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Related papers: Stable all nitrogen metallic salt at terapascal pr…

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We investigate the binary phase diagram of helium and iron using first-principles calculations. We find that helium, which is a noble gas and inert at ambient conditions, forms stable crystalline compounds with iron at terapascal pressures.…

Materials Science · Physics 2018-07-05 Bartomeu Monserrat , Miguel Martinez-Canales , Richard J. Needs , Chris J. Pickard

Transition metal nitrides have attracted much interest of the scientific community for their intriguing properties and technological applications. Here we focus on yttrium dinitride (YN$_{2}$) and its formation and structural transition…

Materials Science · Physics 2020-12-18 Francesca Menescardi , Emma Ehrenreich-Petersen , Davide Ceresoli

A study of high pressure solid Te was carried out at room temperature using Raman spectroscopy and Density Functional Theory (DFT) calculations. The analysis of the P-dependence of the experi- mental phonon spectrum reveals the occurrence…

We report direct experimental evidence of antiferroelectric to paraelectric phase transition under pressure in NaNbO3 using neutron diffraction at room temperature. The paraelectric phase is found to stabilize above 8 GPa and its crystal…

Materials Science · Physics 2015-06-11 S. K. Mishra , M. K. Gupta , R. Mittal , S. L. Chaplot , Thomas Hansen

We have studied solid hydrogen up to pressures of 300 GPa and temperatures of 350 K using density functional theory methods and have found "mixed structures" that are more stable than those predicted earlier. Mixed structures consist of…

Materials Science · Physics 2012-06-20 Chris J. Pickard , Miguel Martinez-Canales , Richard J. Needs

Previously known to form only under high pressure synthetic conditions, here we report that the T'-type 214-structure cuprate based on the rare earth atom Tb is stabilized for ambient pressure synthesis through partial substitution of Pd…

Pressure-induced superconductivity and structural phase transitions in phosphorous (P) are studied by resistivity measurements under pressures up to 170 GPa and fully $ab-initio$ crystal structure and superconductivity calculations up to…

Computational searches for structures of solid oxygen under pressures in the multi TPa range have been carried out using density-functional-theory methods. We find that molecular oxygen persists to about 1.9 TPa at which it transforms into…

Materials Science · Physics 2012-07-06 Jian Sun , Miguel Martinez-Canales , Dennis D. Klug , Chris J. Pickard , Richard J. Needs

We study the electronic and lattice dynamical properties of compressed solid germane in the pressure range up to 200 GPa with density functional theory. A stable metallic structure, Aba2, with a base-centered orthorhombic symmetry was found…

Superconductivity · Physics 2008-05-01 Chao Zhang , Yanling Li , Xiaojia Chen , Ruiqin Zhang , Haiqing Lin

Stabilizing nitrogen-rich compound crystals under conventional conditions is a key issue in the development and application of high-energy density materials (HEDMs). Herein, a two-dimensional double-layer interlocked Li4(N5)2 nitrogen-rich…

Materials Science · Physics 2024-12-04 Zhen Gong , Baiqiang Liu , Xinrui Yang , Hongbo Jing , Ruiqi Xu , Zhigang Wang

How to stabilize nitrogen-rich high-energy-density molecules under conventional conditions is particularly important for the energy storage and conversion of such systems and has attracted extensive attention. In this work, our theoretical…

Chemical Physics · Physics 2023-08-10 Zhen Gong , Rui Wang , Famin Yu , Chenxi Wan , Xinrui Yang , Zhigang Wang

Lithium doped sodium niobate is an ecofriendly piezoelectric material that exhibits a variety of structural phase transitions with composition and temperature. We have investigated the phase stabilities of an important composition…

We have combined ab initio molecular dynamics with the intrinsic reaction coordinate in order to investigate the mechanisms of stability and pyrolysis of N$_{4}$-- N$_{120}$ fullerene-like nitrogen cages. The stability of the cages was…

Materials Science · Physics 2020-11-03 Konstantin Katin , Valeriy Merinov , Alexey Kochaev , Savas Kaya , Mikhail Maslov

Understanding the high-pressure behavior of C-H system is of great importance due to its key role in organic, bio-, petroleum and planetary chemistry. We have performed a systematic investigation of the pressure-composition phase diagram of…

Materials Science · Physics 2020-01-07 Anastasia S. Naumova , Sergey V. Lepeshkin , Artem R. Oganov

In this work we present an experimental study of structure and phase stability in ternary Cu-Sn-In alloys around 55 at.% Cu in the temperature range 100^{\circ}C < T < 550^{\circ}C. We have followed in real-time the sequence of phase…

Materials Science · Physics 2015-06-05 G. Aurelio , S. A. Sommadossi , G. J. Cuello

Uranium nitrides have been the subject of intense research owing to their potential applications as advanced nuclear fuels. However, the phase diagram of the U-N system at low temperature and high pressure still remains unclear. In this…

Computational Physics · Physics 2018-04-03 Dawei Zhou , JiaHui Yu , Chunying Pu , Yuling Song

Ab initio random structure searching with density functional theory was used to determine the zero-temperature structures of atomic metallic hydrogen from 500 GPa to 5 TPa. Including zero point motion in the harmonic approximation, we…

Materials Science · Physics 2015-05-20 Jeffrey M. McMahon , David M. Ceperley

Silver pentazolate, a high energy density compound containing cyclo-N5- anion, has recently been synthesized at ambient conditions. However, due to high sensitivity to irradiation, its crystal structure has not been determined. In this…

Materials Science · Physics 2021-11-03 Ashley S. Williams , Kien Nguyen Cong , Joseph M. Gonzalez , Ivan I. Oleynik

Studies of polynitrogen phases are of great interest for fundamental science and for the design of novel high energy density materials. Laser heating of pure nitrogen at 140 GPa in a diamond anvil cell led to the synthesis of a polymeric…

Sodium pentazolates NaN5 andNa2N5, new high energy density materials, are discovered during first principles crystal structure search for the compounds of varying amounts of elemental sodium and nitrogen. The pentazole anion N5- is…

Materials Science · Physics 2016-01-20 Brad A. Steele , Ivan I. Oleynik