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The efficiency of the frequency conversion process at the heart of Raman heterodyne spectroscopy was improved by nearly four orders of magnitude by resonant enhancement of both the pump and signal optical fields. Our results using an erbium…
By using the inverse spectral transform, the SRS equations are solved and the explicit output data is given for arbitrary laser pump and Stokes seed profiles injected on a vacuum of optical phonons. For long duration laser pulses, this…
Two simultaneous three wave mixing processes are analyzed, where an input frequency is converted to an output frequency via an intermediate stage. By employing simultaneous phase-matching and an adiabatic modulation of the nonlinear…
This work investigates the utility of femtosecond pulse shaping in increasing the efficiency of Raman excitation of molecules in the strong-field interaction regime. We study experimentally and theoretically the effect of pulse shaping on…
A quantum amplifier usually adds extra noise inevitably through coupling to internal degrees of freedom while amplifying the signal. The introduction of quantum correlations can effectively suppress this extra noise. In this work, we…
We report coherent association of atoms into a single weakly bound NaCs molecule in an optical tweezer through an optical Raman transition. The Raman technique uses a deeply bound electronic excited intermediate state to achieve a large…
We propose a scheme of generating and verifying mesoscopic-level entanglement between two atomic ensembles using non-resonant stimulated Raman scattering. Entanglement can be generated by direct detection or balanced homodyne detection of…
By using spontaneous Raman processes in the high gain regime, we produce two independent Raman Stokes fields from an atomic ensemble. Temporal beating is observed between the two directly generated Stokes fields in a single realization. The…
We study the conversion of $^{40}$K and $^{87}$Rb atoms into stable molecules through the stimulated Raman adiabatic passage (STIRAP) in photoassociation assisted with Feshbach resonance. Starting with the mean-field Langrange density, we…
Raman transitions have a wide range of applications in atomic physics and have recently been proposed as a means for improving high-precision high-voltage measurements. Here, we present a theoretical analysis and a first experimental…
Frequency modulation coherent anti-Stokes Raman scattering (FM CARS) is presented, using a compact as well as fast and widely tunable fiber-based light source. With this light source Raman resonances between 700 cm$^{-1}$ and 3200 cm$^{-1}$…
We present general analytical expressions of Stokes and anti-Stokes spectral photon-flux densities that are spontaneously generated by a single monochromatic pump wave propagating in a single-mode optical fiber. We validate our results by…
Nonclassicality is studied through a quasidistribution of phases for the Raman process under both weak and strong pump conditions. In the former case, the solution is applicable to both resonant and off-resonant Raman processes, while…
Radiative transfer equations are derived and solved for the stimulated Raman scattering of water maser lines in the astrophysical plasmas with electron density of about 10^6 - 10^7 cm-3. In stimulated Raman scattering, the energy of water…
We investigate the arrival statistics of Stokes (S) and anti-Stokes (aS) Raman photons generated in diamond membranes. Strong quantum correlations between the S and aS signals are observed, which implies that the two processes share the…
The temperature dependence of the asymmetry between Stokes and anti-Stokes Raman scattering can be exploited for self-calibrating, optically-based thermometry. In the context of cavity optomechanics, we observe the cavity-enhanced…
Compact, power efficient and fiber compatible lasers, wavelength converters and amplifiers are vital ingredients for the future fiber optic systems and networks. Nonlinear optical effects, like Raman scattering and parametric four wave…
We present an experimental demonstration of converting a microwave field to an optical field via frequency mixing in a cloud of cold $^{87}$Rb atoms, where the microwave field strongly couples to an electric dipole transition between…
Quantum memories with high efficiency and fidelity are essential for long-distance quantum communication and information processing. Techniques have been developed for quantum memories based on atomic ensembles. The atomic memories relying…
Raman phonons are quantized molecular motions that arise from the inelastic scattering of light and mediate a wide range of spectroscopic and nonlinear optical phenomena. These can play a major role in frequency-conversion processes, but…