English
Related papers

Related papers: A proposal to first principles electronic structur…

200 papers

We introduce highly local basis sets for electronic structure which are very efficient for correlation calculations near the complete basis set limit. Our approach is based on gausslets, recently introduced wavelet-like smooth orthogonal…

Chemical Physics · Physics 2019-02-20 Steven R. White , E. Miles Stoudenmire

Existing structural analysis methods may fail to find all hidden constraints for a system of differential-algebraic equations with parameters if the system is structurally unamenable for certain values of the parameters. In this paper, for…

Numerical Analysis · Mathematics 2024-01-11 Wenqiang Yang , Wenyuan Wu , Greg Reid

We present a method for calculating the electronic structure of correlated materials based on a truly first-principles LDA+U scheme. Recently we suggested how to calculate U from first-principles, using a method which we named constrained…

Strongly Correlated Electrons · Physics 2010-06-17 K. Karlsson , F. Aryasetiawan , O. Jepsen

Computing many-body ground state energies and resolving electronic structure calculations are fundamental problems for fields such as quantum chemistry or condensed matter. Several quantum computing algorithms that address these problems…

Quantum Physics · Physics 2023-01-12 Karen J. Morenz Korol , Kenny Choo , Antonio Mezzacapo

We present a method for the calculation of electronic structure of systems that contain tens of thousands of atoms. The method is based on the division of the system into mutually overlapping fragments and the representation of the…

Materials Science · Physics 2011-03-09 Nenad Vukmirović , Lin-Wang Wang

We present fully numerical electronic structure calculations on diatomic molecules exposed to an external magnetic field at the unrestricted Hartree-Fock limit, using a modified version of a recently developed finite element program,…

Chemical Physics · Physics 2020-02-12 Susi Lehtola , Maria Dimitrova , Dage Sundholm

Atomic effective one-electron potentials in a compact analytic form in terms of a few Gaussian charge distributions are developed, for Hydrogen through Nobelium, for starting molecular electronic structure calculations by a simple…

Chemical Physics · Physics 2020-01-07 Dimitri N. Laikov , Ksenia R. Briling

A numerical method using implicit surface representations is proposed to solve the linearized Poisson-Boltzmann equations that arise in mathematical models for the electrostatics of molecules in solvent. The proposed method used an implicit…

Numerical Analysis · Mathematics 2018-04-04 Yimin Zhong , Kui Ren , Richard Tsai

Manipulating expressions in many-body perturbation theory becomes unwieldily with increasing order of the perturbation theory. Here I derive a set of theorems for efficient simplification of such expressions. The derived rules are…

Atomic Physics · Physics 2015-05-14 Andrei Derevianko

A strong link between information geometry and algebraic statistics is made by investigating statistical manifolds which are algebraic varieties. In particular it it shown how first and second order efficient estimators can be constructed,…

Statistics Theory · Mathematics 2014-01-13 Kei Kobayashi , Henry P. Wynn

Ab initio electronic structure calculations of two-dimensional layered structures are typically performed using codes that were developed for three-dimensional structures, which are periodic in all three directions. The introduction of a…

Strongly Correlated Electrons · Physics 2016-06-22 Paolo E. Trevisanutto , Giovanni Vignale

Spectral decomposition of matrices is a recurring and important task in applied mathematics, physics and engineering. Many application problems require the consideration of matrices of size three with spectral decomposition over the real…

Numerical Analysis · Mathematics 2021-11-04 Michal Habera , Andreas Zilian

We give a detailed description of a recently proposed first principles approach to the electronic structure of strongly correlated materials. The method combines the GW approximation with dynamical mean field theory. It is designed to…

Strongly Correlated Electrons · Physics 2007-05-23 Ferdi Aryasetiawan , Silke Biermann , Antoine Georges

In the near future, material and drug design may be aided by quantum computer assisted simulations. These have the potential to target chemical systems intractable by the most powerful classical computers. However, the resources offered by…

In this paper, we construct an efficient numerical scheme for full-potential electronic structure calculations of periodic systems. In this scheme, the computational domain is decomposed into a set of atomic spheres and an interstitial…

Numerical Analysis · Mathematics 2024-12-20 Xiaoxu Li , Huajie Chen

The representation of polynomials by arithmetic circuits evaluating them is an alternative data structure which allowed considerable progress in polynomial equation solving in the last fifteen years. We present a circuit based computation…

Computational Complexity · Computer Science 2012-04-26 Joos Heintz , Bart Kuijpers , Andres Rojas Paredes

We developed a fast numerical methodfor complex symmetric shifted linear systems, which is motivated by the quantum-mechanical (electronic-structure) theory in nanoscale materials. The method is named shifted Conjugate Orthogonal Conjugate…

Numerical Analysis · Mathematics 2007-05-23 T. Sogabe , T. Hoshi , S. -L. Zhang , T. Fujiwara

When neural networks are used to solve differential equations, they usually produce solutions in the form of black-box functions that are not directly mathematically interpretable. We introduce a method for generating symbolic expressions…

Machine Learning · Computer Science 2020-11-05 Maysum Panju , Ali Ghodsi

We present here a review of the fundamental topics of Hartree-Fock theory in Quantum Chemistry. From the molecular Hamiltonian, using and discussing the Born-Oppenheimer approximation, we arrive to the Hartree and Hartree-Fock equations for…

Chemical Physics · Physics 2008-11-25 Pablo Echenique , J. L. Alonso

The computation of electronic structure properties at the quantum level is a crucial aspect of modern physics research. However, conventional methods can be computationally demanding for larger, more complex systems. To address this issue,…

Quantum Physics · Physics 2023-12-05 Nouhaila Innan , Muhammad Al-Zafar Khan , Mohamed Bennai