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Density functional theory (DFT) calculations are used to study the magnetic and ferroelectric properties of Sr$_{1-x}$Ba$_{x}$MnO$_3$, with focus on $x=0.5$, under isotropic volume expansion/compression and biaxial strain. Our results…

Materials Science · Physics 2020-11-11 Alexander Edström , Claude Ederer

In the scientific description of unconventional transport properties of oxides (spin-dependent transport, superconductivity etc.), the spin-state degree of freedom plays a fundamental role. Because of this, temperature- or magnetic…

Materials Science · Physics 2014-11-12 M. Rotter , Z. -S. Wang , A. T. Boothroyd , D. Prabhakaran , A. Tanaka , M. Doerr

We study energetics and the nature of both homogeneous and mixed spin (MS) states in LaCoO$_3$ incorporating structural changes of the crystal volume expansion and the Co-O bond disproportionation (BD) during the spin-state transition using…

Strongly Correlated Electrons · Physics 2020-05-20 Hyowon Park , Ravindra Nanguneri , Anh T. Ngo

We present a detailed mean-field study to address the fundamental discrepancy in the ground state magnetization of $\mathrm{Sr_{2}CoO_{4}}$ (SCO). In contrast to the ferromagnetic metallic ground state obtained from density functional…

Strongly Correlated Electrons · Physics 2024-01-11 Shivani Bhardwaj , Sudhir K. Pandey

We present combined spin model and first principles electronic structure calculations to study the weak ferromagnetism in bulk Mn$_3$Z (Z=Sn, Ge, Ga) compounds. The spin model parameters were determined from a spin-cluster expansion…

Computational Physics · Physics 2019-10-16 Bendegúz Nyári , András Deák , László Szunyogh

We have studied the electronic structure of BaCoO$_3$ using soft x-ray absorption spectroscopy at the Co-$L_{2,3}$ and O-$K$ edges, magnetic circular dichroism at the Co-$L_{2,3}$ edges, as well as valence band hard x-ray photoelectron…

A single-site dynamical mean field study of a three band model with the rotationally invariant interactions appropriate to the t_2g levels of a transition metal oxide reveals a quantum phase transition between a paramagnetic metallic phase…

Strongly Correlated Electrons · Physics 2008-10-27 Philipp Werner , Emanuel Gull , Matthias Troyer , Andrew J. Millis

We present a thorough $^{77}$Se NMR study of a single crystal of the magnetoelectric compound Cu$_2$OSeO$_3$. The temperature dependence of the local electronic moments extracted from the NMR data is fully consistent with a magnetic phase…

Strongly Correlated Electrons · Physics 2010-09-17 M. Belesi , I. Rousochatzakis , H. C. Wu , H. Berger , I. V. Shvets , F. Mila , J. P. Ansermet

The electronic, magnetic and optical properties of the double perovskite Sr$_2$CoIrO$_6$ (SCIO) under biaxial strain are explored in the framework of density functional theory (DFT) including a Hubbard $U$ term and spin-orbit coupling (SOC)…

Strongly Correlated Electrons · Physics 2021-11-24 Jiongyao Wu , Marcel Ney , Sebastian Esser , Vijaya Begum , Günther Prinz , Axel Lorke , Philipp Gegenwart , Rossitza Pentcheva

We report a study of the local magnetism in thin films of SrRuO3 grown on (111) and (001) oriented SrTiO3 substrates using x-ray magnetic circular dichroism spectroscopy (XMCD) at the Ru-L2,3 edges. The application of the sum rules to the…

We theoretically investigate the ground state magnetic properties of the brownmillerite phase of SrCoO2.5. Strong correlations within Co d electrons are treated within the local spin density approximations of Density Functional theory (DFT)…

Materials Science · Physics 2013-09-23 Chandrima Mitra , Randy S. Fishman , Satoshi Okamoto , Ho Nyung Lee , Fernando A. Reboredo

The spin order in cubic perovskite SrFeO3 and BaFeO3 under high pressure is studied by density functional theory (DFT) calculation with local spin density approximation plus Hubbard U (LSDA+U). At ambient pressure, A-type and G-type helical…

Strongly Correlated Electrons · Physics 2015-06-11 Zhi Li , Toshiaki Iitaka , Takami Tohyama

First-principles calculations to study the electronic and magnetic properties of bulk, oxygen-deficient SrTiO$_3$ (STO) under different doping conditions and densities have been conducted. The appearance of magnetism in oxygen-deficient STO…

Materials Science · Physics 2016-03-30 Alejandro Lopez-Bezanilla , P. Ganesh , Peter B. Littlewood

We have investigated electronic structures of antiferromagnetic YBaCo_2O_5 using the local spin-density approximation (LSDA) + U method. The charge and orbital ordered insulating ground state is correctly obtained with the strong on-site…

Strongly Correlated Electrons · Physics 2009-10-31 S. K. Kwon , B. I. Min

We theoretically study origins of the ferroelectricity in the multiferroic phases of the rare-earth (R) Mn perovskites, RMnO3, by constructing a realistic spin model including the spin-phonon coupling, which reproduces the entire…

Strongly Correlated Electrons · Physics 2011-02-21 Masahito Mochizuki , Nobuo Furukawa , Naoto Nagaosa

We study the magnetic phases of two coupled two-dimensional electron gases in order to determine under what circumstances these phases may occur in real semiconductor quantum wells and what the experimental properties of the broken-symmetry…

Condensed Matter · Physics 2007-05-23 P. I. Tamborenea , R. J. Radtke , S. Das Sarma

Non-adiabatic contribution of environmental degrees of freedom yields effective inertia of spin in effective spin dynamics. In this paper, we study several aspects of the inertia of spin in metallic ferromagnets. (i) a concrete expression…

Mesoscale and Nanoscale Physics · Physics 2015-11-17 Toru Kikuchi , Gen Tatara

Charge dipole moment and spin moment rarely coexist in single-phase bulk materials except in some multiferroics. Despite the progress in the past decade, for most multiferroics their magnetoelectric performance remains poor due to the…

Materials Science · Physics 2015-10-13 P. X. Zhou , S. Dong , H. M. Liu , C. Y. Ma , Z. B. Yan , C. G. Zhong , J. -M. Liu

We have employed one of the well-known many-body techniques, density functional theory plus dynamical mean-field theory (DFT + DMFT), to investigate the electronic structure of ferromagnetic monolayer CrI3 as a function of temperature and…

Materials Science · Physics 2022-04-18 Chang-Jong Kang , Jeonghoon Hong , Jeongwoo Kim

Antiferromagnets with vanishing net magnetization are naturally expected to host higher-order magnetic multipole moments. Understanding and utilizing the multipole degrees of freedom are imperative for novel conceptual designs and…

Materials Science · Physics 2026-04-07 Hua Chen , Guang-Yu Guo , Di Xiao