Related papers: Coherent Ro-vibrational Revivals in a Thermal Mole…
Echo is a ubiquitous phenomenon found in many physical systems, ranging from spins in magnetic fields to particle beams in hadron accelerators. It is typically observed in inhomogeneously broadened ensembles of nonlinear objects, and is…
We report new inelastic Raman and neutron scattering spectra for glasses with different degrees of fragility; the data are compared for each sample to obtain the Raman coupling function $C(\omega)$. The study indicates a general linear…
Probing vibronic coherence in molecules has been a central topic in ultrafast science, as it is an essential prerequisite to monitoring electronic motion. While experiments have demonstrated that attosecond transient absorption spectroscopy…
Molecular magnets are attractive as spin qubits due to their chemical tunability, addressability through electron-spin resonance techniques, and long coherence times. Clock transitions (CTs), for which the system is immune to the effect of…
The effect of temperature dependent asymmetric line broadening is investigated in Cu(NO$_3$)$_2\cdot$2.5D$_2$O, a model material for a 1-D bond alternating Heisenberg chain, using the high resolution neutron-resonance spin-echo (NRSE)…
We demonstrate long rotational coherence of individual polar molecules in the motional ground state of an optical trap. In the present, previously unexplored regime, the rotational eigenstates of molecules are dominantly quantized by…
Coherent dynamics of coupled molecules are effectively characterized by the two-dimensional (2D) electronic coherent spectroscopy. Depending on the coupling between electronic and vibrational states, oscillating signals of purely…
Cooling the rotation and the vibration of molecules by broadband light sources was possible for trapped molecular ions or ultracold molecules. Because of a low power spectral density, the cooling timescale has never fell below than a few…
The dynamics of a spin-1/2 particle coupled to a nuclear spin bath through an isotropic Heisenberg interaction is studied, as a model for the spin decoherence in quantum dots. The time-dependent polarization of the central spin is…
We present a practical method to compute the vibrational resonant Raman spectra in solids with delocalized excitations. We apply this approach to the study of tetrahedrous amorphous carbon. We determine the vibrational eigenmodes and…
A general formalism to describe the dynamics of quantum emitters in structured reservoirs is introduced. As an application, we investigate the optical coherence of an atom-like emitter diagonally coupled via a link-boson to a structured…
We investigate the performance of dynamical decoupling methods at suppressing electron spin decoherence from a low-temperature nuclear spin reservoir in a quantum dot. The controlled dynamics is studied through exact numerical simulation,…
Alignment of OCS, CS$_2$ and I$_2$ molecules embedded in helium nanodroplets is measured as a function of time following rotational excitation by a non-resonant, comparatively weak ps laser pulse. The distinct peaks in the power spectra,…
We study the spectrum of a system of coupled disordered harmonic oscillators in the thermodynamic limit. This Euclidean random matrix ensemble has been suggested as model for the low-temperature vibrational properties of glass. Exact…
We study the storage of coherences in atomic rubidium vapor with a three-level coupling scheme with two ground states and one electronically excited state driven by one optical (control) and one radiofrequency field. We initially store an…
We investigate the collective scattering of coherent light from a thermal alkali-metal vapor with temperatures ranging from 350 to 450 K, corresponding to average atomic spacings between $0.7 \lambda$ and $0.1 \lambda$. We develop a…
Coupling of nuclear and electronic degrees of freedom mediates energy flow in molecules after optical excitation. The associated coherent dynamics in polyatomic systems, however, remain experimentally unexplored. Here, we combined transient…
By implementing four-wave mixing (FWM) micro-spectroscopy we measure coherence and population dynamics of the exciton transitions in monolayers of MoSe$_2$. We reveal their dephasing times T$_2$ and radiative lifetime T$_1$ in a…
Coherent Raman scattering spectroscopy is studied purposely, with the Gaussian ultrashort pulses as a hands-on elucidatory extraction tool of the clean coherent Raman resonant spectra from the overall measured data contaminated with the…
We investigate a number of complex patterns driven by the electro-convection instability in a planarly aligned layer of a nematic liquid crystal. They are traced back to various secondary instabilities of the ideal roll patterns bifurcating…