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Coherent conversion between a Raman pump field and its Stokes field is observed in a Raman process with a strong atomic spin wave initially prepared by another Raman process operated in the stimulated emission regime. The oscillatory…
A quantum model of the Raman process with the independent Stokes and anti-Stokes nonlinear interactions is developed to study nonclassical correlations between the photons in the Stokes and anti-Stokes fields. The role of the laser pump…
We present a quantum-mechanical model that describes fiber-based frequency conversion by four-wave-mixing Bragg scattering in the presence of Raman interactions. In the case of continuous-wave pumps we find closed-form expressions for the…
A general fundamental relation connecting the correlation of Stokes and anti-Stokes modes to the quantum statistical behavior of vibration and pump modes in Raman-active materials is derived. We show that under certain conditions this…
In spontaneous Raman process in atomic cell at high gain, both the Stokes field and the accompanying collective atomic excitation (atomic spin wave) are coherent. We find that, due to the spontaneous nature of the process, the phases of the…
We study Raman scattering in active media placed in proximity of different types of metal nanostructures, at wavelengths that display either Fabry-Perot or plasmonic resonances, or a combination of both. We use a semi-classical approach to…
When a laser pump beam of sufficient intensity is incident on a Raman-active medium such as hydrogen gas, a strong Stokes signal, red-shifted by the Raman transition frequency {\Omega}$_R$, is generated. This is accompanied by the creation…
Backward stimulated Raman scattering in gases provides a promising route to compression and amplification of a Stokes seed-pulse by counter-propagating against a pump-pulse, as has been already demonstrated in various platforms, mainly in…
Implementing stimulated Raman scattering in a low-loss microresonator could lead to Raman lasing. Here, we report the demonstration of an efficient Raman laser with $>50 \%$ power efficiency in an integrated silicon carbide platform for the…
Stimulated Raman scattering, employing a pump and a Stokes beam, exhibits itself through both the Raman loss observed in the pump beam and the Raman gain in the Stokes beam. This phenomenon finds application in spectroscopy for chemical…
Robust stimulated Raman exact passages are requisite for controlling nonlinear quantum systems, with the wide applications ranging from ultracold molecules, non-linear optics to superchemistry. Inspired by shortcuts to adiabaticity, we…
We demonstrate a novel technique of coherent Raman spectroscopy with a femtosecond laser. We apply to a molecular sample a sequence of pairs of ultrashort excitation and probe pulses, with a linearly increasing time delay between the two…
State-preserving frequency conversion in the optical domain is a necessary component in many configurations of quantum information processing and communication. Thus far, nonlinear crystals are used for this purpose. Here, we report on a…
We discuss layout and performance of a high-resolution Stimulated Raman Loss spectrometer that has been newly developed for accurate studies of spectral lineshapes and line center frequencies of hydrogen isotopologues and in general of…
We propose a method for increasing the Raman scattering from an ensemble of molecules by up to four orders of magnitude. Our method requires an additional coherent source of IR radiation with the half-frequency of the Stokes shift. This…
We present mirror and beamsplitter pulse designs that improve the fidelity of atom interferometry and increase its tolerance of systematic inhomogeneities. These designs are demonstrated experimentally with a cold thermal sample of…
We investigate the evolution of coherence property of noise-seeded Stokes wave in short (< 1 ps) and long pulse (> 1 ps) regimes. Nonlinear equations expressing the evolution of pump and Stokes wave are solved numerically for both the…
We demonstrate microwave-to-optical conversion using six-wave mixing in $^{87}$Rb atoms where the microwave field couples to two atomic Rydberg states, and propagates collinearly with the converted optical field. We achieve a photon…
Many reports on stimulated Raman scattering in mixtures of Raman-active and noble gases indicate that the addition of a dispersive buffer gas increases the phase-mismatch to higher-order Stokes and antiStokes sidebands, resulting in…
We demonstrate a new high efficiency architecture for cascaded Raman fiber lasers based on a single pass cascaded amplifier configuration. Conversion is seeded at all intermediate Stokes wavelengths using a multi-wavelength seed source. A…