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Recently we reported a series of numerical simulations proving that it is possible in principle to create an electronic wave packet and subsequent electronic motion in a neutral molecule photoexcited by a UV pump pulse within a few…
We discuss harmonic generation in the case of laser field-dressed Hamiltonians that are invariant under so-called dynamical symmetry operations. Examples for such systems are molecules which exhibit a discrete rotational symmetry of order N…
The Quantitative Rescattering Theory (QRS) for high-order harmonic generation (HHG) by intense laser pulses is presented. According to the QRS, HHG spectra can be expressed as a product of a returning electron wave packet and the…
We investigate a two-level atom in the field of a strong laser pulse. The resulting time-dependent polarization is the source of a radiation the frequency components of which are essentially harmonics of the driving field's carrier…
The coherent radiation spectrum of two-level polar molecules with UV transition is studied at the multiphoton resonant excitation by a moderately strong laser field. The spectrum corresponding to harmonic generation and low-frequency…
We study numerically the Bloch electron wavepacket dynamics in periodic potentials to simulate laser-solid interactions. We introduce a new perspective in the coordinate space combined with the motion of the Bloch electron wavepackets…
We present an experimental technique using orbital angular momentum (OAM) in a fundamental laser field to drive High Harmonic Generation (HHG). The mixing of beams with different OAM allows to generate two laser foci tightly spaced to study…
We investigated the high-order harmonic generation by interacting time-delayed, linearly polarized bi-chromatic laser pulses with the atomic target. The frequency ratio of secondary to primary fields ($\omega_2/\omega_1$), along with the…
New approach to study the spontaneous emission of the atomic system in the presence of the high-intensity laser field is used to study the process of harmonic generation. The analysis is based on the consideration of quantum system…
Generation of circularly-polarized high-harmonics with the same helicity to all orders is indispensable for chiral-sensitive spectroscopy with attosecond temporal resolution. Solid-state samples have added a valuable asset in controlling…
We report on the first simultaneous measurement of high-order harmonics, relativistic electrons and low divergence proton beams generated from plasma mirrors driven at kHz repetition rate by relativistic-intensity milliJoule-energy…
Coherent control of ultrafast quantum phenomena benefits from pulse-shaping capabilities allowing to modulate the envelope and instantaneous phase of optical fields on femtosecond time scales. While such control is available for optical…
High-harmonic spectroscopy driven by circularly-polarized laser pulses and their counter-rotating second harmonic is a new branch of attosecond science which currently lacks quantitative interpretations. We extend this technique to the…
A new physical mechanism to achieve spin-to-orbital angular momentum conversion based on the interaction of an intense circularly polarized (CP) laser beam with a plane foil is presented and studied for the first time. It has been verified…
We study the temporal and spatial dynamics of the large amplitude and frequency modulation that can be induced in an intense, few cycle laser pulse as it propagates through a rapidly ionizing gas. Our calculations include both single atom…
High-order harmonic generation in polyatomic molecules generally involves multiple channels, each associated with a different orbital. Their unambiguous assignment remains a major challenge for high-harmonic spectroscopy. Here we present a…
We propose an effective scheme for the generation of intense coherent extreme ultraviolet light beams carrying orbital angular momentum (OAM). The light is produced by a high-gain harmonic-generation free-electron laser (FEL), seeded using…
Anomalously high generation efficiency of coherent higher field-harmonics in collisions between {\em oppositely charged particles} in the field of femtosecond lasers is predicted. This is based on rigorous numerical solutions of a quantum…
For decades, most research on high harmonic generation (HHG) considered matter as quantum but light as classical, leaving the quantum-optical nature of the harmonics an open question. Here we explore the quantum properties of high…
We demonstrate strong adiabatic laser alignment and mixed-field orientation at kHz repetition rates. We observe degrees of alignment as large as cos\Theta=0.94 at 1 kHz operation for iodobenzene. The experimental setup consist of a kHz…