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A high-power laser pulse at normal incidence onto a plane solid target will generate odd harmonics of its frequency. However, the spacing of the harmonic lines in this configuration is fixed. Here, we study harmonic generation using two…

Optics · Physics 2025-01-20 Raoul Trines , Holger Schmitz , Martin King , Paul McKenna , Robert Bingham

Due to its linear dispersion, monolayer graphene is expected to generate a third harmonic response at terahertz frequencies. There have been a variety of different models of this effect and recently it has been experimentally observed.…

Mesoscale and Nanoscale Physics · Physics 2022-04-06 Parvin Navaeipour , Marc M. Dignam

Extreme intensity contrast is considered essential for ultraintense, femtosecond laser excitation of solid targets, in particular for studies with structured or ultra-thin targets. Second-harmonic generation has been used to maximize the…

The correlated behavior of electrons determines the structure and optical properties of molecules, semiconductor and other systems. Valuable information on these correlations is provided by measuring the response to femtosecond laser…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Shaul Mukamel , Rafal Oszwaldowski , Lijun Yang

High-order harmonic responses from three $C_{20}$ isomers: fullerene, ring, and bowl, are calculated within the modified Lewenstein model for molecular systems. Spectra for all three structures exhibit intense modulations of the harmonic…

Quantum Physics · Physics 2022-03-31 F. Cajiao - Vélez , A. Jaron

We perform a detailed analysis of high-order harmonic generation in diatomic molecules within the strong-field approximation, with emphasis on quantum-interference effects. Specifically, we investigate how the different types of electron…

Atomic Physics · Physics 2011-11-10 C. Figueira de Morisson Faria

Light generation through optical harmonics plays a pivotal role in photonics, driving innovations in coherent light sources, biological imaging, and spectroscopy. Traditional methods for tuning optical harmonics, including electrostatic…

Optics · Physics 2025-04-01 George Trivizas , Matthew D. Feinstein , Euclides Almeida

Harmonic generation in the limit of ultra-steep density gradients is studied experimentally. Observations demonstrate that while the efficient generation of high order harmonics from relativistic surfaces requires steep plasma density…

In a superconductor the third-harmonic generation (THG) of a strong THz pulse is enhanced below Tc by the resonant excitation of lattice-modulated charge fluctuations (LCF), which modulate the response according to the polarization of the…

Superconductivity · Physics 2018-04-04 T. Cea , P. Barone , C. Castellani , L. Benfatto

High-harmonic generation (HHG) involves the up-conversion of a high-intensity driving field into its harmonic orders. This process is intrinsically non-classical, requiring from quantum mechanics for a complete explanation as, under…

Quantum Physics · Physics 2024-09-25 Javier Rivera-Dean

In recent years, techniques of intense THz laser have enabled us to experimentally observe nonlinear spin dynamics in antiferromagnets since the elementary excitations such as magnons reside on a THz to GHz range in antiferromagnets and THz…

Strongly Correlated Electrons · Physics 2026-04-09 Yuto Jita , Minoru Kanega , Takumi Ogawa , Shunsuke C. Furuya , Masahiro Sato

We report the enhancement of individual harmonics generated at a relativistic ultra-steep plasma vacuum interface. Simulations show the harmonic emission to be due to the coupled action of two high velocity oscillations -- at the…

Electromagnetic emissions, known as Brunel radiations, are produced in plasmas through the coupling between the free electron density and ultrafast ionizing laser pulses. The radiation spectrum generated in laser-gas interactions is here…

Optics · Physics 2025-03-14 Paul David , Fabrice Catoire , Luc Bergé

We investigate the influence of intense, elliptically polarized driving fields on high-order harmonic spectra from aligned diatomic molecules. We derive a generalized two-center interference condition for elliptically polarized fields,…

Atomic Physics · Physics 2015-06-16 T. Das , B. B. Augstein , C. Figueira de Morisson Faria

Asymmetric molecules look different when viewed from one side or the other. This difference influences the electronic structure of the valence electrons, thereby giving stereo sensitivity to chemistry and biology. We show that attosecond…

We present theoretical studies of high-order harmonic generation (HHG) produced by non-homogeneous fields as resulting from the illumination of plasmonic nanostructures with a short laser pulse. We show that both the inhomogeneity of the…

Atomic Physics · Physics 2012-04-27 M. F. Ciappina , J. Biegert , R. Quidant , M. Lewenstein

We generate high-order harmonics of a mid-infrared laser from a silicon single crystal and find their origin in the recollision of coherently accelerated electrons with their holes, analogously to the atomic and molecular case, and to ZnO…

We perform a detailed analysis of high-order harmonic generation (HHG) in atoms within the strong field approximation (SFA) by considering spatially inhomogeneous monochromatic laser fields. We investigate how the individual pairs of…

Atomic Physics · Physics 2015-06-05 T. Shaaran , M. F. Ciappina , M. Lewenstein

We develop a numerical scheme to investigate the high-order harmonic generation (HHG) in intense laser-matter interactions. Tracing the time evolution of every electronic laser-field-free state, we "observe" the HHG in a time-integrated…

Atomic Physics · Physics 2008-11-14 Y. J. Chen , J. Liu , Bambi Hu

We experimentally investigate second harmonic generation from strongly coupled localized and propagative phonon polariton modes in arrays of silicon carbide nanopillars. Our results clearly demonstrate the hybrid nature of the system's…