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In this paper, we use density functional theory to calculate the electronic structure and properties of 46 metallic and semi-metallic elements. The binding energy and bond charge model (BBC) model is combined with the tight binding and…

Materials Science · Physics 2023-06-21 Liangjing Ge , Maolin Bo

We present a study of the electronic structure of two laterally coupled gaussian quantum dots filled with two particles. The exact diagonalization method has been used in order to inspect the spatial correlations and examine the particular…

Mesoscale and Nanoscale Physics · Physics 2008-01-29 Jaime Zaratiegui , Pekka Pietilainen , Hong-Yi Chen , Tapash Chakraborty

We report on a many-electron wavefunction theory study for the reaction energetics of hydrogen dissociation on the Si(100) surface. We demonstrate that quantum chemical wavefunction based methods using periodic boundary conditions can…

Materials Science · Physics 2019-01-30 Theodoros Tsatsoulis , Sung Sakong , Axel Groß , Andreas Grüneis

Obtaining the total wavefunction evolution of interacting quantum systems provides access to important properties, such as entanglement, shedding light on fundamental aspects, e.g. quantum energetics and thermodynamics, and guiding towards…

Quantum Physics · Physics 2022-02-02 Maria Maffei , Patrice A. Camati , Alexia Auffèves

Accurate solution of the many-electron problem including correlations remains intractable except for few-electron systems. Describing interacting electrons as a superposition of independent electron configurations results in an apparent…

Computational Physics · Physics 2024-02-20 J. C. Greer

We present the concept, derivation, and implementation of dynamical configuration interaction, a quantum embedding theory that combines Green's function methodology with the many-body wave function. In a strongly-correlated active space, we…

Chemical Physics · Physics 2019-04-03 Marc Dvorak , Patrick Rinke

While the treatment of chemically relevant systems containing hundreds or even thousands of electrons remains beyond the reach of quantum devices, the development of quantum-classical hybrid algorithms to resolve electronic correlation…

We study the formation of molecular states in a two-electron quantum dot as a function of the barrier potential dividing the dot. The increasing barrier potential drives the two electron system from an artificial helium atom to an…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 W. Dybalski , P. Hawrylak

We derive an accurate molecular orbital based expression for the coherent time evolution of a two-electron wave function in a quantum dot molecule where the electrons interact with each other, with external time dependent electromagnetic…

Other Condensed Matter · Physics 2009-11-13 R. Nepstad , L. Sælen , J. P. Hansen

We demonstrate that in semiconductor quantum dots wave functions probed by imaging techniques based on local tunneling spectroscopies like STM show characteristic signatures of electron-electron Coulomb correlation. We predict that such…

Strongly Correlated Electrons · Physics 2007-05-23 Massimo Rontani , Elisa Molinari

We present a new approach to treat correlations in nonequilibrium quantum many-particle system. The method is based on ideas of configuration interaction theory of exact nonperturbative ground state electronic structure calculations. We use…

Mesoscale and Nanoscale Physics · Physics 2014-05-20 Alan A. Dzhioev , D. S. Kosov

The static and dynamic properties of many-body quantum systems are often well described by collective excitations, known as quasiparticles. Engineered quantum systems offer the opportunity to study such emergent phenomena in a precisely…

Quantum Physics · Physics 2015-09-09 P. Jurcevic , P. Hauke , C. Maier , C. Hempel , B. P. Lanyon , R. Blatt , C. F. Roos

Employing a local formula for the electron-electron interaction energy, we derive a self-consistent approximation for the total energy of a general $N$-electron system. Our scheme works as a local variant of the Thomas-Fermi approximation…

Chemical Physics · Physics 2013-10-31 E. Rasanen , A. Odriazola , I. Makkonen , A. Harju

We report the realization of a quadruple quantum dot device in a square-like configuration where a single electron can be transferred on a closed path free of other electrons. By studying the stability diagrams of this system, we…

Mesoscale and Nanoscale Physics · Physics 2012-09-05 Romain Thalineau , Sylain Hermelin , Andreas D. Wieck , Christopher Bäuerle , Laurent Saminadayar , Tristan Meunier

A simple expression for a ground state energy for a two-electron atom is derived. For this, assumption based upon the Niels Bohr ''old'' quantum mechanics idea about electron correlation in a two-electron atom is exploited. Results are…

Quantum Physics · Physics 2007-05-23 M. Auzinsh , R. Damburg

Analytical solutions for a tight-binding model are presented for a position-based qubit and N interacting qubits realized by quasi-one-dimensional network of coupled quantum dots expressed by connected or disconnected graphs of any topology…

Mesoscale and Nanoscale Physics · Physics 2020-08-26 Krzysztof Pomorski , Robert Bogdan Staszewski

The possibility of a novel type of semiconductor quantum dots obtained by spatially modulating the spin-orbit coupling intensity in III-V heterostructures is discussed. Using the effective mass model we predict confined one-electron states…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 M. Valin-Rodriguez , A. Puente , L. Serra

A universal energy eigenvalue equation is proposed in this paper. It is proven that the unique set of eigenfunctions or preferred basis exists for any non-isolated sub-system. Applying the new eigenvalue equation to the relative motion of a…

Quantum Physics · Physics 2026-02-18 Shizhong Mei

The thermopower of few-electron quantum dots with Kondo correlations is investigated via a hierarchial equations of motion approach. The thermopower is determined by the line shape of spectral function within a narrow energy window defined…

Strongly Correlated Electrons · Physics 2015-06-16 LvZhou Ye , Dong Hou , Rulin Wang , Xiao Zheng , YiJing Yan

Quantum entanglement is a concept commonly used with reference to the existence of certain correlations in quantum systems that have no classical interpretation. It is a useful resource to enhance the mutual information of memory channels…

Quantum Physics · Physics 2009-11-13 Tina A. C. Maiolo , Fabio Della Sala , Luigi Martina , Giulio Soliani