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Electrons in certain two-dimensional crystals possess a pseudospin degree of freedom associated with the existence of two inequivalent valleys in the Brillouin zone. If, as in monolayer MoS2, inversion symmetry is broken and time-reversal…

Disordered Systems and Neural Networks · Physics 2015-09-28 Thomas Olsen , Ivo Souza

The polarization analysis of optical transitions in monolayer and bilayer transition-metal dichalcogenides provides invaluable information on the spin and valley (pseudospin) degrees of freedom. To explain optical properties of a given…

Materials Science · Physics 2015-10-06 Hanan Dery , Yang Song

Monolayers of transition metal dichalcogenides (TMDCs) are atomically thin direct-gap semiconductors with potential applications in nanoelectronics, optoelectronics, and electrochemical sensing. Recent theoretical and experimental efforts…

Mesoscale and Nanoscale Physics · Physics 2013-02-26 Sanfeng Wu , Chunming Huang , Grant Aivazian , Jason S Ross , David H Cobden , Xiaodong Xu

A direct band gap, remarkable light-matter coupling as well as strong spin-orbit and Coulomb interaction establish two-dimensional (2D) crystals of transition metal dichalcogenides (TMDs) as an emerging material class for fundamental…

We investigate electrical gating of photoluminescence and optical absorption in monolayer molybdenum disulfide (MoS$_2$) configured in field effect transistor geometry. We observe an hundredfold increase in photoluminescence intensity and…

Mesoscale and Nanoscale Physics · Physics 2012-11-19 A. K. M. Newaz , D. Prasai , J. I. Ziegler , D. Caudel , S. Robinson , R. F. Haglund , K. I. Bolotin

The topological properties of a material's electronic structure are encoded in its Berry curvature, a quantity which is intimately related to the transverse electrical conductivity. In transition metal dichalcogenides with broken inversion…

Mesoscale and Nanoscale Physics · Physics 2020-10-21 Fei Xue , V. P. Amin , P. M. Haney

We report experimental evidences on selective occupation of the degenerate valleys in MoS2 monolayers by circularly polarized optical pumping. Over 30% valley polarization has been observed at K and K' valley via the polarization resolved…

Mesoscale and Nanoscale Physics · Physics 2013-04-17 Hualing Zeng , Junfeng Dai , Wang Yao , Di Xiao , Xiaodong Cui

Spins confined to atomically-thin semiconductors are being actively explored as quantum information carriers. In transition metal dichalcogenides (TMDCs), the hexagonal crystal lattice gives rise to an additional valley degree of freedom…

Mesoscale and Nanoscale Physics · Physics 2023-06-29 Radha Krishnan , Sangram Biswas , Yu-Ling Hsueh , Hongyang Ma , Rajib Rahman , Bent Weber

Heavy metal-based two-dimensional van der Waals materials have a large, coupled spin and valley Hall effect (SVHE) that has potential use in spintronics and valleytronics. Optical measurements of the SVHE have largely been performed below…

Mesoscale and Nanoscale Physics · Physics 2022-02-25 Xintong Li , Zhida Liu , Yihan Liu , Suyogya Karki , Xiaoqin Li , Deji Akinwande , Jean Anne C. Incorvia

The quantum magnetotransport properties of a monolayer of molybdenum disulfide are derived using linear response theory. Especially, the effect of topological terms on longitudinal and Hall conductivity is analyzed. The Hall conductivity…

Mesoscale and Nanoscale Physics · Physics 2016-08-22 SK Firoz Islam , Colin Benjamin

The valley degree of freedom and the possibility of spin-valley coupling of solid materials have attracted growing interest, and the relaxation dynamics of spin- and valley-polarized states has become an important focus of recent studies.…

Materials Science · Physics 2018-09-24 Dongbin Shin , Hosub Jin , Noejung Park

Controlling the momentum of carriers in semiconductors, known as valley polarization, is a new resource for optoelectronics and information technologies. Materials exhibiting high polarization are needed for valley-based devices. Few-layer…

Mesoscale and Nanoscale Physics · Physics 2022-12-14 Rasmus H. Godiksen , Shaojun Wang , T. V. Raziman , Jaime Gómez Rivas , Alberto G. Curto

In this letter we present photoluminescence measurements with different excitation energies on single-layer MoS$_2$ and MoSe$_2$ in order to examine the resonance behavior of the conservation of circular polarization in these transition…

Applied Physics · Physics 2018-11-06 Hans Tornatzky , Anne-Marie Kaulitz , Janina Maultzsch

We calculate the magneto-optical conductivity and electronic density of states for silicene, the silicon equivalent of graphene, and similar crystals such as germanene. In the presence of a perpendicular magnetic field and electric field…

Mesoscale and Nanoscale Physics · Physics 2013-05-10 Calvin J. Tabert , Elisabeth J. Nicol

Manipulating spin polarization of electrons in nonmagnetic semiconductors by means of electric fields or optical fields is an essential theme of the conceptual nonmagnetic semiconductor-based spintronics. Here we experimentally demonstrate…

Mesoscale and Nanoscale Physics · Physics 2016-03-31 Xie Lu , Xiaodong Cui

MoS2 atomic layers have recently attracted much interest because of their two-dimensional structure as well as tunable optical, electrical, and mechanical properties for next generation electronic and electro-optical devices. Here we have…

Materials Science · Physics 2016-11-15 Chih-Shan Tan , Yu-Jung Lu , Chun-Chi Chen , Pei-Hsuan Liu , Shangjr Gwo , Guang-Yu Guo , Lih-Juann Chen

The electronic properties of ultrathin crystals of molybdenum disulfide consisting of N = 1, 2, ... 6 S-Mo-S monolayers have been investigated by optical spectroscopy. Through characterization by absorption, photoluminescence, and…

Materials Science · Physics 2015-05-18 Kin Fai Mak , Changgu Lee , James Hone , Jie Shan , Tony F. Heinz

Adding a small subdominant quadratic in momentum term to a dominant linear Dirac dispersion curve affects conduction and valence band differently and leads to an hourglass-like structure for energy as a function of momentum. This applies to…

Mesoscale and Nanoscale Physics · Physics 2013-07-09 Zhou Li , J. P. Carbotte

The optical selection rules obeyed by two-dimensional materials with spin-valley coupling enable the selective excitation of carriers. We show that six members of the monolayer MA2Z4 (M = Mo and W; A = C, Si, and Ge; Z = N, P, and As)…

Materials Science · Physics 2022-06-15 Jiaren Yuan , Qingyuan Wei , Minglei Sun , Xiaohong Yan , Yongqing Cai , Lei Shen , Udo Schwingenschlögl

We present a study on the growth and characterization of high-quality single-layer MoS$_2$ with a single orientation, i.e. without the presence of mirror domains. This single orientation of the MoS$_2$ layer is established by means of x-ray…