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We present a theoretical study of the influence of resonant enhancement on quantum path dynamics in the generation of harmonics above and below the ionization threshold in helium. By varying the wavelength and intensity of the driving field…

Atomic Physics · Physics 2015-06-23 Seth Camp , Kenneth J. Schafer , Mette B. Gaarde

Ever since the advent of high-order harmonic generation, one of the main goals has been to maximize the high harmonic yield. This is due to the wide range of applications in multidisciplinary research fields, including nonlinear XUV optics…

We theoretically study high-harmonic generation (HHG) from transition metal elements Mn and Mn$^+$, using full-dimensional, all-electron, first-principles simulations. The HHG spectra calculated with the time-dependent complete-active-space…

Atomic Physics · Physics 2019-06-26 Imam S. Wahyutama , Takeshi Sato , Kenichi L. Ishikawa

The dependence of inter-particle correlations on the orientation of particle relative-momentum can yield unique information on the space-time features of emission in reactions with multiparticle final states. In the present paper, the…

Nuclear Theory · Physics 2008-11-26 Pawel Danielewicz , Scott Pratt

Plasmon resonances are known to amplify the electromagnetic fields near metallic nanostructures. Therefore, they are considered to provide a promising scheme to generate extreme-ultraviolet harmonics, using low power drivings. During…

Isotropic gases irradiated by long pulses of intense IR light can generate very high harmonics of the incident field. It is generally accepted that, due to the symmetry of the generating medium, be it an atomic or an isotropic molecular…

Atomic Physics · Physics 2016-09-28 R. E. F. Silva , P. Rivière , F. Morales , O. Smirnova , M. Ivanov , F. Martín

We demonstrate second and third harmonic generation from a GaP substrate 500{\mu}m thick. The second harmonic field is tuned at the absorption resonance at 335nm, and the third harmonic signal is tuned at 223nm, in a range where the…

Optics · Physics 2015-05-20 V. Roppo , J. Foreman N. Akozbek , M. A. Vincenti , M. Scalora

We theoretically and experimentally investigate orientation-dependent high-harmonic generation (HHG) in zinc oxide subjected to intense femtosecond mid-infrared (MIR) laser pulses. In agreement with past measurements from literature, we…

Classical nonlocality in conducting nanostructures has been shown to dramatically alter the linear optical response, by placing a fundamental limit on the maximum field enhancement that can be achieved. This limit directly extends to all…

Mesoscale and Nanoscale Physics · Physics 2013-11-14 Cristian Ciracì , Michael Scalora , David R. Smith

It is shown that under optimal conditions, the generation of the 3rd, 5th, 7th, and 9th harmonics of the short-wave, ultraviolet or vacuum ultraviolet, laser field by helium atoms is mainly due to transitions between bound states, and the…

A manifestation of electron-hole pairing in nonlinear electromagnetic response of a double layer graphene system is studied. It is shown that the pairing causes the appearance of a number of peaks in the frequency dependence of the…

Strongly Correlated Electrons · Physics 2017-10-20 K. V. Germash , D. V. Fil

We investigate the nonlinear optical response of bulk ZnO under intense short-wave infrared excitation, focusing on the interplay between high-harmonic generation (HHG) and photoluminescence (PL). While HHG exhibits non-perturbative…

A microscopic model of non-reciprocal optical effects in antiferromagnets is developed by considering the case of Cr_2O_3 where such effects have been observed. These effects are due to a direct coupling between light and the…

Condensed Matter · Physics 2009-10-28 V. N. Muthukumar , Roser Valenti , Claudius Gros

The spectral line polarization produced by optically pumped atoms contains a wealth of information on the thermal and magnetic structure of a variety of astrophysical plasmas, including that of the solar atmosphere. A correct decoding of…

Solar and Stellar Astrophysics · Physics 2015-05-30 Luca Belluzzi , Javier Trujillo Bueno

We report measurements and theoretical simulations of high-order harmonic generation (HHG) in aligned N$_2$ molecules using a 1200-nm intense laser field when the generating pulse is perpendicular to the aligning one. With increasing laser…

Bilayer antiferromagnets CrX$_{3}$ (X $=$ Cl, Br, and I) are promising materials for spintronics and optoelectronics that are rooted in their peculiar electronic structures. However, their bands are often hybridized from the interlayer…

Optics · Physics 2024-02-20 Y. Q. Liu , M. S. Si , G. P. Zhang

The radiation of harmonics during the interaction of nonrelativistic electrons with a powerful standing laser wave is studied. Expressions for the harmonic frequencies and the corresponding intensities of the spontaneous radiation are…

General Physics · Physics 2017-10-30 K. S. Badikyan

Two-dimensional materials constitute an exciting platform for nonlinear optics with large nonlinearities that are tunable by gating. Hence, gate-tunable harmonic generation and intensity-dependent refraction have been observed in e.g.…

Mesoscale and Nanoscale Physics · Physics 2019-05-15 F. Hipolito , Darko Dimitrovski , T. G. Pedersen

We propose and theoretically analyse an experimental configuration in which lasers induce 3-spin interactions between trapped ions.By properly choosing the intensities and frequencies of the lasers, 3-spin couplings may be dominant or…

Quantum Physics · Physics 2009-06-10 A. Bermudez , D. Porras , M. A. Martin-Delgado

We show that the dependence of high-order harmonic generation (HHG) on the molecular orientation can be understood within a theoretical treatment that does not involve the strong field of the laser. The results for H_2 show excellent…

Atomic Physics · Physics 2009-11-10 B. Zimmermann , M. Lein , J. M. Rost