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In this work, we study the Raman spectra of twisted bilayer graphene samples as a function of their twist-angles ($\theta$), ranging from 0.03$^\circ$ to 3.40$^\circ$, where local $\theta$ are determined by analysis of their associated…

Bilayer graphene has been a subject of intense study in recent years. We extend a structural phase field crystal method to include an external potential from adjacent layer(s), which is generated by the corresponding phase field and changes…

Materials Science · Physics 2020-12-24 Kai Liu

Using non-equilibrium molecular dynamics method(NEMD), we have found that the thermal conductivity of multilayer graphene nanoribbons monotonously decreases with the increase of the number of layers, such behavior can be attributed to the…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 Hai-Yuan Cao , Zhi-Xin Guo , Hongjun Xiang , Xin-Gao Gong

Previous Raman measurements on supported graphene under high pressure reported a very different shift rate of in-plane phonon frequency of graphene (16 cm$^{-1}$GPa$^{-1}$) from graphite (4.7 cm$^{-1}$GPa$^{-1}$), implying very different…

Materials Science · Physics 2019-10-02 Y. W. Sun , W. Liu , I. Hernandez , J. Gonzalez , F. Rodriguez , D. J. Dunstan , C. J. Humphreys

Graphene layers placed on SrTiO3 single-crystal substrates were investigated using temperature-dependent confocal Raman spectroscopy. This approach successfully resolved distinct Raman modes of graphene that are often untraceable in…

Materials Science · Physics 2022-09-22 S. Shrestha , C. S. Chang , S. Lee , N. L. Kothalawala , D. Y. Kim , M. Minola , J. Kim , A. Seo

We report that gold thermally deposited onto n-layer graphenes interacts differently with these substrates depending on the number layer, indicating the different surface properties of graphenes. This results in thickness-dependent…

Chemical Physics · Physics 2011-03-24 Haiqing Zhou , Caiyu Qiu , Zheng Liu , Huaichao Yang , Lijun Hu , Ji Liu , Haifang Yang , Changzhi Gu , Lianfeng Sun

Stacking graphene sheets forms graphite. Two in-plane vibrational modes of graphite, E1u and E2g(2), are derived from graphene E2g mode, the shifts of which under compression are all considered as results of in-plane bond shortening. Values…

Mesoscale and Nanoscale Physics · Physics 2015-09-30 Y. W. Sun , D. Holec , D. J. Dunstan

Twisted-bilayer graphene (tBLG) exhibits van Hove singularities in the density of states that can be tuned by changing the twisting angle $\theta$. A $\theta$-defined tBLG has been produced and characterized with optical reflectivity and…

Mesoscale and Nanoscale Physics · Physics 2015-06-22 Ado Jorio , Mark Kasperczyk , Nick Clark , Elke Neu , Patrick Maletinsky , Aravind Vijayaraghavan , Lukas Novotny

Conventional Raman spectroscopy faces inherent limitations in detecting interlayer layer breathing (LB) vibrations with inherently weak electron-phonon coupling or Raman inactivity in two-dimensional materials, hindering insights into…

We study the optical transmittance of multilayer graphene films up to 65 layers thick. By combing large-scale tight-binding simulation and optical measurement on CVD multilayer graphene, the optical transmission through graphene films in…

Materials Science · Physics 2015-06-22 Shou-En Zhu , Shengjun Yuan , G. C. A. M. Janssen

In this paper a systematic examination of graphene/hexagonal boron nitride (g/hBN) bilayers is presented, through a recently developed two-dimensional phase field crystal model that incorporates out-of-plane deformations. The system…

Materials Science · Physics 2023-02-09 K. R. Elder , Zhi-Feng Huang , T. Ala-Nissila

Group theory analysis for two-dimensional elemental systems related to phosphorene is presented, including (i) graphene, silicene, germanene and stanene, (ii) dependence on the number of layers and (iii) two stacking arrangements. Departing…

Mesoscale and Nanoscale Physics · Physics 2016-08-10 J. Ribeiro-Soares , R. M. Almeida , L. G. Cançado , M. S. Dresselhaus , A. Jorio

Many-body effects resulting from strong electron-electron and electron-phonon interactions play a significant role in graphene physics. We report on their manifestation in low B field magneto-phonon resonances in high quality exfoliated…

We study the thermal distribution of phonons in a graphene sheet. Due to the two electronic bands there are two out-of-plane phonon modes with respect to the two sublattices. One of these modes undergoes an Ising transition by spontaneously…

Materials Science · Physics 2011-08-24 K. Ziegler , E. Kogan , E. Majernikova , S. Shpyrko

Kohn anomalies in three-dimensional metallic crystals are dips in the phonon dispersion that are caused by abrupt changes in the screening of the ion-cores by the surrounding electron-gas. These anomalies are also present at the…

Mesoscale and Nanoscale Physics · Physics 2013-11-19 F. Forster , A. Molina-Sanchez , S. Engels , A. Epping , K. Watanabe , T. Taniguchi , L. Wirtz , C. Stampfer

We have implemented a generic method, based on the 2n+1 theorem within density functional perturbation theory, to calculate the anharmonic scattering coefficients among three phonons with arbitrary wavevectors. The method is used to study…

Materials Science · Physics 2014-06-24 Lorenzo Paulatto , Francesco Mauri , Michele Lazzeri

We perform polarization-resolved Raman spectroscopy on graphene in magnetic fields up to 45T. This reveals a filling-factor-dependent, multi-component anticrossing structure of the Raman G peak, resulting from magnetophonon resonances…

Mesoscale and Nanoscale Physics · Physics 2013-06-20 Y. Kim , J. M. Poumirol , A. Lombardo , N. G. Kalugin , T. Georgiou , Y. J. Kim , K. S. Novoselov , A. C. Ferrari , J. Kono , O. Kashuba , V. I. Fal'ko , D. Smirnov

We derive the frequency shifts and the broadening of $\Gamma$ point longitudinal optical (LO) and transverse optical (TO) phonon modes, due to electron-phonon interaction, in graphene under uniaxial strain as a function of the electron…

Mesoscale and Nanoscale Physics · Physics 2015-06-19 Mohamed Assili , Sonia Haddad

We study vibrational states localized at the edges of graphene nanoribbons. Such surface oscillations can be considered as a phonon analog of Tamm states well known in the electronic theory. We consider both armchair and zigzag graphene…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 Alexander V. Savin , Yuri S. Kivshar

$N$-layer transition metal dichalcogenides provide a unique platform to investigate the evolution of the physical properties between the bulk (three dimensional) and monolayer (quasi two-dimensional) limits. Here, using high-resolution…

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