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The behavior of mesoscopic particles dissolved in a dilute solution of long, flexible, and nonadsorbing polymer chains is studied by field-theoretic methods. For spherical and cylindrical particles the solvation free energy for immersing a…

Soft Condensed Matter · Physics 2009-10-31 A. Hanke , E. Eisenriegler , S. Dietrich

Monte Carlo simulations of crystal nuclei coexisting with the fluid phase in thermal equilibrium in finite volumes are presented and analyzed, for fluid densities from dense melts to the vapor. Generalizing the lever-rule for two-phase…

Statistical Mechanics · Physics 2017-11-01 Peter Koß , Antonia Statt , Peter Virnau , Kurt Binder

We study phase separation and transient gelation in a mixture consisting of polydisperse colloids and non-adsorbing polymers, where the ratio of the average size of the polymer to that of the colloid is approximately 0.063. Unlike what has…

Soft Condensed Matter · Physics 2011-06-23 S. M. Liddle , T. Narayanan , W. C. K. Poon

A new model for a colloidal size-asymmetric binary mixture is proposed: The Square-Shoulder-Asakura-Oosawa. This belongs to the larger class of non-additive hard-spheres models and has the property that its effective pair formulation is…

Soft Condensed Matter · Physics 2016-11-30 Riccardo Fantoni

When a colloid is mixed with a depletant such as a non-adsorbing polymer, one observes attractive effective interactions between the colloidal particles. If these particles are anisotropic, analysis of these effective interactions is…

Soft Condensed Matter · Physics 2016-09-08 Clement Law , Douglas J. Ashton , Nigel B. Wilding , Robert L. Jack

Large-scale Monte Carlo simulations of a phase-separating colloid-polymer mixture are performed and compared to recent experiments. The approach is based on effective interaction potentials in which the central monomers of self-avoiding…

Soft Condensed Matter · Physics 2007-05-23 R. L. C. Vink , A. Jusufi , J. Dzubiella , C. N. Likos

We discuss the reliability of integral-equation methods based on several commonly used closure relations in determining the phase diagram of coarse-grained models of soft-matter systems characterized by mutually interacting soft and…

Soft Condensed Matter · Physics 2015-10-28 Roberto Menichetti , Andrea Pelissetto , Giuseppe D'Adamo , Carlo Pierleoni

We investigate critical phenomena in colloids by means of the renormalization-group based hierarchical reference theory of fluids (HRT). We focus on three experimentally relevant model systems: namely, the Asakura-Oosawa model of a…

Soft Condensed Matter · Physics 2009-11-13 D. Pini , F. Lo Verso , M. Tau , A. Parola , L. Reatto

We investigate effective interactions between a colloidal particle, immersed in a binary mixture of smaller spheres, and a semipermeable membrane. The colloid is modeled as a big hard sphere and the membrane is represented as an infinitely…

Soft Condensed Matter · Physics 2007-05-23 Pawel Bryk

The structural and thermodynamic properties of mixtures of colloidal spheres and non-adsorbing polymer chains are studied within a novel general two-component macromolecular liquid state approach applicable for all size asymmetry ratios.…

Soft Condensed Matter · Physics 2009-11-07 M. Fuchs , K. S. Schweizer

When non-adsorbing polymers are added to an isotropic suspension of rod-like colloids, the colloids effectively attract each other via depletion forces. We performed Monte Carlo simulations to study the phase diagram of such rod-polymer…

Soft Condensed Matter · Physics 2009-11-13 S. Jungblut , R. Tuinier , K. Binder , T. Schilling

The depletion interactions between two colloidal plates or between two colloidal spheres, induced by interacting polymers in a good solvent, are calculated theoretically and by computer simulations. A simple analytical theory is shown to be…

Soft Condensed Matter · Physics 2009-11-07 A. A. Louis , P. G. Bolhuis , E. J. Meijer , J. P. Hansen

We consider a model for a polymer interacting with an attractive wall through a random sequence of charges. We focus on the so-called diluted limit, when the charges are very rare but have strong intensity. In this regime, we determine the…

Probability · Mathematics 2008-07-26 Erwin Bolthausen , Francesco Caravenna , Béatrice de Tilière

In the presence of a non-adsorbing polymer, monodisperse rod-like colloids assemble into one-rod-length thick liquid-like monolayers, called colloidal membranes. The density of the rods within a colloidal membrane is determined by a balance…

We study the phase behavior of mixtures of monodisperse colloidal spheres with a depletion agent which can have arbitrary shape and can possess a polydisperse size or shape distribution. In the low concentration limit, considered here, we…

Soft Condensed Matter · Physics 2009-11-11 C. Grodon , R. Roth

We map dilute or semi-dilute solutions of non-intersecting polymer chains onto a fluid of ``soft'' particles interacting via a concentration dependent effective pair potential, by inverting the pair distribution function of the centers of…

Soft Condensed Matter · Physics 2009-10-31 A. A. Louis , P. G. Bolhuis , J. P. Hansen , E. J. Meijer

We consider a model mixture of hard colloidal spheres and non-adsorbing polymer chains in a theta solvent. The polymer component is modelled as a polydisperse mixture of effective spheres, mutually noninteracting but excluded from the…

Soft Condensed Matter · Physics 2009-11-10 A. R. Denton , M. Schmidt

It has been recently shown that a colloidal monolayer, e.g., formed at a fluid interface or by means of a suitable confining potential, exhibits anomalous collective diffusion. This is a consequence of the hydrodynamic interactions mediated…

Soft Condensed Matter · Physics 2017-04-05 Johannes Bleibel , Alvaro Domínguez , Martin Oettel

Colloid-polymer mixtures may undergo either fluid-fluid phase separation or gelation. This depends on the depth of the quench (polymer concentration) and polymer-colloid size ratio. We present a real-space study of dynamics in phase…

Soft Condensed Matter · Physics 2012-09-19 Isla Zhang , C. Patrick Royall , Paul Bartlett , Malcolm A. Faers

Comprehensive calculations were performed to predict the phase behaviour of large spherical colloids mixed with small spherical colloids that act as depletant. To this end, the free volume theory (FVT) of Lekkerkerker et al. [Europhys.…

Soft Condensed Matter · Physics 2021-01-29 J. Opdam , M. P. M. Schelling , R. Tuinier