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Related papers: Infrared phonon activity in pristine graphite

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We observe a giant increase of the infrared intensity and a softening of the in-plane antisymmetric phonon mode Eu (~0.2 eV) in bilayer graphene as a function of the gate-induced doping. The phonon peak has a pronounced Fano-like asymmetry.…

Strongly Correlated Electrons · Physics 2015-05-13 A. B. Kuzmenko , L. Benfatto , E. Cappelluti , I. Crassee , D. van der Marel , P. Blake , K. S. Novoselov , A. K. Geim

We report the observation of an intense anomalous peak at 1608 cm$^{-1}$ in the Raman spectrum of graphene associated to the presence of chromium nanoparticles in contact with graphene. Bombardment with an electron beam demonstrates that…

Since their discovery, graphene-based systems represent an exceptional playground to explore the emergence of peculiar quantum effects. The present paper focuses on the anomalous appearence of strong infrared phonon resonances in the…

Mesoscale and Nanoscale Physics · Physics 2012-10-04 E. Cappelluti , L. Benfatto , M. Manzardo , A. B. Kuzmenko

The in-plane optical phonons around 200 meV in few-layer graphene are investigated utilizing infrared absorption spectroscopy. The phonon spectra exhibit unusual asymmetric features characteristic of Fano resonances, which depend critically…

Mesoscale and Nanoscale Physics · Physics 2015-05-30 Zhiqiang Li , Chun Hung Lui , Emmanuele Cappelluti , Lara Benfatto , Kin Fai Mak , G. Larry Carr , Jie Shan , Tony F. Heinz

We develop an ab initio method to simulate the infrared vibrational response of metallic systems in the framework of time-dependent density functional perturbation theory. By introducing a generalized frequency-dependent Born effective…

Materials Science · Physics 2021-04-21 Luca Binci , Paolo Barone , Francesco Mauri

We obtained the spectral function of very high quality natural graphite single crystals using angle resolved photoelectron spectroscopy (ARPES). A clear separation of non-bonding and bonding bands and asymmetric lineshape are observed. The…

Strongly Correlated Electrons · Physics 2009-11-13 C. S. Leem , B. J. Kim , Chul Kim , S. R. Park , T. Ohta , A. Bostwick , E. Rotenberg , H. -D. Kim , M. K. Kim , H. J. Choi , C. Kim

We report the complex dielectric function of high-quality Na_3Ir_3O_8 single crystals determined by spectroscopic ellipsometry in the spectral range from 15 meV to 2 eV. The far-infrared phonon spectra exhibit highly asymmetric line shapes…

Strongly Correlated Electrons · Physics 2014-02-28 D. Pröpper , A. N. Yaresko , T. I. Larkin , T. N. Stanislavchuk , A. A. Sirenko , T. Takayama , A. Matsumoto , H. Takagi , B. Keimer , A. V. Boris

Excitation of electron-hole pairs in the vicinity of the Dirac cone by the Coulomb interaction gives rise to an asymmetric Breit-Wigner-Fano lineshape in the phonon Raman spectra in graphene. This asymmetric lineshape appears due to the…

Mesoscale and Nanoscale Physics · Physics 2015-06-22 Eddwi H. Hasdeo , Ahmad R. T. Nugraha , Mildred S. Dresselhaus , Riichiro Saito

We investigate the role of electron-hole correlations in the absorption of freestanding monolayer and bilayer graphene using optical transmission spectroscopy from 1.5 to 5.5 eV. Line shape analysis demonstrates that the ultraviolet region…

Mesoscale and Nanoscale Physics · Physics 2015-05-20 Dong-Hun Chae , Tobias Utikal , Siegfried Weisenburger , Harald Giessen , Klaus. v. Klitzing , Markus Lippitz , Jurgen H. Smet

A Fano-like phonon resonance is observed in few-layer (~3) graphene at room temperature using infrared Fourier transform spectroscopy. This Fano resonance is the manifestation of a strong electron-phonon interaction between the discrete…

Mesoscale and Nanoscale Physics · Physics 2013-05-29 Zhihong Liu , Xiaoxiang Lu , Peng Peng , Wei Wu , Steven Pei , Qingkai Yu , Jiming Bao

The detailed temperature dependence of the infrared-active mode in Fe$_{1.03}$Te ($T_N\simeq 68$ K) and Fe$_{1.13}$Te ($T_N\simeq 56$ K) has been examined, and the position, width, strength, and asymmetry parameter determined using an…

Strongly Correlated Electrons · Physics 2016-05-18 C. C. Homes , Y. M. Dai , J. Schneeloch , R. D. Zhong , G. D. Gu

We study the infrared conductivity of graphene at finite chemical potential and temperature taking into account the effect of phonons and disorder due to charged impurities and unitary scatterers. The screening of the long-range Coulomb…

Mesoscale and Nanoscale Physics · Physics 2008-10-16 N. M. R. Peres , T. Stauber , A. H. Castro Neto

We determine from first-principles the finite-temperature properties--linewidths, line shifts, and lifetimes--of the key vibrational modes that dominate inelastic losses in graphitic materials. In graphite, the phonon linewidth of the…

Materials Science · Physics 2007-10-25 Nicola Bonini , Michele Lazzeri , Nicola Marzari , Francesco Mauri

The linewidths of the electronic bands originating from the electron-phonon coupling in graphene are analyzed based on model tight-binding calculations and experimental angle-resolved photoemission spectroscopy (ARPES) data. Our…

Materials Science · Physics 2018-12-05 B. Hellsing , T. Frederiksen , F. Mazzola , T. Balasubramanian , J. Wells

Significant excitonic effects were observed in graphene by measuring its optical conductivity in a broad spectral range including the two-dimensional {\pi}-band saddle-point singularities in the electronic structure. The strong…

Materials Science · Physics 2015-05-20 Kin Fai Mak , Jie Shan , Tony F. Heinz

Radio-frequency compressed ultrafast electron diffraction has been used to probe the coherent and incoherent coupling of impulsive electronic excitation at 1.55 eV (800 nm) to optical and acoustic phonon modes directly from the perspective…

Materials Science · Physics 2015-06-23 Robert P. Chatelain , Vance R. Morrison , Bart L. M. Klarenaar , Bradley J. Siwick

The Raman peak position and linewidth provide insight into phonon anharmonicity and electron-phonon interactions (EPI) in materials. For monolayer graphene, prior first-principles calculations have yielded decreasing linewidth with…

Materials Science · Physics 2022-01-27 Zherui Han , Xiaolong Yang , Sean E. Sullivan , Tianli Feng , Li Shi , Wu Li , Xiulin Ruan

We perform a comparative experimental and theoretical study of the temperature dependence up to 700 K of the frequency and linewidths of the graphite E1u and E2g optical phonons (~1590 and 1580 cm-1) by infra-red (IR) and Raman…

Materials Science · Physics 2012-09-21 P. Giura , N. Bonini , G. Creff , J. B. Brubach , P. Roy , M. Lazzeri

We have investigated shot noise in graphene field effect devices in the temperature range of 4.2--30 K at low frequency ($f$ = 600--850 MHz). We find that for our graphene samples with large width over length ratio $W/L$, the Fano factor…

Mesoscale and Nanoscale Physics · Physics 2008-07-01 R. Danneau , F. Wu , M. F. Craciun , S. Russo , M. Y. Tomi , J. Salmilehto , A. F. Morpurgo , P. J. Hakonen

Recent infrared measurements of phonon peaks in gated bilayer graphene reveal two striking signatures of electron-phonon interaction: an asymmetric Fano lineshape and a giant variation of the peak intensity as a function of the applied gate…

Strongly Correlated Electrons · Physics 2010-07-26 E. Cappelluti , L. Benfatto , A. B. Kuzmenko
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