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Ionic Liquids feature thermophysical properties that are of interest in solvents, energy storage materials and tenable lubrication applications. Recently, a series of coarse grained (CG) models was developed to investigate…

Soft Condensed Matter · Physics 2020-02-19 Oscar Y. Fajardo , Silvia Di Lecce , Fernando Bresme

New ionic liquids (ILs) are continuously introduced involving an increasing number of organic and inorganic ions. Amino acid based ILs (AAILs) represent a specific interest due to their natural origin and, allegedly, low cost. We apply our…

Materials Science · Physics 2014-12-09 Vitaly V. Chaban , Eudes Eterno Fileti

Finding new ionic conductors that enable significant advancements in the development of energy-storage devices is a challenging goal of current material science. Aside of material classes as ionic liquids or amorphous ion conductors, the…

Materials Science · Physics 2015-09-02 K. Geirhos , P. Lunkenheimer , M. Michl , D. Reuter , A. Loidl

Ability to encapsulate molecules is one of the outstanding features of nanotubes. The encapsulation alters physical and chemical properties of both nanotubes and guest species. The latter normally form a separate phase, exhibiting…

Materials Science · Physics 2014-07-23 Vitaly Chaban , Oleg Prezhdo

We investigate the effect of pectin on the structure and ion transport properties of the room-temperature ionic liquid electrolyte 1-n-butyl-3-methylimidazolium hexafluorophosphate ([BMIM][PF6]) using molecular dynamics simulations. We find…

Soft Condensed Matter · Physics 2023-10-03 Sipra Mohapatra , Sougata Halder , Sachin R. Chaudhary , Roland R. Netz , Santosh Mogurampelly

The coexistence curves of liquid-liquid equilibrium (LLE) for the mixtures: phenylacetonitrile + heptane, + octane, + nonane, + cyclooctane, or + 2,2,4-trimethylpentane and for 3-phenylpropionitrile + heptane, or + octane are reported.…

We use molecular dynamics simulations to explore the impact of a non-ionic solvent on the structural and capacitive properties of supercapacitors based on an ionic liquid electrolyte and carbon electrodes. The study is focused on two pure…

Materials Science · Physics 2013-08-27 Céline Merlet , Mathieu Salanne , Benjamin Rotenberg , Paul A Madden

Large ammonia clusters represent a model system of ices which are omnipresent throughout the space. The interaction of ammonia ices with other hydrogen-boding molecules such as methanol or water and their behavior upon an ionization are…

Atomic and Molecular Clusters · Physics 2018-10-15 Michal Fárník , Andriy Pysanenko , Kamila Moriová , Lorenz Ballauf , Paul Scheier , Jan Chalabala , Petr Slavícek

Room temperature ionic liquids (RTILs) are solvent with unusual properties, which are difficult to characterize experimentally because of their intrinsic complexity (large number of atoms, strong Coulomb interactions). Molecular simulations…

Chemical Physics · Physics 2015-06-01 Mathieu Salanne

Room-temperature ionic liquids (RTILs) constitute a fine-tunable class of compounds. Morpholinium-based cations are new to the field. They are promising candidates for electrochemistry, micellization and catalytic applications. We…

Materials Science · Physics 2015-06-01 Vitaly V. Chaban , Oleg V. Prezhdo

We have determined the temperature dependence of the solvation behavior of a large collection of light gases in imidazolium-based Ionic Liquids (ILs) with the help of extensive molecular dynamics simulations. The solubility of molecular…

The static dielectric properties of dense ionic fluids, e.g., room temperature ionic liquids (RTILs) and inorganic fused salts, are investigated on different length scales by means of grandcanonical Monte Carlo simulations. A generally…

Soft Condensed Matter · Physics 2015-05-14 Grigory Zarubin , Markus Bier

In this work, we report the results from molecular dynamics simulations of lithium salt-ionic liquid electrolytes (ILEs) based either on the symmetric bis[(trifluoromethyl)sulfonyl]imide ($\text{TFSI}^-$) anion or its asymmetric analog…

Chemical Physics · Physics 2022-03-23 Alina Wettstein , Diddo Diddens , Andreas Heuer

Parametrizing energy functions for ionic systems can be challenging. Here, the total energy function for an eutectic system consisting of water, SCN$^-$, K$^+$ and acetamide is improved vis-a-vis experimentally measured properties. Given…

Chemical Physics · Physics 2024-10-25 Kai Töpfer , Eric Boittier , Michael Devereux , Andrea Pasti , Peter Hamm , Markus Meuwly

Imidazolium-based ionic liquids are widely used in conjunction with molecular liquids for various applications. Solvation, miscibility and similar properties are of fundamental importance for successful implementation of theoretical…

Chemical Physics · Physics 2015-05-20 Vitaly Chaban

Ionic Liquids (ILs) are organic molten salts characterized by the total absence of solvent. They show remarkable properties: low vapor pressure, high ionic conductivity, high chemical, thermal and electrochemical stability. These…

Ionic liquids (ILs) feature a tailorable and wide range of structural, chemical and electronic properties that make this class of materials suitable to a broad variety of forefront applications in next-generation electronics. Yet, their…

Materials Science · Physics 2022-11-28 Irene Amiehe Essomba , Mauro Boero , Kerstin Falk , Guido Ori

The enthalpy of mixing in the liquid phase is an important property for predicting phase formation in alloys. It can be estimated in a large compositional space from pair wise interactions between elements, for which machine learning has…

Materials Science · Physics 2026-02-10 Quentin Bizot , Ryo Tamura , Guillaume Deffrennes

Among the distinctive structural features of lithium ionic liquids (LILs), a novel class of single-component electrolytes, the variation of the electron-withdrawing group stands out as a key factor in determining their dynamics. To…

Chemical Physics · Physics 2024-02-28 Volodymyr Koverga , Selvaraj S. Chandrasekaran , Anh T. Ngo

Lithium chloride LiCl is widely used as a prototype system to study the strongly dissociated 1-1 electrolyte solution. Here, we combined experimental measurements and classical molecular dynamics simulations to study the ion conduction in…

Soft Condensed Matter · Physics 2019-05-14 Are Yllö , Chao Zhang