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Monte Carlo simulations at constant pressure are performed to study coexistence and interfacial properties of the liquid-solid transition in hard spheres and in colloid-polymer mixtures. The latter system is described as a one-component…

Soft Condensed Matter · Physics 2015-05-18 T. Zykova-Timan , J. Horbach , K. Binder

We study numerically the critical behavior of a modified, active Asakura-Oosawa model for colloid-polymer mixtures. The colloids are modeled as self-propelled particles with Vicsek-like interactions. This system undergoes phase separation…

Soft Condensed Matter · Physics 2017-03-08 Benjamin Trefz , Jonathan Tammo Siebert , Thomas Speck , Kurt Binder , Peter Virnau

We investigate the structure of colloid-polymer mixtures by calculating the structure factors for the Asakura-Oosawa model in the PY approximation. We discuss the role of potential range, polymer concentration and polymer-polymer…

Soft Condensed Matter · Physics 2009-10-31 A. A. Louis , R. Finken , J-P. Hansen

As first explained by the classic Asakura-Oosawa (AO) model, effective attractive forces between colloidal particles induced by depletion of nonadsorbing polymers can drive demixing of colloid-polymer mixtures into colloid-rich and…

Soft Condensed Matter · Physics 2021-08-27 Alan R. Denton , Wyatt J. Davis

The problem of demixing in the Asakura-Oosawa colloid-polymer model is considered. The critical constants are computed using truncated virial expansions up to fifth order. While the exact analytical results for the second and third virial…

We computed the phase-separation behavior and effective interactions of colloid-polymer mixtures in the "protein limit", where the polymer radius of gyration is much larger than the colloid radius. For ideal polymers, the critical colloidal…

Soft Condensed Matter · Physics 2009-11-07 Peter G. Bolhuis , Evert Jan Meijer , Ard A. Louis

We study the stability of mixtures of highly screened repulsive charged spheres and non-adsorbing ideal polymer chains in a common solvent using free volume theory. The effective interaction between charged colloids in an aqueous salt…

Soft Condensed Matter · Physics 2015-06-25 Andrea Fortini , Marjolein Dijkstra , Remco Tuinier

Monte Carlo simulations of the Asakura-Oosawa (AO) model for colloid-polymer mixtures confined between two parallel repulsive structureless walls are presented and analyzed in the light of current theories on capillary condensation and…

Soft Condensed Matter · Physics 2009-11-13 Andres De Virgiliis , Richard L. C. Vink , Jürgen Horbach , Kurt Binder

Interfacial properties of colloid--polymer mixtures are examined within an effective one--component representation, where the polymer degrees of freedom are traced out, leaving a fluid of colloidal particles interacting via polymer--induced…

Soft Condensed Matter · Physics 2007-05-23 A. Moncho-Jorda' , J. Dzubiella , J. P. Hansen , A. A. Louis

We study a system of few colloids confined in a small spherical cavity by event driven molecular dynamics simulations in the canonical ensemble. The colloidal particles interact through a short range square-well potential, which takes into…

Soft Condensed Matter · Physics 2015-04-10 Iván Paganini , Claudio Pastorino , Ignacio Urrutia

The Asakura-Oosawa model for colloid-polymer mixtures is studied by Monte Carlo simulations at densities inside the two-phase coexistence region of fluid and solid. Choosing a geometry where the system is confined between two flat walls,…

Soft Condensed Matter · Physics 2015-06-04 Debabrata Deb , Alexander Winkler , Peter Virnau , Kurt Binder

Understanding the phase behaviour of mixtures continues to pose challenges, even for systems that might be considered "simple". Here we consider a very simple mixture of two colloidal and one non-adsorbing polymer species which can be…

The critical behavior of a model colloid-polymer mixture, the so-called AO model, is studied using computer simulations and finite size scaling techniques. Investigated are the interfacial tension, the order parameter, the susceptibility…

Soft Condensed Matter · Physics 2007-05-23 R. L. C. Vink , J. Horbach , K. Binder

We present a numerical study of the effective potential $V_\mathrm{eff}$ between two hard-sphere colloids dispersed in a solvent of interacting particles, for several values of temperature and solvent density, approaching the solvent…

Soft Condensed Matter · Physics 2013-04-08 Nicoletta Gnan , Emanuela Zaccarelli , Piero Tartaglia , Francesco Sciortino

The surface tension of interacting polymers in a good solvent is calculated theoretically and by computer simulations for a planar wall geometry and for the insertion of a single colloidal hard-sphere. This is achieved for the planar wall…

Soft Condensed Matter · Physics 2016-08-31 A. A. Louis , P. G. Bolhuis , E. J. Meijer , J. P. Hansen

The influence of poor solvent quality on fluid demixing of a model mixture of colloids and nonadsorbing polymers is investigated using density functional theory. The colloidal particles are modelled as hard spheres and the polymer coils as…

Soft Condensed Matter · Physics 2009-11-07 Matthias Schmidt , Alan R. Denton

We present a Monte Carlo method to simulate asymmetric binary mixtures in the grand canonical ensemble. The method is used to study the colloid-polymer model of Asakura and Oosawa. We determine the phase diagram of the fluid-fluid unmixing…

Soft Condensed Matter · Physics 2007-05-23 R. L. C. Vink , J. Horbach

We consider a binary mixture of colloid and polymer particles with positions on a simple cubic lattice. Colloids exclude both colloids and polymers from nearest neighbor sites. Polymers are treated as effective particles that are mutually…

Statistical Mechanics · Physics 2007-07-18 Jose A. Cuesta , Luis Lafuente , Matthias Schmidt

We show that the critical behavior of a colloid-polymer mixture inside a random porous matrix of quenched hard spheres belongs to the universality class of the random-field Ising model. We also demonstrate that random-field effects in…

Soft Condensed Matter · Physics 2007-05-23 R. L. C. Vink , K. Binder , H. Loewen

We develop a theory based on the method of collective variables to study the vapor-liquid equilibrium of asymmetric ionic fluids confined in a disordered porous matrix. The approach allows us to formulate the perturbation theory using an…

Statistical Mechanics · Physics 2018-02-14 O. V. Patsahan , T. M. Patsahan , M. F. Holovko