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Few-layer graphene (FLG) has been predicted to exist in various crystallographic stacking sequences, which can strongly influence the electronic properties of FLG. We demonstrate an accurate and efficient method to characterize stacking…

Materials Science · Physics 2011-02-01 Chun Hung Lui , Zhiqiang Li , Zheyuan Chen , Paul V. Klimov , Louis E. Brus , Tony F. Heinz

This paper reports the experimental determination of the phase-breaking length L of conduction electrons in graphene using Raman spectroscopy. Based on the double-resonance model, we extract L from the spatial dependence of the D band…

Materials Science · Physics 2008-02-27 Luiz Gustavo Cancado , Ryan Beams , Lukas Novotny

Taking into account the constraints imposed by the lattice symmetry, we calculate the phonon dispersion for graphene with interactions between the first, second, and third nearest neighbors in the framework of the Born--von Karman model.…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 L. A. Falkovsky

We present a computational study of the two-phonon Raman spectra of silicene and graphene within a density-functional non-orthogonal tight-binding model. Due to the presence of linear bands close to the Fermi energy in the electronic…

Mesoscale and Nanoscale Physics · Physics 2016-04-29 Valentin N. Popov , Philippe Lambin

A Raman study of a back gated bilayer graphene sample is presented. The changes in the Fermi level induced by charge transfer splits the Raman G-band, hardening its higher component and softening the lower one. These two components are…

Mesoscale and Nanoscale Physics · Physics 2008-12-16 L. M. Malard , D. C. Elias , E. S. Alves , M. A. Pimenta

Phosphorene is a new family member of two-dimensional materials. We observed strong and highly layer-dependent photoluminescence in few-layer phosphorene (2 to 5 layers). The results confirmed the theoretical prediction that few-layer…

Mesoscale and Nanoscale Physics · Physics 2014-09-05 Shuang Zhang , Jiong Yang , Renjing Xu , Fan Wang , Weifeng Li , Muhammad Ghufran , Yong-wei Zhang , Zongfu Yu , Gang Zhang , Qinghua Qin , Yuerui Lu

The magneto-phonon resonance or MPR occurs in semiconductor materials when the energy spacing between Landau levels is continuously tuned to cross the energy of an optical phonon mode. MPRs have been largely explored in bulk semiconductors,…

Materials Science · Physics 2015-06-04 Sarah Goler , Jun Yan , Vittorio Pellegrini , Aron Pinczuk

Magneto-Raman scattering experiments from the surface of graphite reveal novel features associated to purely electronic excitations which are observed in addition to phonon-mediated resonances. Graphene-like and graphite domains are…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 C. Faugeras , M. Amado , P. Kossacki , M. Orlita , M. Kühne , A. A. L. Nicolet , Yu. I. Latyshev , M. Potemski

Layered materials such as graphite and transition metal dichalcogenides have extremely anisotropic mechanical properties owing to orders of magnitude difference between in-plane and out-of-plane interatomic interaction strengths. Although…

Materials Science · Physics 2017-11-10 Jae-Ung Lee , Sungjong Woo , Jaesung Park , Hee Chul Park , Young-Woo Son , Hyeonsik Cheong

Raman spectroscopy is an integral part of graphene research. It is used to determine the number and orientation of layers, the quality and types of edge, and the effects of perturbations, such as electric and magnetic fields, strain,…

Materials Science · Physics 2015-06-16 Andrea C. Ferrari , Denis M. Basko

Relative out of plane displacements of the constituent layers of two dimensional materials gives rise to unique low frequency breathing modes. By computing the height-height correlation functions in momentum space, we show that, the layer…

Materials Science · Physics 2018-05-02 Indrajit Maity , Prabal K Maiti , Manish Jain

Membranes of suspended two-dimensional materials show a large variability in mechanical properties, in part due to static and dynamic wrinkles. As a consequence, experiments typically show a multitude of nanomechanical resonance peaks,…

We describe a peculiar fine structure acquired by the in-plane optical phonon at the Gamma-point in graphene when it is brought into resonance with one of the inter-Landau-level transitions in this material. The effect is most pronounced…

Mesoscale and Nanoscale Physics · Physics 2009-09-24 M. O. Goerbig , J. -N. Fuchs , K. Kechedzhi , Vladimir I. Fal'ko

We present detailed multi frequency resonant Raman measurements of potassium graphite intercalation compounds (GICs). From a well controlled and consecutive in-situ intercalation and high temperature de-intercalation approach the response…

Materials Science · Physics 2013-10-25 J. C. Chacon-Torres , L. Wirtz , T. Pichler

We probe electronic excitations between Landau levels in freestanding $N-$layer graphene over a broad energy range, with unprecedented spectral and spatial resolution, using micro-magneto Raman scattering spectroscopy. A characteristic…

Mesoscale and Nanoscale Physics · Physics 2014-10-03 Stéphane Berciaud , Marek Potemski , Clément Faugeras

The dispersion of electrons and phonons near the K point of bilayer graphene was investigated in a resonant Raman study using different laser excitation energies in the near infrared and visible range. The electronic structure was analyzed…

Mesoscale and Nanoscale Physics · Physics 2011-04-08 D. L. Mafra , L. M. Malard , S. K. Doorn , H. Htoon , J. Nilsson , A. H. Castro Neto , M. A. Pimenta

We report the observation of an intense anomalous peak at 1608 cm$^{-1}$ in the Raman spectrum of graphene associated to the presence of chromium nanoparticles in contact with graphene. Bombardment with an electron beam demonstrates that…

We report two new first-order Raman modes in the spectra of few-layer MoS$_2$ at 286~cm$^{-1}$ and 471~cm$^{-1}$ for excitation energies above 2.4~eV. These modes appear only in few-layer MoS$_2$; therefore their absence provides an easy…

Materials Science · Physics 2015-06-17 Nils Scheuschner , Roland Gillen , Matthias Staiger , Janina Maultzsch

We compare the main feature of the measured Raman scattering spectra from single layer graphene with a bilayer in which the two layers are arbitrarily misoriented. The profiles of the 2D bands are very similar having only one component,…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Philippe Poncharal , Anthony Ayari , Thierry Michel , Jean-Louis Sauvajol

In this letter we use graphene bubbles to study the Raman spectrum of graphene under biaxial (e.g. isotropic) strain. Our Gruneisen parameters are in excellent agreement with the theoretical values. Discrepancy in the previously reported…

Mesoscale and Nanoscale Physics · Physics 2012-01-09 Jakob Zabel , Rahul R. Nair , Anna Ott , Thanasis Georgiou , Andre K. Geim , Kostya S. Novoselov , Cinzia Casiraghi
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