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While the diffusion of hydrogen on silicon surfaces has been relatively well characterised both experimentally and theoretically, the diffusion around corners between surfaces, as will be found on nanowires and nanostructures, has not been…

Materials Science · Physics 2014-05-19 Richard Smith , Veronika Brazdova , David R. Bowler

The initial steps of MBE growth of GaAs on beta 2-reconstructed GaAs(001) are investigated by performing total energy and electronic structure calculations using density functional theory and a repeated slab model of the surface. We study…

Condensed Matter · Physics 2009-10-31 P. Kratzer , C. G. Morgan , M. Scheffler

We investigate Co nanostructures on Bi$_{2}$Se$_{3}$ by means of scanning tunneling microscopy and spectroscopy [STM/STS], X-ray absorption spectroscopy [XAS], X-ray magnetic dichroism [XMCD] and calculations using the density functional…

Mesoscale and Nanoscale Physics · Physics 2016-03-27 T. Eelbo , M. Sikora , G. Bihlmayer , M. Dobrzański , A. Kozłowski , I. Miotkowski , R. Wiesendanger

Alkali metal atoms (Li, Na, K, Rb, Cs), dimers and (2$\times$2) monolayers on a graphite (0001) surface have been studied using density functional theory, pseudopotentials, and a periodic substrate. The adatoms bind at the hollow site…

Materials Science · Physics 2009-11-11 K. Rytkönen , J. Akola , M. Manninen

We have studied the chemisorption processes of O2 on the (100) surface of uranium using generalized gradient approximation to density functional theory. Dissociative adsorptions of O2 are significantly favored compared to molecular…

Strongly Correlated Electrons · Physics 2015-06-24 M. N. Huda , A. K. Ray

Sodium atoms and clusters (N<5) on graphite (0001) are studied using density functional theory, pseudopotentials and periodic boundary conditions. A single Na atom is observed to bind at a hollow site 2.45 A above the surface with an…

Atomic and Molecular Clusters · Physics 2009-11-10 K. Rytkonen , J. Akola , M. Manninen

We observed 1E 1207.4--5209, a neutron star in the center of the supernova remnant PKS 1209--51/52, with the ACIS detector aboard the Chandra X-ray observatory and detected two absorption features in the source spectrum. The features are…

Astrophysics · Physics 2009-11-07 D. Sanwal , G. G. Pavlov , V. E. Zavlin , M. A. Teter

Vacancies in graphene present sites of altered chemical reactivity and open possibilities to tune graphene properties by defect engineering. The understanding of chemical reactivity of such defects is essential for successful implementation…

Adsorption of $O_{2}$ molecule on Al surface has been a long standing puzzle for the first principles calculation. We have studied the adsorption of $O_{2}$ molecule on the Al(111) surface using hybrid functionals. In contrast to the…

Materials Science · Physics 2012-10-30 Heng-Rui Liu , Hongjun Xiang , X. G. Gong

Adsorption of the molecule CO on metallic surfaces is an important unsolved problem in Kohn-Sham density functional theory (KS-DFT). We present a detailed study of carbon monoxide adsorption on fcc (111) surfaces of 3d, 4d and 5d metals…

Materials Science · Physics 2019-08-07 Abhirup Patra , Haowei Peng , Jianwei Sun , John P. Perdew

We present an ab initio study of the structural and electronic properties of styrene molecules adsorbed on the dimerized Si(100) surface at different coverages, ranging from the single-molecule to the full monolayer. The adsorption…

Soft Condensed Matter · Physics 2009-11-11 A. Calzolari , A. Ruini , M. J. Caldas , E. Molinari

Large scale first-principles calculations based on density functional theory (DFT) employing two different methods (atomic orbitals and plane wave basis sets) were used to study the energetics, geometry, the electronic charge redistribution…

Materials Science · Physics 2010-05-27 Vitaly Alexandrov , Sergei Piskunov , Yuri F. Zhukovskii , Eugene A. Kotomin , Joachim Maier

While the phenomenon of metal substrate adatom incorporation into molecular overlayers is generally believed to occur in several systems, the experimental evidence for this relies on the interpretation of scanning tunnelling microscopy…

Isolated and full monolayer adsorption of various carboranethiol (C$_2$B$_{10}$H$_{12}$S) isomers on gold (111) surface have been investigated using both the standard and van der Waals density functional theoretical calculations. The effect…

Materials Science · Physics 2020-05-20 Ersen Mete , Ayşen Yılmaz , M. Fatih Danışman

We report on a combined scanning tunneling microscopy (STM) and density functional theory (DFT) based investigation of Co atoms on Ge(111)2x1 surfaces. When deposited on cold surfaces, individual Co atoms have a limited diffusivity on the…

Materials Science · Physics 2012-03-14 D. A. Muzychenko , K. Schouteden , M. Houssa , S. V. Savinov , C. Van Haesendonck

We investigate the atomic and electronic structure of a single layer of pentacene on the Au(111) surface using density functional theory. To find the candidate structures we strain match the pentacene crystal geometry with the Au(111)…

Materials Science · Physics 2013-08-06 Kurt Stokbro , Søren Smidstrup

DFT calculation of various atomic species on graphene sheet is investigated as prototypes for formation of nano-structures on carbon nanotube (CNT) wall. We investigate computationally adsorption energies and adsorption sites on graphene…

Materials Science · Physics 2009-11-13 Akira Ishii , Masana Yamamoto , Hiroki Asano , Katsutoshi Fujiwara

We report an experimental refinement of the local charge density at the Si (111) 7x7 surface utilizing a combination of x-ray and high energy electron diffraction. By perturbing about a bond-centered pseudoatom model, we find experimentally…

Materials Science · Physics 2015-05-13 J. Ciston , A. Subramanian , I. K. Robinson , L. D. Marks

When two or more atoms bind to a solid surface, the substrate can mediate an interaction between them. In this paper, we use density-functional theory to quantify the substrate-mediated pair interaction between two adatoms on a…

Materials Science · Physics 2007-05-23 Kristen A. Fichthorn , Matthias Scheffler

Hydrocarbon tribopolymer, a type of polymer formed due to friction between surfaces, is a major impediment to the development of micro- and nanoelectromechanical systems (MEMS/NEMS) devices for industrial application. Tribopolymer buildup…

Materials Science · Physics 2016-12-12 Hyeong-Seok D. Kim , Jing Yang , Yubo Qi , Andrew M. Rappe