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We describe a powerful and intuitive technique for modeling light-matter interactions in classical and quantum nanoplasmonics. Our approach uses a quasinormal mode expansion of the Green function within a metal nanoresonator of arbitrary…

Quantum Physics · Physics 2015-06-18 Rong-Chun Ge , Philip Trost Kristensen , Jeff. F. Young , Stephen Hughes

Second-order nonlinear optical processes do not manifest in the bulk of centrosymmetric materials, but may occur in the angstroms-thick layer at surfaces. At such length-scales, quantum mechanical effects come into play which could be…

Optics · Physics 2021-05-11 Muhammad Khalid , Cristian Ciracì

We investigate the effect of a cavity on nonlinear two-photon transitions of a molecular system and how such an effect depends on the cavity quality factor, the field enhancement and the possibility of dephasing. We find that the molecular…

Quantum Physics · Physics 2023-10-16 Zeyu Zhou , Hsing-Ta Chen , Maxim Sukharev , Joseph E. Subotnik , Abraham Nitzan

A mechanism for additional enhancement of SERS in the nanoparticle-on-mirror scheme is proposed. This new mechanism is based on the use of a substrate made of material with a near-minus-one permittivity. The setup involves a plasmonic…

Optics · Physics 2026-05-11 Alexey P. Vinogradov , Evgeny S. Andrianov

Silicon T centers present the promising possibility to generate optically active spin qubits in an all-silicon device. However, these color centers exhibit long excited state lifetimes and a low Debye-Waller factor, making them dim emitters…

We have studied theoretically the Purcell factor which characterizes a change in the emission rate of an electric or magnetic dipole embedded in the center of a spherical cavity. The main attention is paid to the analysis of cavities with…

Mesoscale and Nanoscale Physics · Physics 2011-04-01 M. M. Glazov , E. L. Ivchenko , A. N. Poddubny , G. Khitrova

We study theoretically the enhancement of spontaneous emission in wire metamaterials. We analyze the dependence of the Purcell factor dependence on wire dielectric constant for both electric and magnetic dipole sources, and find an optimal…

Optics · Physics 2013-05-30 Alexander N. Poddubny , Pavel A. Belov , Yuri S. Kivshar

We consider the theory of spontaneous emission for a random medium of stationary two-level atoms. We investigate the dynamics of the field and atomic probability amplitudes for a one-photon state of the system. At long times and large…

Optics · Physics 2021-04-27 Joseph Kraisler , John C Schotland

Subwavelength aperture arrays in thin metal films can enable enhanced transmission of light and matter (atom) waves. The phenomenon relies on resonant excitation and interference of the plasmon or matter waves on the metal surface. We show…

Optics · Physics 2009-11-13 S. V. Kukhlevsky

The Purcell factor and the spontaneous emission spectrum of a quantum emitter (QE) placed close to the edge of a graphene half-space nanostructure is investigated, using semi-analytical methods at the electrostatic regime. The half-space…

Optics · Physics 2019-12-11 Vasilios Karanikolas , Pelin Tozman , Emmanuel Paspalakis

Hybrid quantum photonics combines classical photonics with quantum emitters in a postprocessing step. It facilitates to link ideal quantum light sources to optimized photonic platforms. Optical cavities enable to harness the Purcell-effect…

Near-field enhancement and sub-wavelength imaging properties of a system comprising a coupled pair of two-dimensional arrays of resonant nanospheres are studied. The concept of using two coupled material sheets possessing surface mode…

Optics · Physics 2009-11-13 Pekka Alitalo , Constantin Simovski , Ari Viitanen , Sergei Tretyakov

Surface waves in a thin uniform metal film are described in terms of quantum electrodynamics.The interaction of surface waves with a quantum oscillator is discussed in the dipole approximation. The increase in the spontaneous emission rate…

Optics · Physics 2009-12-03 V. V. Lidsky

Controlling quantum light-matter interactions at scales smaller than the diffraction limit at the single quantum emitter level is a critical challenge to the goal of advancing quantum technologies. We introduce a novel material platform…

We report on two orders of magnitude reduction in the fluorescence lifetime when a single molecule placed in a thin film is surrounded by two gold nanospheres across the film interface. By attaching one of the gold particles to the end of a…

Optics · Physics 2015-06-11 K. -G. Lee , H. Eghlidi , X-W. Chen , A. Renn , S. Götzinger , V. Sandoghdar

The effect of spatial correlations on the Purcell effect in a bidimensional dispersion of resonant nanoparticles is analyzed. We perform extensive calculations on the fluorescence decay rate of a point emitter embedded in a system of…

In recent years there has been great interest towards optical cavities as a tool to manipulate the properties and phases of embedded quantum materials. Due to the Purcell effect, a cavity changes the photon phase space and thus the rate of…

Optics · Physics 2024-10-25 Giuliano Chiriacò

The importance of considering near-field effects on photon recycling and spontaneous emission in a thermophotovoltaic device is investigated. Fluctuational electrodynamics is used to calculate external luminescence from a photovoltaic cell…

Optics · Physics 2017-08-02 John DeSutter , Rodolphe Vaillon , Mathieu Francoeur

Resonance fluorescence of natural or artificial atoms constitutes a prime method for generating non-classical light. While most efforts have focused on producing single-photons, multi-photon emission is unavoidably present in the resonant…

Quantum emitters, such as q-dots and dye molecules, in the immediate vicinity of plasmonic nanostructures, resonantly excite surface plasmon-polaritons (SPPs) under incoherent pump. The efficiency in the excitation of SPPs increases as the…

Quantum Physics · Physics 2017-06-28 Igor Protsenko , Shunping Zhang , Alexander Uskov , Xuewen Chen , Hongxing Xu