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A coherent superposition of rotational states in D$_2$ has been excited by nonresonant ultrafast (12 femtosecond) intense (2 $\times$ 10$^{14}$ Wcm$^{-2}$) 800 nm laser pulses leading to impulsive dynamic alignment. Field-free evolution of…

High-harmonic generation is one of the most extreme nonlinear-optical processes observed to date. By focusing an intense laser pulse into a gas, the light-atom interaction that occurs during the process of ionising the atoms results in the…

High-order harmonic generation (HHG) from aligned acetylene molecules interacting with mid infra-red (IR), linearly polarized laser pulses is studied theoretically using a mixed quantum-classical approach in which the electrons are…

Atomic Physics · Physics 2018-05-18 Peter Mulholland , Daniel Dundas

We show that high-order harmonics generated from molecules by intense laser pulses can be expressed as the product of a returning electron wave packet and the photo-recombination cross section (PRCS) where the electron wave packet can be…

Atomic Physics · Physics 2008-04-04 Anh-Thu Le , R. Della Picca , P. D. Fainstein , D. A. Telnov , M. Lein , C. D. Lin

We identify that both the dynamic core polarization and dynamic orbital deformation are important in the orientation-dependent high-harmonic generation of CO molecules subjected to intense few cycle laser fields. These polarization dynamics…

Atomic Physics · Physics 2015-06-19 Bin Zhang , Jianmin Yuan , Zengxiu Zhao

The laser interaction with an electron-positron-ion mixed plasma is studied, from the perspective of the associated high-order harmonic generation. For an idealized mixed plasma which is assumed with a sharp plasma-vacuum interface and…

Plasma Physics · Physics 2021-01-20 W. L. Zhang , T. Grismayer , K. M. Schoeffler , R. A. Fonseca , L. O. Silva

This paper presents the method for the first time to generate intense high-order optical vortices that carry orbital angular momentum in the extreme ultraviolet region. In three-dimensional particle-in-cell simulation, both the reflected…

We present analytically and numerically the spectrum of high harmonic emission generated by twisted electrons in the presence of linearly polarized light. Ensuing transitions from electronic continuum states with orbital angular momentum to…

Atomic Physics · Physics 2019-10-23 Sebastian Gemsheim , Jan-Michael Rost

We study numerically the interaction between an intense circularly polarized laser field and an electron moving in a potential which has a discrete cylindrical symmetry with respect to the laser pulse propagation direction. This setup…

Atomic Physics · Physics 2009-11-07 F. Ceccherini , D. Bauer

Lasers provide intense coherent radiation, essential to cool and trap atoms into a Bose-Einstein condensate or can alternatively drive the non-linear dynamics of high-order harmonic generation. Yet, these two fundamental processes remained…

Quantum Physics · Physics 2025-10-14 Philipp Stammer

We generate high-order harmonics at high pulse repetition rates using a turnkey laser. High-order harmonics at 400 kHz are observed when argon is used as target gas. In neon we achieve generation of photons with energies exceeding 90 eV…

We investigate the orientation dependence of molecular high-order harmonic generation (HHG) both numerically and analytically. We show that the molecular recollision electronic wave packets (REWPs) in the HHG are closely related to the…

Atomic Physics · Physics 2009-11-13 Yanjun. Chen , Yan. Li , Shiping. Yang , Jie. Liu

We present studies of high-order harmonic generation (HHG) at laser intensities well above saturation. We use driving laser pulses which present a particular electron dynamics in the turn-on stage. Our results predict an increasing on the…

Atomic Physics · Physics 2015-06-19 J. A. Pérez-Hernández , M. F. Ciappina , M. Lewenstein , A. Zaïr , L. Roso

High-order harmonic generation (HHG) in the relativistic regime is employed to obtain zeptosecond pulses of $\gamma$-rays. The harmonics are generated from atomic systems in counterpropagating strong attosecond laser pulse trains of linear…

Atomic Physics · Physics 2007-07-20 Michael Klaiber , Karen Z. Hatsagortsyan , Christoph H. Keitel

We present ab initio calculations using the $R$-matrix with time dependence (RMT) method for high-order harmonic generation (HHG) in argon in a short, intense pulse regime. The calculations employ a $6$-cycle $\sin^2$ pulse at $850$ nm with…

Atomic Physics · Physics 2026-04-23 Aaron T. Bondy , Klaus Bartschat

Plasma high harmonics generation from an extremely intense short-pulse laser is explored by including the effects of ion motion, electron-ion collisions and radiation reaction force in the plasma dynamics. The laser radiation pressure…

Plasma Physics · Physics 2017-05-17 Suo Tang , Naveen Kumar , Christoph H. Keitel

Molecular rotational spectroscopy based on strong-field-ionization-induced nitrogen laser is employed to investigate the time evolution of the rotational wave packet composed by a coherent superposition of quantum rotational states created…

High order harmonic (HOH) generation by interacting extremely intense electromagnetic waves in the quantum vacuum is investigated within the framework of the Heisenberg-Euler formalism. We consider here the process in the lowest order of a…

Plasma Physics · Physics 2026-01-13 Pavel Sasorov , Sergei Bulanov

High-order harmonic generation (HHG) is combined with resonant x-ray excitation of a core electron into the transient valence vacancy that is created in the course of the HHG process. To describe this setting, I develop a…

Atomic Physics · Physics 2015-10-15 Christian Buth

High harmonic generation in benzene is studied using a mixed quantum-classical approach in which the electrons are described using time-dependent density functional theory while the ions move classically. The interaction with both…

Atomic Physics · Physics 2016-03-02 Abigail Wardlow , Daniel Dundas
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