Related papers: Coherent Ro-vibrational Revivals in a Thermal Mole…
We study the ultrafast dynamics initiated by a coherent superposition of core-excited states of nitrous oxide molecule. Using high-level \textit{ab-initio} methods, we show that the decoherence caused by the electronic decay and the nuclear…
We analyze collisional decoherence of atoms or molecules prepared in a coherent superposition of nondegenerate internal states at ultralow temperatures and placed in an ultracold buffer gas. Our analysis is applicable for an arbitrary bath…
Molecular hydrogen in silicon has been studied by path-integral molecular dynamics simulations in the canonical ensemble. Finite-temperature properties of these point defects were analyzed in the range from 300 to 900 K. Interatomic…
We investigate the coherence properties of thermal atoms confined in optical dipole traps where the underlying classical dynamics is chaotic. A perturbative expression derived for the coherence of the echo scheme of [Andersen et. al., Phys.…
Ultrafast laser excitation can trigger multiplex coherent dynamics in molecules. Here, we report attosecond transient absorption experiments addressing simultaneous probing of electronic and vibrational dynamics in a prototype molecule,…
The effect of decoherence, induced by spontaneous emission, on the dynamics of cold atoms periodically kicked by an optical lattice is experimentally and theoretically studied. Ideally, the mean energy growth is essentially unaffected by…
We present coherence-enhanced imaging, an in situ technique that uses Raman superradiance to probe the spatial coherence properties of an ultracold gas. Applying this method, we obtain a spatially resolved measurement of the condensate…
It is shown that a nonequilibrium environment can be instrumental in suppressing decoherence between distinct decoherence free subspaces in quantum registers. The effect is found in the framework of exact coherent-product solutions for…
We demonstrate active control of inhomogeneous dephasing and rephasing for single collective atomic spin excitations (spin-waves) created by spontaneous Raman scattering in a quantum memory based on cold $^{87}$Rb atoms. The control is…
We investigate the spin dynamics of a Nitrogen-Vacancy (NV) center contained in an individual diamond nanocrystal in the presence of continuous microwave excitation. Upon periodic reversal of the microwave phase, we observe a train of…
Molecular spins are a versatile platform for quantum sensing. Not only are the spin-bearing molecules themselves widely tunable, they are also capable of being used as sensors as crystals, films and in solution. Using thin-films offers the…
We use an optical centrifuge to excite coherent rotational wave packets in N$_2$O, CS$_2$ and OCS molecules with rotational quantum numbers reaching up to J=465, 690 and 1186, respectively. Time-resolved rotational spectroscopy at such…
Numerical modelling of coherent spin relaxation in nanomagnets, formed by magnetic molecules of high spins, is accomplished. Such a coherent spin dynamics can be realized in the presence of a resonant electric circuit coupled to the magnet.…
We report first ns-resolved absorption measurements of the ro-vibrational excitation of CO$_2$. The high temporal resolution of 8 ns is made possible by a fast detector (rise-time 5 ns), sensitive in the mid-infrared region. The resolution…
In this paper we use the important interferences of Macro-Orbital theory of superfluidity clubbed with several factors that can change the rotational constant (B) and vibrational frequency of N2O in 4HeN-N2O clusters with N to account for…
Rabi nutations of a single electron spin in a single defect center have been detected. The coherent evolution of the spin quantum state is followed via optical detection of the spin state. Coherence times up to several microseconds at room…
We investigate nitrogen-vacancy center (NV) ensembles in diamond under the influence of strongly-correlated electron-spin baths. We thoroughly calculate the decoherence properties of the NV central spin for bath concentrations of 0.1-100…
Coherent resonance is the effect of resonant excitation of nonlinear coherent modes in trapped Bose condensates. This novel effect is shown to be feasible for Bose-condensed trapped gases. Conditions for realizing this effect are derived. A…
The mechanism of decoherence for a quantum system with rotational degrees of freedom is studied. From a simple model of elastic scattering, we show that the non-diagonal density matrix elements of the system exponentially decay. The decay…
We describe a new mechanism of decoherence in excited atoms as a result of thermal particles scattering by the atomic nucleus. It is based on the idea that a single scattering will produce a sudden displacement of the nucleus, which will be…