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A possible route to extract electronic and nuclear dynamics from molecular targets with attosecond temporal and nanometer spatial resolution is to employ recolliding electrons as `probes'. The recollision process in molecules is, however,…
The basic properties of atoms, molecules and solids are governed by electron dynamics which take place on extremely short time scales. To measure and control these dynamics therefore requires ultrafast sources of radiation combined with…
Temporal correlations in pulsed electron beams reflect the microscopic dynamics of emission and interparticle interaction. In femtosecond electron emission from nanoscale field emitters, Coulomb interactions result in structured…
We investigate the quantum dynamics of fermionic particles interacting with a laser field in a gaseous medium, in the regime of inelastic diffraction scattering on the phase lattice of a slowed travelling wave, below the critical field of…
Manipulating at will the propagation dynamics of high power laser pulses is a long-standing dream whose accomplishment would lead to the control of a plethora of fascinating physical phenomena emerging from laser-matter interaction. The…
Double ionization of diatomic molecules by short linearly polarized laser pulses is analyzed. We consider the final stage of the ionization process, that is the decay of a highly excited two electron molecule, which is formed after…
Exposing a molecule to intense light pulses may bring this molecule to a nonstationary quantum state, thus launching correlated dynamics of electronic and nuclear subsystems. Although much had been achieved in the understanding of…
We studied the photoelectron spectra generated by an intense few-cycle infrared laser pulse. By focusing on the angular distributions of the back rescattered high energy photoelectrons, we show that accurate differential elastic scattering…
Attosecond science has demonstrated that electrons can be controlled on the sub-cycle time scale of an optical wave, paving the way toward optical frequency electronics. Using controlled few-cycle optical waveforms, the study of sub-cycle…
Shaping electron beams with the cycles of light provides femtosecond and attosecond time resolution in electron microscopy and enables fundamental quantum-coherent measurements. However, efficient light-electron control requires a prolonged…
We introduce and experimentally demonstrate a method, where the two intrinsic time scales of a molecule, the slow nuclear motion and the fast electronic motion, are simultaneously measured in a photo-electron photo-ion coincidence…
In molecular systems, the ultrafast motion of electrons initiates the process of chemical change. Tracking this electronic motion across molecules requires coupling attosecond time resolution to atomic-scale spatial sensitivity. In this…
We investigate the attosecond response of the electronic cloud of a molecular system to an outer-valence ionization. The time needed for the remaining electrons to respond to a sudden perturbation in the electronic structure of the molecule…
Ultrashort XUV pulses of the Free-Electron-LASer in Hamburg (FLASH) were used to investigate laser-induced fragmentation patterns of the prototypical chiral molecule 1-iodo-2-methyl-butane (C$_5$H$_{11}$I) in a pump-probe scheme. Ion…
We theoretically demonstrate the possibility to tune the temporal waveform of optical unipolar pulses upon their coherent interaction with a multi-level resonant medium. This is achieved through the coherent control of the response of a…
Globally optimal solution describing a phase conjugated field of Raman scattering on the resonant $B\gets X$ transition of iodine $I_2$ is studied. Maximum optical coherence is found as a top eigenvalue problem. A reversibility theorem has…
High harmonic light sources make it possible to access attosecond time-scales, thus opening up the prospect of manipulating electronic wave packets for steering molecular dynamics. However, two decades after the birth of attosecond physics,…
We propose utilizing a polarization-tailored high-power laser pulse to extract and accelerate electrons from the edge of a solid foil target to produce isolated attosecond electron bunches. The laser pulse consists of two…
Recent technological advances allowed the coherent optical manipulation of high-energy electron wavepackets with attosecond precision. Here we theoretically investigate the collision of optically-modulated pulsed electron beams with atomic…
In molecular photofragmentation processes by soft X-rays, a number of ionic fragments can be produced, each having a different abundance and correlation with the emitted electron kinetic energy. For investigating these fragmentation…