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We present an extension of the spin-adapted configuration-interaction method for the computation of four electrons in a quasi two-dimensional quantum dot. By a group-theoretical decomposition of the basis set and working with relative and…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 Peter Kramer , Tobias Kramer

An alternative methodology to evaluate two-electron-repulsion integrals based on numerical approximation is proposed. Computational chemistry has branched into two major fields with methodologies based on quantum mechanics and classical…

Chemical Physics · Physics 2016-09-22 Pedro E. M. Lopes

This paper provides details of the massless three-loop three-point integrals calculation at the symmetric point. Our work aimed to extend known two-loop results for such integrals to the three-loop level. Obtained results can find their…

High Energy Physics - Phenomenology · Physics 2021-06-17 Andrey Pikelner

We present a general method for determining screened Coulomb parameters in molecular assemblies, in particular organic molecular crystals. This allows us to calculate the interaction parameters used in a generalized Hubbard model…

Strongly Correlated Electrons · Physics 2015-05-18 Laura Cano-Cortes , Andreas Dolfen , Jaime Merino , Erik Koch

Evaluating multi-center molecular integrals with Cartesian Gaussian-type basis sets has been a long-standing bottleneck in electronic structure theory calculation for solids and molecules. We have developed a vector-coupling and…

Quantum Physics · Physics 2024-05-17 Hang Hu , Gilles Peslherbe , Hsu Kiang Ooi , Anguang Hu

Slater-Condon rules are at the heart of any quantum chemistry method as they allow to simplify $3N$-dimensional integrals as sums of 3- or 6-dimensional integrals. In this paper, we propose an efficient implementation of those rules in…

Computational Physics · Physics 2013-11-26 Anthony Scemama , Emmanuel Giner

By using Poisson's summation formula, we calculate periodic integrals over Gaussian basis functions by partitioning the lattice summations between the real and reciprocal space, where both sums converge exponentially fast with a large…

Strongly Correlated Electrons · Physics 2021-04-06 Sandeep Sharma , Gregory Beylkin

Few-body problems involving Coulomb or gravitational interactions between pairs of particles, whether in classical or quantum physics, are generally handled through a standard multipole expansion of the two-body potentials. We discuss an…

Some typical overlap/potential energy integrals which occur in the use of extended Hylleraas-configuration interaction (E-Hy-CI) functions with Slater-type orbital (STO) basis for two-electron atomic structure calculations, have been…

Atomic Physics · Physics 2019-01-23 B Padhy

We present an efficient approach to evaluate two-center two-electron integrals with exponential functions and with an arbitrary polynomial in electron-nucleus and electron-electron distances. We show that the master integral with the single…

Chemical Physics · Physics 2009-09-29 Krzysztof Pachucki

In this work we propose a novel composite method for accurate calculation of the energies of many-electron atoms. The dominant contribution to the energy (pair energies) are calculated by using explicitly correlated factorisable coupled…

Atomic Physics · Physics 2018-12-12 Michal Przybytek , Michal Lesiuk

The first discussion of basis sets consisting of exponentially decaying Coulomb Sturmian functions for modelling electronic structures is presented. The proposed basis set construction selects Coulomb Sturmian functions using separate upper…

Chemical Physics · Physics 2019-01-23 Michael F. Herbst , James Emil Avery , Andreas Dreuw

Euler angles determining rotations of a system as a whole are conveniently separated in three-particle basis functions. Analytic integration of matrix elements over Euler angles is done in a general form. Results for the Euler angle…

Nuclear Theory · Physics 2009-11-07 V. D. Efros

In this paper, we investigate new integrable extensions of two-center Coulomb systems. We study the most general $n$-dimensional deformation of the two-center problem by adding arbitrary functions supporting second order commuting conserved…

High Energy Physics - Theory · Physics 2023-12-05 Francisco Correa , Octavio Quintana

In this work we make some progress on studying four center integrals for the Coulomb energy for both Hartree Fock (HF) and Density Functional Theory (DFT) calculations for small molecules. We consider basis wave functions of the form of an…

Other Condensed Matter · Physics 2024-04-16 Garry Goldstein

Recently published formulas for the calculation of radial part of overlap integrals (E.Oztekin, M.Yavuz, S.Atalay, Theor.Cmem.Acc., (2001), 106, 264) are critically analyzed. It is demonstrated that the presented in this work formulas are…

Chemical Physics · Physics 2007-05-23 I. I. Guseinov

We study the behaviour of total-energy supercell calculations for dipolar molecules and charged clusters. Using a cutoff Coulomb interaction within the framework of a plane-wave basis set formalism, with all other aspects of the method…

Materials Science · Physics 2009-10-30 M. R. Jarvis , I. D. White , R. W. Godby , M. C. Payne

Calculations of the leading quantum electrodynamics effects in few electron systems involve singular matrix elements of the inter-electronic distances of the form $1/r_i^3$ and $1/r_{ij}^3$. Integrals that result when the nonrelativistic…

Atomic Physics · Physics 2009-11-13 Krzysztof Pachucki , Mariusz Puchalski

The resistance coefficients in screen Coulomb potential of stellar plasma are evaluated in high accuracy. I have analyzed the possible singularities in the integral of scattering angle. There are possible singularities in the case of…

Solar and Stellar Astrophysics · Physics 2017-01-18 Q. S. Zhang

The influence of electron-electron Coulomb repulsion on nonsequential double ionization of rare-gas atoms is investigated. Several variants of the quantum-mechanical transition amplitude are evaluated that differ by the form of the…

Atomic Physics · Physics 2007-05-23 C. Figueira de Morisson Faria , X. Liu , H. Schomerus , W. Becker