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MgV$_{2}$O$_{4}$ is a spinel based on magnetic V$^{3+}$ ions which host both spin ($S=1$) and orbital ($l_{eff}=1$) moments. Owing to the underlying pyrochlore coordination of the magnetic sites, the spins in MgV$_{2}$O$_{4}$ only…

The ferrimagnetic spinel $\mathrm{CoV_2O_4}$ has been a topic of intense recent interest, both as a frustrated insulator with unquenched orbital degeneracy and as a near-itinerant magnet which can be driven metallic with moderate applied…

Strongly Correlated Electrons · Physics 2016-02-03 D. Reig-i-Plessis , D. Casavant , V. O. Garlea , A. A. Aczel , M. Feygenson , J. Neuefeind , H. D. Zhou , S. E. Nagler , G. J. MacDougall

With electron filling $n=1$ in the $\rm Sr_2VO_4$ compound, the octahedrally coordinated $t_{\rm 2g}$ orbitals are strongly active due to tetragonal distortion induced crystal field tuning by external agent such as pressure. Considering the…

Strongly Correlated Electrons · Physics 2022-02-25 Shubhajyoti Mohapatra , Dheeraj Kumar Singh , Rajyavardhan Ray , Sayandip Ghosh , Avinash Singh

Motivated by recent experiments, we present a comprehensive theoretical study of the geometrically frustrated strongly correlated magnetic insulator Mn$_3$O$_4$ spinel oxide based on a microscopic Hamiltonian involving lattice, spin and…

Strongly Correlated Electrons · Physics 2017-08-23 Santanu Pal , Siddhartha Lal

Neutron inelastic scattering and diffraction techniques have been used to study the MnV2O4 spinel system. Our measurements show the existence of two transitions to long-range ordered ferrimagnetic states; the first collinear and the second…

Strongly Correlated Electrons · Physics 2009-11-13 V. O. Garlea , R. Jin , D. Mandrus , B. Roessli , Q. Huang , M. Miller , A. J. Schultz , S. E. Nagler

Two magnetic ordering transitions are found in InMnO3, the paramagnetic to antiferromagnetic transition near ~118 K and a lower possible spin rotation transition near ~42 K. Multiple length scale structural measurements reveal enhanced…

Materials Science · Physics 2015-06-22 T. Yu , T. A. Tyson , P. Gao , T. Wu , X. Hong , S. Ghose , Y. -S. Chen

We present a neutron diffraction study of FeV2O4, which is rare in exhibiting spin and orbital degrees of freedom on both cation sublattices of the spinel structure. Our data confirm the existence of three structural phase transitions…

Strongly Correlated Electrons · Physics 2012-09-03 G. J. MacDougall , V. O. Garlea , A. A. Aczel , H. D. Zhou , S. E. Nagler

High-entropy spinel oxides provide an excellent platform for investigating entropy-stabilized correlated systems with strong configurational disorder. In this work, we systematically study the temperature evolution of the structural and…

We present neutron scattering measurements on powder samples of the spinel FeSc2S4 that reveal a previously unobserved magnetic ordering transition occurring at 11.8(2)~K. Magnetic ordering occurs subsequent to a subtle cubic-to-tetragonal…

Strongly Correlated Electrons · Physics 2016-12-21 K. W. Plumb , Jennifer Morey , J. A. Rodriguez-Rivera , Hui Wu , A. A. Podlesnyak , T. M. McQueen , C. L. Broholm

In frustrated spinel antiferromagnets, dilution with non-magnetic ions can be a powerful strategy for probing unconventional spin states or uncovering interesting phenomena. Here, we present X-ray, neutron scattering and thermodynamic…

Strongly Correlated Electrons · Physics 2018-06-20 A. V. Zakrzewski , S. Gangopadhyay , A. A. Aczel , S. Calder , T. J. Williams , G. J. MacDougall

The recent discovery of Spin-ice is a spectacular example of non-coplanar spin arrangements that can arise in the pyrochlore A2B2O7 structure. We present magnetic and thermodynamic studies on the metallic-ferromagnet pyrochlore Sm2Mo2O7.…

Strongly Correlated Electrons · Physics 2009-11-13 Surjeet Singh , R. Suryanarayanan , R. Tackett , G. Lawes , A. K. Sood , P. Berthet , A. Revcolevschi

We investigate the evolution of spin and orbital order in undoped LaMnO$_3$ under increasing temperature with a model including both superexchange and Jahn-Teller interactions. We used several cluster mean field calculation schemes and find…

Strongly Correlated Electrons · Physics 2016-12-26 Mateusz Snamina , Andrzej M. Oleś

Crystal and magnetic structures of the high-pressure stabilized perovskite phase of TlMnO3 have been studied by neutron powder diffraction. The crystal structure involves two types of primary structural distortions: a+b-b-octahedral tilting…

Strongly Correlated Electrons · Physics 2019-03-07 Dmitry D. Khalyavin , Pascal Manuel , Wei Yi , Alexei A. Belik

In spinel-type nickelate NiRh$_2$O$_4$, magnetic ordering is observed upon the sample synthesized via kinetically controlled low-temperature solid-state metathesis, as opposed to previously-reported samples obtained through conventional…

Strongly Correlated Electrons · Physics 2023-10-24 Yuya Haraguchi , Daisuke Nishio-Hamane , Hiroko Aruga Katori

We determined the magnetic structure of CuCr$_2$O$_4$ using neutron diffraction and irreducible representation analysis. The measurements identified a new phase between 155 K and 125 K as nearly collinear magnetic ordering in the Cr…

Strongly Correlated Electrons · Physics 2018-03-20 K. Tomiyasu , S. Lee , H. Ishibashi , Y. Takahashi , T. Kawamata , Y. Koike , T. Nojima , S. Torii , T. Kamiyama

Spin density waves, based on modulated local moments, are usually associated with metallic materials, but have recently been reported in insulators which display coupled magnetic and structural order parameters. We discuss one such example,…

Materials Science · Physics 2020-07-30 N. Giles-Donovan , N. Qureshi , R. D. Johnson , L. Y. Zhang , S. -W. Cheong , S. Cochran , C. Stock

We analyze electronic, magnetic, and structural properties of the spinel compound MgTi$_2$O$_4$ using the local density approximation+U method. We show how MgTi$_2$O$_4$ undergoes to a canted orbital-spin ordered state, where charge, spin…

Other Condensed Matter · Physics 2009-11-13 S. Leoni , A. N. Yaresko , N. Perkins , H. Rosner , L. Craco

The cubic spinel FeCr2S4 has been receiving immense research interest because of its emergent phases and the interplay of spin, orbital and lattice degrees of freedom. Despite the intense research, several fundamental questions are yet to…

The high-pressure synthesized quasi-one-dimensional compounds NaMn$_2$O$_4$ and Li$_{0.92}$Mn$_2$O$_4$ are both antiferromagnetic insulators, and here their atomic and magnetic structures were investigated using neutron powder diffraction.…

Crystal structure, magnetic susceptibility, and specific heat were measured in the normal cubic spinel compounds MnSc_2S_4 and FeSc_2S_4. Down to the lowest temperatures, both compounds remain cubic and reveal strong magnetic frustration.…

Strongly Correlated Electrons · Physics 2009-11-10 V. Fritsch , J. Hemberger , N. Buettgen , E. W. Scheidt , H. A. Krug von Nidda , A. Loidl , V. Tsurkan