Related papers: Extraction of the homogeneous linewidth of a fast …
Spectral diffusion is a result of random spectral jumps of a narrow line as a result of a fluctuating environment. It is an important issue in spectroscopy, because the observed spectral broadening prevents access to the intrinsic line…
We investigate the possibility of measuring the homogeneous and inhomogeneous contribution to the linewidth of a spectrally diffusing single photon emitter using a simple photon correlation spectroscopy method (PCS). The photon energy…
The homogeneous photoluminescence spectral linewidth in semiconductors carries a wealth of information on the coupling of primary photoexcitations with their dynamic environment as well as between multi-particles. In the limit in which…
We have observed strong photoluminescence from a single CdSe quantum dot embedded in a ZnSe nanowire. Exciton, biexciton and charged exciton lines have been identified unambiguously using photon correlation spectroscopy. This technique has…
We show that the single emitter linewidth underlying a broadened ensemble emission spectrum can be extracted from correlations among the stochastic intensity fluctuations in the ensemble spectrum. Spectral correlations can be observed at…
The observation of quantum dot resonance fluorescence enabled a new solid-state approach to generating single photons with a bandwidth almost as narrow as the natural linewidth of a quantum dot transition. Here, we operate in the Heitler…
Diffusing-Wave Spectroscopy (DWS) treats the transport of photons through turbid samples as a diffusion process, thereby making it possible to extract the dynamics of scatterers from measured correlation functions. The analysis of DWS data…
The ability to identify and characterize homogeneous and inhomogeneous dephasing processes is crucial in solid-state quantum optics. In particular, spectral diffusion leading to line broadening is difficult to evidence when the associated…
The near- and far-field photoluminescence spectra of a gated two-dimensional electron gas have been measured. Spatial fluctuations in the electron density are found to be manifested as spatial fluctuations in the emission amplitude of the…
We formulate and demonstrate experimentally the high-resolution spectral method based on Bloch-wave symmetry properties for extracting mode dispersion in periodic waveguides from measurements of near-field profiles. We characterize both the…
The paper considers the process of Thomson scattering of coherent diffraction radiation (CDR) produced by the preceding bunch of the accelerator on one of the following bunches. It is shown that the yield of scattered hard photons is…
A robust process for fabricating intrinsic single-photon emitters in silicon nitride has been recently established. These emitters show promise for quantum applications due to room-temperature operation and monolithic integration with the…
We measure the homogeneous excitation linewidth of regioregular poly(3-hexylthiophene), a model semicrystalline polymeric semiconductor, by means of two-dimensional coherent photoluminescence excitation spectroscopy. At a temperature of…
We perform photoluminescence excitation measurements on individual CdSe/ZnS nanocrystal quantum dots (NCQDs) at room temperature to study optical transition energies and broadening. The observed features in the spectra are identified and…
"Spin noise spectroscopy" (SNS) is a powerful optical technique for probing electron and hole spin dynamics that is based on detecting their intrinsic and random fluctuations while in thermal equilibrium, an approach guaranteed by the…
Two-dimensional coherent spectroscopy (2DCS) provides simultaneous measurement of homogeneous and inhomogeneous linewidths through quantitative lineshape analysis. However, conventional lineshape analysis methods assume Gaussian…
Exciton-phonon coupling limits the homogeneous emission linewidth of nanocrystals. Hence, a full understanding of it is crucial. In this work, we statistically investigate exciton-phonon coupling by performing single-particle spectroscopy…
A robust and streamlined method is presented for efficiently extracting spectral diffusion from two-dimensional coherent spectra by employing the projection-slice theorem. The method is based on the optical Bloch equations for a single…
In the solid state, a large variety of single-photon emitters present high quality photophysical properties together with a potential for integration. However, in many cases, the host matrix induces fluctuations of the emission wavelength…
Single-shot ultrafast spectroscopy based on the frequency encoding of transient absorbance kinetics (FDSS) is demonstrated. These kinetics are sampled spectrally using linearly chirped pulses derived from a Ti:sapphire laser. A variable…