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Semiconductor nanoplatelets possess exceptional optical properties that make them promising candidates for next-generation optoelectronic applications. However, unlike quantum dots where absorption spectroscopy alone can determine both size…

We investigate the time-resolved photocurrent response of CdSe quantum dot (QD) thin films sensitized with zinc beta-tetraaminophthalocyanine (Zn4APc) on three different substrates, namely silicon with 230 nm SiO2 dielectric, glass as well…

Mesoscale and Nanoscale Physics · Physics 2021-09-07 Christine Schedel , Fabian Strauß , Krishan Kumar , Andre Maier , Kai M. Wurst , Patrick Michel , Marcus Scheele

Colloidal quantum dots (cQDs) recently emerged as building blocks for semiconductor materials with tuneable properties. Electro-hydrodynamic printing can be used to obtain sub-micrometre patterns of cQDs without elaborate and aggressive…

Cu(In,Ga)Se2 (CIGSe)-based solar cells are promising candidates for efficient sunlight harvesting. However, their complex composition and microstructure can change under operation conditions, for instance heating from sun light illumination…

Quantum dot (QD) assemblies are nanostructured networks made from aggregates of QDs and feature improved charge and energy transfer efficiencies compared to discrete QDs. Using first-principles many-body perturbation theory, we…

Materials Science · Physics 2022-10-25 Sandip Aryal , Joseph Frimpong , Zhen-Fei Liu

We report thin-film InAs/GaAs quantum dot (QD) solar cells with $n-i-p{+}$ deep junction structure and planar back reflector fabricated by epitaxial lift-off (ELO) of full 3-inch wafers. External quantum efficiency measurements demonstrate…

Applied Physics · Physics 2018-05-28 F Cappelluti , D Kim , M van Eerden , AP Cédola , T Aho , G Bissels , F Elsehrawy , J Wu , H Liu , P Mulder , G Bauhuis , J Schermer , T Niemi , M Guina

Understanding, optimizing, and controlling the optical absorption process, exciton gemination, and electron-hole separation and conduction in low dimensional systems is a fundamental problem in materials science. However, robust and…

Mesoscale and Nanoscale Physics · Physics 2020-08-26 Keenan Lyon , María Rosa Preciado-Rivas , Duncan John Mowbray , Vito Despoja

The present work deals with the comparison of sizes, optical and electronic properties of COOH functionalized CdTe quantum dots (QDs) in freezed solid polymeric (polyvinyl alcohol (PVA) matrix and in solution phase (water). PVA has been…

Materials Science · Physics 2020-11-10 Pooja , Papia Chowdhury

Thin films of colloidal semiconductor CdSe quantum-dots (QDs) and a styrene/maleic anhydride copolymer were prepared by the Langmuir-Blodgett technique and their photoluminescence was characterized by confocal fluorescence lifetime…

Metal oxide nanostructures are widely used in energy applications like super capacitors and Li-on battery. Smaller size nanocrystals show better stability, low ion diffusion time, higher-ion flux and low pulverization than bigger size…

Materials Science · Physics 2016-05-12 V. Bonu , B. Gupta , S. Chandra , A Das , S. Dhara , A. K. Tyagi

The first principles density functional theory (DFT) calculations have been used to investigate the atomic and electronic properties of thiadiazole adsorption on the Si(001) surface. A (2x2) reconstructed clean substrate surface has been…

Materials Science · Physics 2018-05-07 Cagil Kaderoglu

The theoretical formalism of the local density approximation (LDA) to density functional theory (DFT) has been used to study the electronic and geometric structures of SimCn (1<=m, n<=4;n<=m) clusters. An all electron 6-311++G** basis set…

Atomic and Molecular Clusters · Physics 2007-05-23 Prachi Pradhan , Asok K. Ray

We present a systematic study of the photo-absorption spectra of various Si$_{n}$H$_{m}$ clusters (n=1-10, m=1-14) using the time-dependent density functional theory (TDDFT). The method uses a real-time, real-space implementation of TDDFT…

Mesoscale and Nanoscale Physics · Physics 2012-02-29 Juzar Thingna , R. Prasad , S. Auluck

Time Dependent Density Functional Theory (TDDFT) calculations have been used to understand the excited state properties of "modified-chlorophyll" f ('Chlide' f), Chlide a, Chlide b and axial ligated (with Imidazole, H2O, CH3OH, CH3COOH,…

Materials Science · Physics 2013-06-24 S R K Chaitanya Sharma Y , Ganga Periyasamy , Swapan K Pati

Zinc-blende CdSe semiconducting nanoplatelets (NPL) show outstanding quantum confinement properties thanks to their small, atomically-controlled, thickness. For example, they display extremely sharp absorption peaks that make them very…

Applied Physics · Physics 2019-12-09 Ivan Dozov , Claire Goldmann , Patrick Davidson , Benjamin Abécassis

This work presents epitaxial growth and optical spectroscopy of CdTe quantum dots (QDs) in (Cd,Zn,Mg)Te barriers placed on the top of (Cd,Zn,Mg)Te distributed Bragg reflector. The formed photonic mode in our half-cavity structure permits to…

Mesoscale and Nanoscale Physics · Physics 2017-03-24 W. Pacuski , J. -G. Rousset , V. Delmonte , T. Jakubczyk , K. Sobczak , J. Borysiuk , K. Sawicki , E. Janik , J. Kasprzak

We investigate the influence of X-ray and gamma-ray irradiation on the photophysical properties of sub-monolayer CdTe/CdS quantum dots (QDs) immobilized in porous silica (PSiO2) scaffolds. The highly luminescent QD-PSiO2 thin films allow…

Mesoscale and Nanoscale Physics · Physics 2015-08-25 Girija Gaur , Dmitry S. Koktysh , Daniel M. Fleetwood , Robert A. Weller , Robert A. Reed , Bridget R. Rogers , Sharon M. Weiss

We report on the fabrication and characterization of superconducting coplanar waveguide (CPW) resonators based on titanium nitride (TiN) thin films deposited on 200\,mm diameter high-resistivity Si(100) substrates. We systematically…

Semiconducting, core-shell nanocrystals (NCs) are promising building blocks for the construction of higher dimensional artificial nanostructures using oriented attachment. However, the assembly and epitaxial attachment steps critical to…

A spherical quantum dot (QD) heterosystem CdS/SiO$_2$ has been studied. Each QD has a hydrogen-like impurity in its center. Besides that, it has been accounted that a polarization trap for electron exists at the interfaces due to the…

Mesoscale and Nanoscale Physics · Physics 2017-12-15 V. I. Boichuk , R. Ya. Leshko , D. S. Karpyn