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Shape resonances in photoionization of atoms and molecules arise from a particular geometry of the ionic potential which traps the receding photoelectron in a quasi-bound state in a particular partial wave. This mechanism allows us to…

Atomic Physics · Physics 2026-03-03 Anatoli S. Kheifets , Stephen Catsamas

Although many physical arguments account for using a modified definition of time delay in multichannel-type scattering processes, one can hardly find rigorous results on that issue in the literature. We try to fill in this gap by showing,…

Mathematical Physics · Physics 2009-11-11 Rafael Tiedra de Aldecoa

The Eisenbud-Wigner-Smith (EWS) time delay of photoemission depends on the phase term of the matrix element describing the transition. Because of an interference process between partial channels, the photoelectrons acquire a spin…

Mesoscale and Nanoscale Physics · Physics 2018-12-12 Mauro Fanciulli , J. Hugo Dil

We analyze the time delay between emission of photoelectrons from the outer valence $ns$ and $np$ sub-shells in noble gas atoms following absorption of an attosecond XUV pulse. By solving the time dependent Schr\"odinger equation and…

Atomic Physics · Physics 2010-12-07 A. S. Kheifets , I. A. Ivanov

Delay time is defined as a time that a wave spent in a scattering medium before it escapes, and this can be derived by the energy derivative of the phase of the scattering wave. Considering the complex reflection amplitude…

Optics · Physics 2018-12-31 Prabhakar Pradhan , Peeyush Sahay , Huda M. Almabadi

Time delays of electrons emitted from an isotropic initial state and leaving behind an isotropic ion are assumed to be angle-independent. Using an interferometric method involving XUV attosecond pulse trains and an IR probe field in…

We investigate the limitations arising from atomic collisions on the storage and delay times of probe pulses in EIT experiments. We find that the atomic collisions can be described by an effective decay rate that limits storage and delay…

Quantum Physics · Physics 2009-11-07 D. C. Roberts , T. Gasenzer , K. Burnett

Intense, ultrashort pulses of 800 nm laser light (12 fs, $\sim$4 optical cycles) of peak intensity 5$\times$10$^{14}$ W cm$^{-2}$ have been used to irradiate gas-phase Xe$_n$ clusters ($n$=500-25,000) so as to induce multiple ionization and…

Atomic and Molecular Clusters · Physics 2015-05-19 D. Mathur , F. A. Rajgara

A clear consensus on how long it takes a particle to tunnel through a potential barrier has never been so urgently required, since the electron dynamics in strong-field ionization can be resolved on attosecond time-scale in experiment and…

Atomic Physics · Physics 2019-03-19 Xiaolei Hao , Zheng Shu , Weidong Li , Jing Chen

Streaked photoemission metrology allows the observation of an apparent relative time delay between the detection of photoelectrons from different initial electronic states. This relative delay is obtained by recording the photoelectron…

Other Condensed Matter · Physics 2015-05-28 Chang-hua Zhang , Uwe Thumm

We investigate laser induced nonsequential multiple ionization using a simple statistical model in which an electron recollides inelastically with its parent ion. In this collision, it thermalizes with the remaining $N-1$ bound electrons…

Atomic Physics · Physics 2007-05-23 C. Figueira de Morisson Faria , X. Liu

Measuring the time it takes to remove an electron from an atom or molecule during photoionization using newly developed attosecond spectroscopies has been a focus of many recent experiments. However, the outcome of such measurement depends…

Atomic Physics · Physics 2017-03-08 Lisa Torlina , Olga Smirnova

Time-resolved studies have so far relied on rapidly triggering a photo-induced dynamic in chemical or biological ions or molecules and subsequently probing them with a beam of fast moving photons or electrons that crosses the studied…

Chemical Physics · Physics 2021-03-19 Hazem Daoud , R. J. Dwayne Miller

We use the soft photon approximation to extract the Wigner time delay from atomic two-color photoionization experiments. Unlike the strong field approximation, the present method does not require introduction of the Coulomb-laser coupling…

Atomic Physics · Physics 2013-05-10 I. A. Ivanov , A. S. Kheifets

We use numerical simulations to test a broad range of plausible observational strategies designed to measure the time delay between the images of gravitationally lensed quasars. Artificial quasar light curves are created along with…

Astrophysics · Physics 2009-11-10 A. Eigenbrod , F. Courbin , C. Vuissoz , G. Meylan , P. Saha , S. Dye

Attosecond streaking of atomic photoemission holds the promise to provide unprecedented information on the release time of the photoelectron. We show that attosecond streaking phase shifts indeed contain timing (or spectral phase)…

The development of ultra-short intense laser sources in the visible and extreme ultraviolet (XUV) spectral range led to fascinating studies in laser-matter interactions and attosecond science. In the majority of these studies the system…

To measure and control the electron motion in atoms and molecules by the strong laser field on the attosecond time scale is one of the research frontiers of atomic and molecular photophysics. It involves many new phenomena and processes and…

Atomic Physics · Physics 2022-03-30 Chao Chen , Jiayin Che , Shang Wang , Guoguo Xin , Yanjun Chen

Photoionization of matter is one of the fastest electronic processes in nature. Experimental measurements of photoionization dynamics have become possible through attosecond metrology. However, all experiments reported to date contain a…

Quantum Physics · Physics 2025-02-11 Meng Han , Jia-Bao Ji , Leung Chung Sum , Kiyoshi Ueda , Hans Jakob Wörner

Attosecond streaking is one of the most fundamental processes in attosecond science allowing for a mapping of temporal (i.e. phase) information on the energy domain. We show that on the single-particle level attosecond streaking time shifts…