Related papers: Attosecond-recollision-controlled selective fragme…
Attosecond pulses can ionize atoms in a coherent process. Since the emerging fragments are entangled, however, each preserves only a fraction of the initial coherence, thus limiting the chance of guiding the ion subsequent evolution. In…
We report on an experimental and theoretical study of the ionization-fragmentation dynamics of argon dimers in intense few-cycle laser pulses with a tagged carrier-envelope phase. We find that a field-driven electron transfer process from…
We describe an apparatus to study the fragmentation of ion-molecule clusters triggered by laser excitation and transfer of an electron from the iodide to the neutral molecule. The apparatus comprises a source to generate ion-molecule…
Attosecond science is based on steering of electrons with the electric field of well-controlled femtosecond laser pulses. It has led to, for example, the generation of XUV light pulses with a duration in the sub-100-attosecond regime, to…
Soft recollisions are laser-driven distant collisions of an electron with its parent ion. Such collisions may cause an energy bunching, since electrons with different initial drift momenta can acquire impacts, which exactly counterbalance…
Tunneling ionization of an atom in ultrashort laser pulses is considered. When the driving laser pulse is switched-on and -off with a steep slope, the photoelectron momentum distribution (PMD) shows an edge-effect because of the…
Coherent manipulation of single-photon wave packets is essentially important for optical quantum communication and quantum information processing. In this paper, we realize controllable splitting and modulation of single-photon-level pulses…
We show that detuned optical pulse trains with a modest spectral width can polarize nuclear spins in InAs quantum dots. The pulse bandwidth is large enough to excite a coherent superposition of both electron spin eigenstates in these…
This paper gives an account of our progress towards performing femtosecond time-resolved photoelectron diffraction on gas-phase molecules in a pump-probe setup combining optical lasers and an X-ray Free-Electron Laser. We present results of…
We experimentally demonstrate optical control of filamentation that occurs during propagation of intense, ultrashort laser pulses through crystals like barium fluoride and sapphire. Control is exercised by rotating the plane of polarization…
In the framework of the time dependent local density approximation, applied to valence electrons, coupled non-adiabatically to molecular dynamics of ions, the irradiations of ethylene by laser and fast charged projectiles are studied. We…
The interaction of high-intensity laser pulses and solid targets provides a promising way to create compact, tunable and bright XUV attosecond sources that can become a unique tool for a variety of applications. However, it is important to…
Increasing ellipticity usually suppresses the recollision probability drastically. In contrast, we report on a recollision channel with large return energy and a substantial probability, regardless of the ellipticity. The laser envelope…
The introduction of femto-chemistry has made it a primary goal to follow the nuclear and electronic evolution of a molecule in time and space as it undergoes a chemical reaction. Using Coulomb Explosion Imaging we have shot the first…
Short pulses from mode-locked lasers can produce background-free atomic fluorescence by allowing temporal separation of the prompt incidental scatter from the subsequent atomic emission. We use this to improve quantum state detection of…
The interaction of ultra-intense laser pulses with an underdense plasma is used in laser-plasma acceleration to create compact sources of ultrashort pulses of relativistic electrons and X-rays. The accelerating structure is a plasma wave,…
We show that electrons recolliding with the ionic core upon tunnel ionization of noble gas atoms driven by a strong circularly polarized laser field in combination with a counter-rotating second harmonic are spin polarized and that their…
An all non-optical method for accurately determining the pulse parameters of individual few-cycle laser shots is presented. By analyzing the "left" and "right" asymmetry of high-energy photoelectrons along the polarization axis using the…
Nonlinear absorption of femtosecond laser pulses provides a unique opportunity to confine energy deposition in any medium to a region that is below the focal diameter of a pulse. Illumination of a polymer film through a transparent high…
We investigate molecular dynamics of multiple ionization in N2 through multiple core-level photoabsorption and subsequent Auger decay processes induced by intense, short X-ray free electron laser pulses. The timing dynamics of the…