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When strained beyond the linear regime, soft colloidal glasses yield to steady-state plastic flow in a way that is similar to the deformation of conventional amorphous solids. Due to the much larger size of the colloidal particles with…

Soft Condensed Matter · Physics 2017-04-12 Antina Ghosh , Zoe Budrikis , Vijayakumar Chikkadi , Alessandro Sellerio , Stefano Zapperi , Peter Schall

We report a comprehensive first-principles study of the relative stability of the various possible crystal structures, and the electronic and optical properties of ternary alkali metal chalcogenides ACuX (A= Na/K and X= S/Se/Te) compounds…

Materials Science · Physics 2023-12-27 Gurudayal Behera , Surabhi Suresh Nair , Nirpendra Singh , K. R. Balasubramaniam , Aftab Alam

Solid State Nuclear Magnetic Resonance (NMR) experiments allow characterizing the local structure and dynamics of oxide glasses and melts. Thanks to the development of new experiments, it now becomes possible to evidence not only the…

We report experiments on hard sphere colloidal glasses that reveal a type of shear banding hitherto unobserved in soft glasses. We present a scenario that relates this to an instability arising from shear-concentration coupling, a mechanism…

Soft Condensed Matter · Physics 2015-05-19 R. Besseling , L. Isa , P. Ballesta , G. Petekidis , M. E. Cates , W. C. K. Poon

Background: Semiconductor-doped glasses are treated actively through many years and continue to be of great interest because challenged features of nanosized semiconductors of various chemical nature. Copper chalcogenides have discovered…

Mesoscale and Nanoscale Physics · Physics 2022-11-28 Valerij S. Gurin , Alexander A. Alexeenko

The problems of the intermediate-range atomic structure of glasses and of the mechanism for the glass transition are approached from the low-temperature end in terms of a scenario for the atomic organization that justifies the use of an…

Mesoscale and Nanoscale Physics · Physics 2017-05-30 Giancarlo Jug

Aging in an attraction-driven colloidal glass is studied by computer simulations. The system is equilibrated without attraction and instantaneously ``quenched'', at constant colloid volume fraction, to one of two states beyond the glass…

Soft Condensed Matter · Physics 2015-06-25 Antonio M. Puertas , Matthias Fuchs , Michael E. Cates

Since the discovery of high-temperature superconductivity in the thin-film FeSe/SrTiO$_3$ system, iron selenide and its derivates have been intensively scrutinized. Using ab initio density functional theory calculations we review the…

Superconductivity · Physics 2017-09-07 Daniel Guterding , Harald O. Jeschke , Roser Valenti

The evolution of porous structure and mechanical properties of binary glasses under tensile loading were examined using molecular dynamics simulations. We consider vitreous systems obtained in the process of phase separation after a rapid…

Soft Condensed Matter · Physics 2018-07-19 Nikolai V. Priezjev , Maxim A. Makeev

We present the first experimental characterization in molecular fragile glassformers of a 'prepeak that appears significantly below the main peak of the static structure factor. The temperature and density dependences of this prepeak are…

We here discuss the results of 3d MonteCarlo simulations of a minimal lattice model for gelling systems. We focus on the dynamics, investigated by means of the time autocorrelation function of the density fluctuations and the particle mean…

Soft Condensed Matter · Physics 2007-05-23 E. Del Gado , A. Fierro , L. de Arcangelis , A. Coniglio

The kinetics of homogenization of binary As$_x$Se$_{100-x}$ melts in the As concentration range $0\%$ $<$ $x$ $<$ $50\%$ are followed in FT-Raman profiling experiments, and show that 2 gram sized melts in the middle concentration range…

Materials Science · Physics 2015-06-18 Sriram Ravindren , K. Gunasekera , Z. Tucker , A. Diebold , P. Boolchand , M. Micoulaut

Recent experiments show a strong rotational-diffusion enhancement for self-propelled microrheological probes in colloidal glasses. Here, we provide microscopic understanding using simulations with a frictional probe-medium coupling that…

Soft Condensed Matter · Physics 2020-12-22 Clara Abaurrea-Velasco , Celia Lozano , Clemens Bechinger , Joost de Graaf

We discuss an inverse approach for atomistic modeling of glassy materials. The focus is on structural modeling and electronic properties of hydrogenated amorphous silicon and glassy GeSe2 alloy. The work is based upon a new approach…

Disordered Systems and Neural Networks · Physics 2009-11-13 Parthapratim Biswas , D. A. Drabold

The nonlinear rheological properties of dense suspensions are discussed within simplified models, suggested by a recent first principles approach to the model of Brownian particles in a constant-velocity-gradient solvent flow. Shear…

Soft Condensed Matter · Physics 2015-06-24 Matthias Fuchs , Michael E. Cates

Concentrated colloidal suspensions are a well-tested model system which has a glass transition. Colloids are suspensions of small solid particles in a liquid, and exhibit glassy behavior when the particle concentration is high; the…

Soft Condensed Matter · Physics 2010-10-01 Luca Cipelletti , Eric R. Weeks

We analyze the dependence of relative proportion of various characteristic clusters in binary alcali-borate glasses on modifier's concentration $x$. A pure $B_2O_3$ glass contains a huge amount of boroxol rings and some amount of boron…

Disordered Systems and Neural Networks · Physics 2022-09-07 Richard Kerner , Dina-Maria dos Santos-Loff , Ana Cristina Rosa

Ab initio molecular-dynamics simulations have been used to investigate the structure, dynamics and electronic properties of the liquid alloy Ag(1-x)Se(x) at 1350 K and at the three compositions x=0.33, 0.42 and 0.65. The calculations are…

mtrl-th · Physics 2009-10-30 F. Kirchhoff , J. M. Holender , M. J. Gillan

Using fast confocal microscopy we image the three-dimensional dynamics of particles in a yielded hard-sphere colloidal glass under steady shear. The structural relaxation, observed in regions with uniform shear, is nearly isotropic but is…

Soft Condensed Matter · Physics 2009-11-11 R. Besseling , Eric R. Weeks , A. B. Schofield , W. C. K. Poon

We report the computational investigation of a series of ternary X$_4$Y$_2$Z and X$_5$Y$_2$Z$_2$ compounds with X={Mg, Ca, Sr, Ba}, Y={P, As, Sb, Bi}, and Z={S, Se, Te}. The compositions for these materials were predicted through a search…

Materials Science · Physics 2019-04-03 Maximilian Amsler , Logan Ward , Vinay I. Hegde , Maarten G. Goesten , Xia Yi , Chris Wolverton
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