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The stability and formation mechanism of the defects relevant to silicon and carbon vacancies at the 4H-SiC(000$\bar{1}$)/SiO$_2$ interface after wet oxidation are investigated by first-principles calculation based on the density functional…

Materials Science · Physics 2024-01-09 Mukai Tsunasaki , Tomoya Ono , Mitsuharu Uemoto

We introduce a first-principles study to clarify the carrier-scattering property at the SiC/SiO$_2$. Interestingly, the electron transport at the conduction-band edge is significantly affected by the introduction of oxygen, even though…

Materials Science · Physics 2017-02-01 Shigeru Iwase , Christopher James Kirkham , Tomoya Ono

Amorphous aluminum oxide Al$_2$O$_3$ (a-Al$_2$O$_3$) layers grown by various deposition techniques contain a significant density of negative charges. In spite of several experimental and theoretical studies, the origin of these charges…

Materials Science · Physics 2019-03-05 Oliver A. Dicks , Jonathon Cottom , Alexander L. Shluger , Valeri V. Afanas'ev

The origin of the apparent negative charge at hydrophobic-water interfaces has fueled one of the biggest debates in physical chemistry for several decades. The most common interpretation given to explain this observation is that negatively…

Chemical Physics · Physics 2020-03-25 Emiliano Poli , Kwang H. Jong , Ali Hassanali

We report first-principles calculations that reveal the atomic forms, stability, and energy levels of carbon-related defects in SiC (0001)/SiO$_{\rm 2}$ systems. We clarify the stable position (SiC side, SiO$_{\rm 2}$ side, or just at the…

Materials Science · Physics 2019-10-15 Takuma Kobayashi , Yu-ichiro Matsushita

Ni-rich cathode materials achieve both high voltages and capacities in Li-ion batteries but are prone to structural instabilities and oxygen loss via the formation of singlet oxygen. Using ab initio molecular dynamics simulations, we…

Silicon carbide (SiC) is an attractive semiconductor material for applications in power electronic devices. However, fabrication of a high-quality SiC/SiO${}_2$ interface has been a challenge. It is well-known that there is a great…

Materials Science · Physics 2018-05-23 So Takamoto , Takahiro Yamasaki , Takahisa Ohno , Chioko Kaneta , Asuka Hatano , Satoshi Izumi

The predictions of the polar catastrophe scenario to explain the occurrence of a metallic interface in heterostructures of the solid solution(LaAlO$_3$)$_{x}$(SrTiO$_3$)$_{1-x}$ (LASTO:x) grown on (001) SrTiO$_3$ were investigated as a…

Surface damage caused by ionizing radiation in SiO$_2$ passivated silicon particle detectors consists mainly of the accumulation of a positively charged layer along with trapped-oxide-charge and interface traps inside the oxide and close to…

Modern electronic devices are unthinkable without the well-controlled formation of interfaces at heterostructures. These often involve at least one amorphous material. Modeling such interfaces poses a significant challenge, since a…

Computational Physics · Physics 2015-06-17 L. E. Hintzsche , C. M. Fang , M. Marsman , M. W. P. E. Lamers , A. W. Weeber , G. Kresse

We report the density-functional calculations that systematically clarify the stable forms of carbon-related defects and their energy levels in amorphous SiO$_2$ using the melt-quench technique in molecular dynamics. Considering the…

Materials Science · Physics 2018-12-03 Yu-ichiro Matsushita , Atsushi Oshiyama

Materials with good carrier mobilities are desired for device applications, but in real devices the mobilities are usually limited by the presence of interfaces and contacts. Mobility degradation at semiconductor-dielectric interfaces is…

Materials Science · Physics 2016-06-13 Xiao Shen , Sokrates T. Pantelides

Identification of microscopic configuration of point defects acting as quantum bits is a key step in the advance of quantum information processing and sensing. Among the numerous candidates, silicon vacancy related centers in silicon…

Materials Science · Physics 2017-11-01 Viktor Ivády , Joel Davidsson , Nguyen Tien Son , Takeshi Ohshima , Igor A. Abrikosov , Adam Gali

The charge transport mechanism of electron via traps in amorphous SiO$_2$ has been studied. Electron transport is limited by phonon-assisted tunneling between traps. Thermal and optical trap energies $W_\mathrm{t}=1.6$ eV,…

Mesoscale and Nanoscale Physics · Physics 2016-08-01 Damir R. Islamov , Vladimir A. Gritsenko , Timofey V. Perevalov , Oleg M. Orlov , Gennady Ya. Krasnikov

A potassium-ion electret, which is a key element of vibration-powered microelectromechanical generators, can store negative charge almost permanently. However, the mechanism by which this negative charge is stored is still unclear. We…

Colossal Ion Conductivity (CIC) is the phenomenon in which large changes in oxygen conductivity are observed when a solid state oxygen electrolyte is placed in a heterolayer super lattice. Several hypotheses have been posed concerning both…

Materials Science · Physics 2019-01-04 M. F. Francis

The dielectric breakdown (BD) of thermal oxide (SiO2) grown on cubic silicon carbide (3C-SiC) was investigated comparing the electrical behavior of macroscopic metal-oxidesemiconductor (MOS) capacitors with nanoscale current and capacitance…

Applied Physics · Physics 2020-05-26 P. Fiorenza , E. Schilirò , F. Giannazzo , C. Bongiorno , M. Zielinski , F. La Via , F. Roccaforte

The total ionizing dose (TID) effect of semiconductor devices stems from radiation-induced $E'_\gamma$ defects in the $a$-SiO$_2$ dielectrics, but the conventional ``hole transport-trapping'' model of defect generation fails to explain…

Materials Science · Physics 2025-09-30 Yu Song , Chen Qiu , Su-Huai Wei

Based on recent first-principles computations in perovskite compounds, especially BaTiO3, we examine the significance of the Born effective charge concept and contrast it with other atomic charge definitions, either static (Mulliken,…

Condensed Matter · Physics 2009-10-31 Ph. Ghosez , J. P. Michenaud , X. Gonze

Certain intrinsic point defects in silicon carbide are promising quantum systems with efficient spin-photon interface. Despite carbon vacancy in silicon carbide is an elementary and relatively abundant intrinsic defect, no optical signal…

Quantum Physics · Physics 2023-05-30 Meysam Mohseni , Péter Udvarhelyi , Gergő Thiering , Adam Gali
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