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Control of the crystalline orientation of nitrogen-vacancy (NV) defects in diamond is here demonstrated by tuning the temperature of chemical vapor deposition (CVD) growth on a (113)-oriented diamond substrate. We show that preferential…

Materials Science · Physics 2018-07-02 S. Chouaieb , L. J. Martínez , W. Akhtar , I. Robert-Philip , A. Dréau , O. Brinza , J. Achard , A. Tallaire , V. Jacques

In semiconductors, quantum confinement can greatly enhance the interaction between band carriers (electrons and holes) and dopant atoms. One manifestation of this enhancement is the increased stability of exciton magnetic polarons in…

Mesoscale and Nanoscale Physics · Physics 2017-04-27 W. D. Rice , W. Liu , V. Pinchetti , D. R. Yakovlev , V. I. Klimov , S. A. Crooker

We present a general theory for using an optically pumped diamond nitrogen-vacancy center as a tunable, non-equilibrium bath to control a variety of nuclear spin dynamics (such as dephasing, relaxation, squeezing, polarization, etc.) and…

Quantum Physics · Physics 2019-08-17 Ping Wang , Jiangfeng Du , Wen Yang

In CuCl bulk crystal negatively charged excitons (trions $X^-$) can be induced by the resonant optical excitation of extra electrons in conduction band minimum. In the case of light polarization and due to the top valence band structure of…

Materials Science · Physics 2009-11-11 W. Ungier , R. Buczko

We demonstrate that efficient optical pumping of nuclear spins in semiconductor quantum dots (QDs) can be achieved by resonant pumping of optically "forbidden" transitions. This process corresponds to one-to-one conversion of a photon…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 E. A. Chekhovich , M. N. Makhonin , K. V. Kavokin , A. B. Krysa , M. S. Skolnick , A. I. Tartakovskii

Highly sensitive nuclear spin detection is crucial in many scientific areas including nuclear magnetic resonance spectroscopy (NMR), imaging (MRI) and quantum computing. The tiny thermal nuclear spin polarization represents a major obstacle…

The current work proposes a method for pulsed-light polarization of nitrogen-vacancy (NV) center electron spin. To evaluate the influence of pulsed spin polarization, we establish a polarization evaluation index based on polarizability and…

Applied Physics · Physics 2020-10-05 Zhang Jixing , Liu Tianzheng , Xu Lixia , Bian Guodong , Fan Pengcheng , Li Mingxin , Zhang Ning , Yuan Heng

Nuclear magnetism underpins areas such as medicine in magnetic resonance imaging (MRI). Hyperpolarization of nuclei enhances the quantity and quality of information that can be determined from these techniques by increasing their signal to…

Superconductivity · Physics 2025-01-16 John Z. Myers , Kai Buckenmaier , Andrey N. Pravdivtsev , Markus Plaumann , Rainer Körber

The production of negative ions is of significant interest for applications including mass spectrometry, particle acceleration, material surface processing, and neutral beam injection for magnetic confinement fusion. Methods to improve the…

Nitrogen vacancy (NV-) color centers in diamond are a prime candidate for use in quantum information devices, owing to their spin-1 ground state, straightforward optical initialization and readout, and long intrinsic coherence times in a…

Quantum Physics · Physics 2015-06-19 Anna J. Parker , Hai-Jing Wang , Yiran Li , Alexander Pines , Jonathan P. King

At low magnetic field, metastability exchange optical pumping of helium-3 is known to provide high nuclear polarizations for pressures around 1 mbar. In a recent paper, we demonstrated that operating at 1.5 T can significantly improve the…

Atomic Physics · Physics 2016-08-16 Marie Abboud , Alice Sinatra , Geneviève Tastevin , Pierre-Jean Nacher , Xavier Maître

A recently proposed theory of chiral discrimination in NMR spectroscopy based on the detection of a molecular electric polarization $\mathbf{P}$ rotating in a plane perpendicular to the NMR magnetic field [A. D. Buckingham, J. Chem. Phys.…

Chemical Physics · Physics 2016-04-26 Alessandro Soncini , Simone Calvello

Herein, we report on the improvement of structural quality and enhancement of photoluminescence (PL) emission for an optimally N doped nanocrystalline diamond (NCD) film. Pure and N doped nanocrystalline diamond films are synthesized on Si…

Materials Science · Physics 2020-06-05 K. Ganesan , P. K. Ajikumar , S. K. Srivatava , P. Magudapathy

Sensing based on Nitrogen-Vacancy (NV) centers in nanodiamonds (NDs) offers significant potential across various applications. However, optimizing their quantum-optical properties remains challenging. This study focuses on enhancing and…

We report high steady-state nuclear polarization of 1 torr $^3$He gas nuclei via metastability-exchange optical pumping at magnetic fields above 2 T. The introduction of highly polarized $^3$He gas into Brookhaven's Electron Beam Ion Source…

Instrumentation and Detectors · Physics 2019-04-15 J. D. Maxwell , J. Alessi , G. Atoian , E. Beebe , C. S. Epstein , R. G. Milner , M. Musgrave , A. Pikin , J. Ritter , A. Zelenski

The negatively-charged nitrogen vacancy (NV$^-$) centre in diamond is a remarkable optical quantum sensor for a range of applications including, nanoscale thermometry, magnetometry, single photon generation, quantum computing, and…

Optical pumping by blackbody radiation is a feature shared by all polar molecules and fundamentally limits the time that these molecules can be kept in a single quantum state in a trap. To demonstrate and quantify this, we have monitored…

High concentration of negatively charged nitrogen-vacancy ($\text{NV}^{-}$) centers was created in diamond single crystals containing approximately 100 ppm nitrogen using electron and neutron irradiation and subsequent thermal annealing in…

Phosphorus-doped diamond is relevant for applications in sensing, optoelectronics and quantum photonics, since the unique optical properties of color centers in diamond can be combined with the n-type conductivity attained by the inclusion…

New-generation X-ray polarimeters currently under development promise to open a new window in the study of high-energy astrophysical sources. Among them, neutron stars appear particularly suited for polarization measurements. Radiation from…

High Energy Astrophysical Phenomena · Physics 2015-09-24 Roberto Taverna , Roberto Turolla , Denis Gonzalez Caniulef , Silvia Zane , Fabio Muleri , Paolo Soffitta