionization time distributions of electrons ionized by an XUV pulse alone and in the presence of an…

Atomic Physics · Physics 2021-09-01 L. Guo , Y. Jia , M. Q. Liu , X. Y. Jia , S. L. Hu , R. H. Lu , S. S. Han , J. Chen

Time-delays in the photoionization of molecules are investigated. As compared to atomic ionization, the time-delays expected from molecular ionization present a much richer phenomenon, with a strong spatial dependence due to the anisotropic…

Atomic Physics · Physics 2017-02-14 P. Hockett , E. Frumker , D. M. Villeneuve , P. B. Corkum

In scattering theory, the Wigner-Smith time delay, calculated through a phaseshift derivative or its multichannel generalization, has been demonstrated to measure the amount of delay or advance experienced by colliding particles during…

Atomic Physics · Physics 2025-11-25 Karim I. Elghazawy , Chris H. Greene

No, we cannot! The concept of Wigner time delay was introduced in scattering theory to quantify the delay or advance of an incoming particle in its interaction with the scattering potential. It was assumed that this concept can be…

Quantum Physics · Physics 2022-10-12 B. Fetić , W. Becker , D. B. Milošević

It is shown that it is feasible to use ultrashort time delay between two XUV femtosecond pulses in order to control two photon resonant ionization. The proposal is demonstrated on the spectrum of Helium, in terms of nonperturbative…

Atomic Physics · Physics 2019-08-22 Theodoros Mercouris , Yannis Komninos , Cleanthes A. Nicolaides

Photoionization is a key step in many attosecond processes. Accurately determining the photoionization time delay is critical to understanding electron dynamics during and after ionization and can guide future efforts to manipulate electron…

Atomic Physics · Physics 2026-02-26 J. Aygun , D. Yaacoub , A. L. Harris

Attosecond photoionisation time delays reveal information about the potential energy landscape an outgoing electron wavepacket probes upon ionisation. In this study we experimentally quantify, for the first time, the dependence of the time…

Upon absorbing a photon, the ionized electron sails through the target force field in attoseconds to reach free space. This navigation probes details of the potential landscape that get imprinted into the phase of the ionization amplitude.…

Atomic Physics · Physics 2024-12-12 Sajad Azizi , Mohamed El-Amine Madjet , Zheng Li , Jan M. Rost , Himadri S. Chakraborty

The electron dynamics in the classically forbidden region during relativistic tunnel-ionization is investigated. The classical forbidden region in the relativistic regime is identified by defining a gauge invariant total energy operator.…

We analyze two-center interference effects in the yields of ionization of a dissociating hydrogen molecular ion by an ultrashort VUV laser pulse. To this end, we performed numerical simulations of the time-dependent Schr\"odinger equation…

Quantum Physics · Physics 2015-05-27 A. Picón , A. Bahabad , H. C. Kapteyn , M. M. Murnane , A. Becker

Electrons in atoms and molecules can not react immediately to the action of intense laser field. A time lag (about 100 attoseconds) between instants of the field maximum and the ionization-rate maximum emerges. This lag characterizes the…

Atomic Physics · Physics 2021-04-01 J. Y. Che , C. Chen , S. Wang , G. G. Xin , Y. J. Chen
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